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Scale-Up of Physics-Based Models for Predicting Degradation of Large Lithium Ion Batteries

Author

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  • Hong-Keun Kim

    (Department of Mechanical & Aerospace Engineering, Seoul National University, Seoul 151-744, Korea
    Current address: Chemical Sciences and Engineering Division, Argonne National Laboratory, Lemont, IL 60439, USA.)

  • Kyu-Jin Lee

    (Department of Mechanical Engineering, Myongji University, Yongin 448-728, Korea)

Abstract

Large lithium-ion batteries (LIBs) demonstrate different performance and lifetime compared to small LIB cells, owing to the size effects generated by the electrical configuration and property imbalance. However, the calculation time for performing life predictions with three-dimensional (3D) cell models is undesirably long. In this paper, a lumped cell model with equivalent resistances (LER cell model) is proposed as a reduced order model of the 3D cell model, which enables accurate and fast life predictions of large LIBs. The developed LER cell model is validated via the comparisons with results of the 3D cell models by simulating a 20-Ah commercial pouch cell (NCM/graphite) and the experimental values. In addition, the LER cell models are applied to different cell types and sizes, such as a 20-Ah cylindrical cell and a 60-Ah pouch cell.

Suggested Citation

  • Hong-Keun Kim & Kyu-Jin Lee, 2020. "Scale-Up of Physics-Based Models for Predicting Degradation of Large Lithium Ion Batteries," Sustainability, MDPI, vol. 12(20), pages 1-18, October.
    • Handle: RePEc:gam:jsusta:v:12:y:2020:i:20:p:8544-:d:428739
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    References listed on IDEAS

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    Cited by:

    1. Kim, Hong-Keun & Lee, Kyu-Jin, 2023. "Use of a multiphysics model to investigate the performance and degradation of lithium-ion battery packs with different electrical configurations," Energy, Elsevier, vol. 262(PB).

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