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Catalytic Pyrolysis of Wild Reed over a Zeolite-Based Waste Catalyst

Author

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  • Myung Lang Yoo

    (Department of Environmental Engineering, Sunchon National University, 255 Jungang-ro, Suncheon, Jeonnam 57922, Korea)

  • Yong Ho Park

    (Department of Environmental Engineering, Sunchon National University, 255 Jungang-ro, Suncheon, Jeonnam 57922, Korea)

  • Young-Kwon Park

    (School of Environmental Engineering, University of Seoul, Seoul 02504, Korea)

  • Sung Hoon Park

    (Department of Environmental Engineering, Sunchon National University, 255 Jungang-ro, Suncheon, Jeonnam 57922, Korea)

Abstract

Fast catalytic pyrolysis of wild reed was carried out at 500 °C. Waste fluidized catalytic cracking (FCC) catalyst disposed from a petroleum refinery process was activated through acetone-washing and calcination and used as catalyst for pyrolysis. In order to evaluate the catalytic activity of waste FCC catalyst, commercial HY zeolite catalyst with a SiO 2 /Al 2 O 3 ratio of 5.1 was also used. The bio-oil produced from pyrolysis was analyzed using gas chromatography/mass spectrometry (GC/MS). When the biomass-to-catalyst ratio was 1:1, the production of phenolics and aromatics was promoted considerably by catalysis, whereas the content of oxygenates was affected little. Significant conversion of oxygenates to furans and aromatics was observed when the biomass-to-catalyst ratio of 1:10 was used. Activated waste FCC catalyst showed comparable catalytic activity for biomass pyrolysis to HY in terms of the promotion of valuable chemicals, such as furans, phenolics and aromatics. The results of this study imply that waste FCC catalyst can be an important economical resource for producing high-value-added chemicals from biomass.

Suggested Citation

  • Myung Lang Yoo & Yong Ho Park & Young-Kwon Park & Sung Hoon Park, 2016. "Catalytic Pyrolysis of Wild Reed over a Zeolite-Based Waste Catalyst," Energies, MDPI, vol. 9(3), pages 1-9, March.
    • Handle: RePEc:gam:jeners:v:9:y:2016:i:3:p:201-:d:65785
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    References listed on IDEAS

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    1. Jin, Sung Ho & Lee, Hyung Won & Ryu, Changkook & Jeon, Jong-Ki & Park, Young-Kwon, 2015. "Catalytic fast pyrolysis of Geodae-Uksae 1 over zeolites," Energy, Elsevier, vol. 81(C), pages 41-46.
    2. Kirubakaran, V. & Sivaramakrishnan, V. & Nalini, R. & Sekar, T. & Premalatha, M. & Subramanian, P., 2009. "A review on gasification of biomass," Renewable and Sustainable Energy Reviews, Elsevier, vol. 13(1), pages 179-186, January.
    3. Choi, Suek Joo & Park, Sung Hoon & Jeon, Jong-Ki & Lee, In Gu & Ryu, Changkook & Suh, Dong Jin & Park, Young-Kwon, 2013. "Catalytic conversion of particle board over microporous catalysts," Renewable Energy, Elsevier, vol. 54(C), pages 105-110.
    4. Park, Young-Kwon & Yoo, Myung Lang & Heo, Hyeon Su & Lee, Hyung Won & Park, Sung Hoon & Jung, Sang-Chul & Park, Sang-Sook & Seo, Seong-Gyu, 2012. "Wild reed of Suncheon Bay: Potential bio-energy source," Renewable Energy, Elsevier, vol. 42(C), pages 168-172.
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    2. Jacek Grams & Agnieszka M. Ruppert, 2017. "Development of Heterogeneous Catalysts for Thermo-Chemical Conversion of Lignocellulosic Biomass," Energies, MDPI, vol. 10(4), pages 1-25, April.

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