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Experimental Study of Oil Non-Condensable Gas Pyrolysis in a Stirred-Tank Reactor for Catalysis of Hydrogen and Hydrogen-Containing Mixtures Production

Author

Listed:
  • Oleg A. Kolenchukov

    (Department of Technological Machines and Equipment of Oil and Gas Complex, School of Petroleum and Natural Gas Engineering, Siberian Federal University, 660041 Krasnoyarsk, Russia)

  • Kirill A. Bashmur

    (Department of Technological Machines and Equipment of Oil and Gas Complex, School of Petroleum and Natural Gas Engineering, Siberian Federal University, 660041 Krasnoyarsk, Russia)

  • Vladimir V. Bukhtoyarov

    (Department of Technological Machines and Equipment of Oil and Gas Complex, School of Petroleum and Natural Gas Engineering, Siberian Federal University, 660041 Krasnoyarsk, Russia
    Digital Material Science, New Materials and Technologies, Bauman Moscow State Technical University, 105005 Moscow, Russia)

  • Sergei O. Kurashkin

    (Digital Material Science, New Materials and Technologies, Bauman Moscow State Technical University, 105005 Moscow, Russia
    Information-Control Systems Department, Institute of Computer Science and Telecommunications, Reshetnev Siberian State University of Science and Technology, 660037 Krasnoyarsk, Russia
    Laboratory of Biofuel Compositions, Siberian Federal University, 660041 Krasnoyarsk, Russia)

  • Vadim S. Tynchenko

    (Department of Technological Machines and Equipment of Oil and Gas Complex, School of Petroleum and Natural Gas Engineering, Siberian Federal University, 660041 Krasnoyarsk, Russia
    Digital Material Science, New Materials and Technologies, Bauman Moscow State Technical University, 105005 Moscow, Russia
    Information-Control Systems Department, Institute of Computer Science and Telecommunications, Reshetnev Siberian State University of Science and Technology, 660037 Krasnoyarsk, Russia)

  • Elena V. Tsygankova

    (Department of Foreign Languages for Natural Science, Siberian Federal University, 660041 Krasnoyarsk, Russia)

  • Roman B. Sergienko

    (Machine Learning Department, Gini Gmbh, 80339 Munich, Germany)

  • Vladislav V. Kukartsev

    (Digital Material Science, New Materials and Technologies, Bauman Moscow State Technical University, 105005 Moscow, Russia
    Department of Informatics, Institute of Space and Information Technologies, Siberian Federal University, 660041 Krasnoyarsk, Russia
    Department of Information Economic Systems, Institute of Engineering and Economics, Reshetnev Siberian State University of Science and Technology, 660037 Krasnoyarsk, Russia)

Abstract

The present study is focused on improving the technology for deep oil sludge processing by pyrolysis methods, considered to be the most promising technology for their environmentally friendly utilization, in which a significant yield of fuel products is expected. The technology developed by the authors of this study is a two-stage process. The first stage, pyrolysis of oil sludge, was investigated in previous papers. A significant yield of non-condensable gases was obtained. This paper presents a study of the second stage of complex deep processing technology—pyrolysis of non-condensable gases (purified propane) using a stirrer with the help of the developed experimental setup. The expected benefit of using the stirrer is improved heat transfer due to circumferential and radial-axial circulation of the gas flow. The effect of a stirrer on the yield of final target decomposition products—H 2 -containing mixtures and H 2 generated during non-catalytic (medium-temperature) and catalytic pyrolysis of non-condensable gases obtained by pyrolysis of oil sludge are estimated. Ni catalyst was used for catalytic pyrolysis. The study shows that the application of the stirrer leads to increasing in H 2 -containing mixtures and H 2 concentrations. In particular, during the whole reaction time (10 h), the average H 2 concentration in pyrolysis gas during catalytic pyrolysis increased by ~5.3%. In this case, the optimum reaction time to produce H 2 was 4 h. The peak H 2 concentration in the pyrolysis gas at reaction temperature 590 ± 10 °C was: 66.5 vol. % with the stirrer versus 62 vol. % without the stirrer with an error of ±0.4 %. A further increase in reaction time is cost-effective in order to obtain H 2 -containing mixtures.

Suggested Citation

  • Oleg A. Kolenchukov & Kirill A. Bashmur & Vladimir V. Bukhtoyarov & Sergei O. Kurashkin & Vadim S. Tynchenko & Elena V. Tsygankova & Roman B. Sergienko & Vladislav V. Kukartsev, 2022. "Experimental Study of Oil Non-Condensable Gas Pyrolysis in a Stirred-Tank Reactor for Catalysis of Hydrogen and Hydrogen-Containing Mixtures Production," Energies, MDPI, vol. 15(22), pages 1-16, November.
    • Handle: RePEc:gam:jeners:v:15:y:2022:i:22:p:8346-:d:966772
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    References listed on IDEAS

    as
    1. Malek Msheik & Sylvain Rodat & Stéphane Abanades, 2021. "Methane Cracking for Hydrogen Production: A Review of Catalytic and Molten Media Pyrolysis," Energies, MDPI, vol. 14(11), pages 1-35, May.
    2. Klinger, Jordan L. & Westover, Tyler L. & Emerson, Rachel M. & Williams, C. Luke & Hernandez, Sergio & Monson, Glen D. & Ryan, J. Chadron, 2018. "Effect of biomass type, heating rate, and sample size on microwave-enhanced fast pyrolysis product yields and qualities," Applied Energy, Elsevier, vol. 228(C), pages 535-545.
    3. Kirill A. Bashmur & Oleg A. Kolenchukov & Vladimir V. Bukhtoyarov & Vadim S. Tynchenko & Sergei O. Kurashkin & Elena V. Tsygankova & Vladislav V. Kukartsev & Roman B. Sergienko, 2022. "Biofuel Technologies and Petroleum Industry: Synergy of Sustainable Development for the Eastern Siberian Arctic," Sustainability, MDPI, vol. 14(20), pages 1-25, October.
    4. Anton Maximov & Aslan Tsivadze & Alexander Fridman & Tatyana Kuchinskaya & Alexander Novikov & Maxim Shabanov & Evgeny Naranov, 2020. "The Prospects for Processing Reservoir Oil Sludge into Hydrocarbons by Low-Temperature Hydrogenation in Sorbing Electrochemical Matrices in Comparison with Conventional High-Temperature Hydrocracking," Energies, MDPI, vol. 13(20), pages 1-12, October.
    5. Umair Yaqub Qazi, 2022. "Future of Hydrogen as an Alternative Fuel for Next-Generation Industrial Applications; Challenges and Expected Opportunities," Energies, MDPI, vol. 15(13), pages 1-40, June.
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