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Development of Honeycomb Methanation Catalyst and Its Application in Power to Gas Systems

Author

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  • Philipp Biegger

    (Montanuniversitaet Leoben, Chair of Process Technology and Industrial Environmental Protection, Franz-Josef-Strasse 18, 8700 Leoben, Austria)

  • Florian Kirchbacher

    (Institute of Chemical, Environmental and Bioscience Engineering, Vienna University of Technology, Getreidemarkt 9/166, 1060 Vienna, Austria)

  • Ana Roza Medved

    (Montanuniversitaet Leoben, Chair of Process Technology and Industrial Environmental Protection, Franz-Josef-Strasse 18, 8700 Leoben, Austria)

  • Martin Miltner

    (Institute of Chemical, Environmental and Bioscience Engineering, Vienna University of Technology, Getreidemarkt 9/166, 1060 Vienna, Austria)

  • Markus Lehner

    (Montanuniversitaet Leoben, Chair of Process Technology and Industrial Environmental Protection, Franz-Josef-Strasse 18, 8700 Leoben, Austria)

  • Michael Harasek

    (Institute of Chemical, Environmental and Bioscience Engineering, Vienna University of Technology, Getreidemarkt 9/166, 1060 Vienna, Austria)

Abstract

Fluctuating energy sources require enhanced energy storage demand, in order to ensure safe energy supply. Power to gas offers a promising pathway for energy storage in existing natural gas infrastructure, if valid regulations are met. To improve interaction between energy supply and storage, a flexible power to gas process is necessary. An innovative multibed methanation concept, based on ceramic honeycomb catalysts combined with polyimide membrane gas upgrading, is presented in this study. Cordierite monoliths are coated with γ -Al 2 O 3 and catalytically active nickel, and used in a two-stage methanation process at different operation conditions ( p = 6–14 bar, GHSV = 3000–6000 h −1 ). To fulfill the requirements of the Austrian natural gas network, the product gas must achieve a CH 4 content of ≥96 vol %. Hence, CH 4 rich gas from methanation is fed to the subsequent gas upgrading unit, to separate remaining H 2 and CO 2 . In the present study, two different membrane modules were investigated. The results of methanation and gas separation clearly indicate the high potential of the presented process. At preferred operation conditions, target concentration of 96 vol % CH 4 can be achieved.

Suggested Citation

  • Philipp Biegger & Florian Kirchbacher & Ana Roza Medved & Martin Miltner & Markus Lehner & Michael Harasek, 2018. "Development of Honeycomb Methanation Catalyst and Its Application in Power to Gas Systems," Energies, MDPI, vol. 11(7), pages 1-17, June.
    • Handle: RePEc:gam:jeners:v:11:y:2018:i:7:p:1679-:d:154841
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    References listed on IDEAS

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    1. Sun, Qie & Li, Hailong & Yan, Jinying & Liu, Longcheng & Yu, Zhixin & Yu, Xinhai, 2015. "Selection of appropriate biogas upgrading technology-a review of biogas cleaning, upgrading and utilisation," Renewable and Sustainable Energy Reviews, Elsevier, vol. 51(C), pages 521-532.
    2. Kirchbacher, Florian & Biegger, Philipp & Miltner, Martin & Lehner, Markus & Harasek, Michael, 2018. "A new methanation and membrane based power-to-gas process for the direct integration of raw biogas – Feasability and comparison," Energy, Elsevier, vol. 146(C), pages 34-46.
    3. Scholz, Marco & Melin, Thomas & Wessling, Matthias, 2013. "Transforming biogas into biomethane using membrane technology," Renewable and Sustainable Energy Reviews, Elsevier, vol. 17(C), pages 199-212.
    4. Collet, Pierre & Flottes, Eglantine & Favre, Alain & Raynal, Ludovic & Pierre, Hélène & Capela, Sandra & Peregrina, Carlos, 2017. "Techno-economic and Life Cycle Assessment of methane production via biogas upgrading and power to gas technology," Applied Energy, Elsevier, vol. 192(C), pages 282-295.
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    Cited by:

    1. Philipp Wolf-Zoellner & Ana Roza Medved & Markus Lehner & Nina Kieberger & Katharina Rechberger, 2021. "In Situ Catalytic Methanation of Real Steelworks Gases," Energies, MDPI, vol. 14(23), pages 1-22, December.
    2. Saman Setoodeh Jahromy & Felix Birkelbach & Christian Jordan & Clemens Huber & Michael Harasek & Andreas Werner & Franz Winter, 2019. "Impact of Partial Pressure, Conversion, and Temperature on the Oxidation Reaction Kinetics of Cu 2 O to CuO in Thermochemical Energy Storage," Energies, MDPI, vol. 12(3), pages 1-15, February.
    3. Sayama, Shogo & Yamamoto, Seiji, 2022. "A 6-kW thermally self-sustained two-stage CO2 methanation reactor: design and experimental evaluation of steady-state performance under full-load conditions," Applied Energy, Elsevier, vol. 325(C).
    4. Jing Liu & Wei Sun & Gareth P. Harrison, 2019. "Optimal Low-Carbon Economic Environmental Dispatch of Hybrid Electricity-Natural Gas Energy Systems Considering P2G," Energies, MDPI, vol. 12(7), pages 1-17, April.

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