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Metal oxide (MgO, CaO, and La2O3) promoted Ni-Ce0.8Zr0.2O2 catalysts for H2 and CO production from two major greenhouse gases

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  • Jang, Won-Jun
  • Jeong, Dae-Woon
  • Shim, Jae-Oh
  • Kim, Hak-Min
  • Han, Won-Bi
  • Bae, Jong Wook
  • Roh, Hyun-Seog

Abstract

The metal oxide (MgO, CaO, and La2O3) promoted Ni-Ce0.8Zr0.2O2 catalysts have been applied for carbon dioxide reforming of methane (CDR) reaction and investigated the coke formation and sintering phenomenon in used catalysts. The Ni-MgO-Ce0.8Zr0.2O2 catalyst exhibits high activity and stability at a very high gas hourly space velocity of 480,000 h−1, resulting from high resistance to coke formation and Ni sintering. This is mainly due to small Ni crystallite size, strong basicity of MgO, and an intimate interaction between Ni and MgO.

Suggested Citation

  • Jang, Won-Jun & Jeong, Dae-Woon & Shim, Jae-Oh & Kim, Hak-Min & Han, Won-Bi & Bae, Jong Wook & Roh, Hyun-Seog, 2015. "Metal oxide (MgO, CaO, and La2O3) promoted Ni-Ce0.8Zr0.2O2 catalysts for H2 and CO production from two major greenhouse gases," Renewable Energy, Elsevier, vol. 79(C), pages 91-95.
    • Handle: RePEc:eee:renene:v:79:y:2015:i:c:p:91-95
    DOI: 10.1016/j.renene.2014.08.032
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    References listed on IDEAS

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    1. Roh, Hyun-Seog & Eum, Ic-Hwan & Jeong, Dae-Woon, 2012. "Low temperature steam reforming of methane over Ni–Ce(1−x)Zr(x)O2 catalysts under severe conditions," Renewable Energy, Elsevier, vol. 42(C), pages 212-216.
    2. Jeong, Dae-Woon & Jang, Won-Jun & Shim, Jae-Oh & Han, Won-Bi & Roh, Hyun-Seog & Jung, Un Ho & Yoon, Wang Lai, 2014. "Low-temperature water–gas shift reaction over supported Cu catalysts," Renewable Energy, Elsevier, vol. 65(C), pages 102-107.
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    Cited by:

    1. Jang, Won-Jun & Jeong, Dae-Woon & Shim, Jae-Oh & Kim, Hak-Min & Roh, Hyun-Seog & Son, In Hyuk & Lee, Seung Jae, 2016. "Combined steam and carbon dioxide reforming of methane and side reactions: Thermodynamic equilibrium analysis and experimental application," Applied Energy, Elsevier, vol. 173(C), pages 80-91.
    2. Park, Min-Ju & Kim, Hak-Min & Gu, Yun-Jeong & Jeong, Dae-Woon, 2023. "Optimization of biogas-reforming conditions considering carbon formation, hydrogen production, and energy efficiencies," Energy, Elsevier, vol. 265(C).
    3. Jeon, Kyung-Won & Shim, Jae-Oh & Jang, Won-Jun & Lee, Da-We & Na, Hyun-Suk & Kim, Hak-Min & Lee, Yeol-Lim & Yoo, Seong-Yeun & Roh, Hyun-Seog & Jeon, Byong-Hun & Bae, Jong Wook & Ko, Chang Hyun, 2019. "Effect of calcination temperature on the association between free NiO species and catalytic activity of Ni−Ce0.6Zr0.4O2 deoxygenation catalysts for biodiesel production," Renewable Energy, Elsevier, vol. 131(C), pages 144-151.

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