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Catalytic co-pyrolysis of torrefied poplar wood and high-density polyethylene over hierarchical HZSM-5 for mono-aromatics production

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  • Lin, Xiaona
  • Kong, Lingshuai
  • Ren, Xiajin
  • Zhang, Donghong
  • Cai, Hongzhen
  • Lei, Hanwu

Abstract

The catalytic co-pyrolysis of torrefied poplar wood sawdust (TPW) and high-density polyethylene (HDPE) was investigated over hierarchical HZSM-5. Compared with raw PW/HDPE, the bio-oil yield from co-pyrolysis of TPW/HDPE decreased gradually while the quality of bio-oil was upgraded. With increasing torrefaction temperature from 220 to 280 °C, the amounts of acids, furans, and anhydrosugars in bio-oil were significantly reduced due to the removal of hemicellulose, whereas the production of phenols and alkenes were improved due to the enhanced hydrogen transfer reaction. In the catalytic co-pyrolysis, increasing torrefaction temperature caused an enhanced production of mono-aromatics as well as the selectivity of BTX (benzene, toluene, and xylene). Nevertheless, severe torrefaction (280 °C) lead to a rapid reduction of aromatic yield and selectivity due to the loss of cellulose. Compared to parent HZSM-5, hierarchical HZSM-5 treated with alkaline concentration (0.2–0.3 mol/L) favored the formation of mono-aromatics at the expense of polyaromatics. The maximum mono-aromatics yield of 71.75% was obtained during catalytic co-pyrolysis of 260-TPW/HDPE over 0.3-HZSM-5. The present work suggests that torrefaction pretreatment followed by the catalysis of hierarchical HZSM-5 is an efficient way to promote the production of valuable mono-aromatic hydrocarbons from biomass and plastic wastes.

Suggested Citation

  • Lin, Xiaona & Kong, Lingshuai & Ren, Xiajin & Zhang, Donghong & Cai, Hongzhen & Lei, Hanwu, 2021. "Catalytic co-pyrolysis of torrefied poplar wood and high-density polyethylene over hierarchical HZSM-5 for mono-aromatics production," Renewable Energy, Elsevier, vol. 164(C), pages 87-95.
    • Handle: RePEc:eee:renene:v:164:y:2021:i:c:p:87-95
    DOI: 10.1016/j.renene.2020.09.071
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    References listed on IDEAS

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    1. Álvarez, Ana & Nogueiro, Dositeo & Pizarro, Consuelo & Matos, María & Bueno, Julio L., 2018. "Non-oxidative torrefaction of biomass to enhance its fuel properties," Energy, Elsevier, vol. 158(C), pages 1-8.
    2. Xin, Shanzhi & Mi, Tie & Liu, Xiaoye & Huang, Fang, 2018. "Effect of torrefaction on the pyrolysis characteristics of high moisture herbaceous residues," Energy, Elsevier, vol. 152(C), pages 586-593.
    3. Zhang, Yayun & Duan, Dengle & Lei, Hanwu & Villota, Elmar & Ruan, Roger, 2019. "Jet fuel production from waste plastics via catalytic pyrolysis with activated carbons," Applied Energy, Elsevier, vol. 251(C), pages 1-1.
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    3. Zhang, Jun & Li, Chengyu & Yuan, Haoran & Chen, Yong, 2022. "Enhancement of aromatics production via cellulose fast pyrolysis over Ru modified hierarchical zeolites," Renewable Energy, Elsevier, vol. 184(C), pages 280-290.

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