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Functionalized graphene/poly(3,4-ethylenedioxythiophene):polystyrenesulfonate as counter electrode catalyst for dye-sensitized solar cells

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  • Yue, Gentian
  • Wu, Jihuai
  • Xiao, Yaoming
  • Lin, Jianming
  • Huang, Miaoliang
  • Lan, Zhang
  • Fan, Leqing

Abstract

A (grapheme/poly(3,4-ethylenedioxythiophene):polystyrenesulfonate) graphene/PEDOT:PSS composite film was electrodeposited on fluorine-doped tin oxide conductive substrate by one-step electrochemical polymerization method. The low-cost and platinum-free film was used as counter electrode in (dye-sensitized solar cell) DSSC. The cyclic voltammetry, electrochemical impedance spectroscopy and Tafel measurements indicate that the graphene/PEDOT:PSS composite film has low charge-transfer resistance on the electrolyte/electrode interface and high catalytic activity for the reduction of triiodide to iodide and. As a result, the DSSC based on the graphene/PEDOT:PSS counter electrode showed high power conversion efficiency of 7.86% under a simulated sunlight illumination of 100 mW cm−2 (AM 1.5), which is comparable with the performance of the DSSC based on Pt counter electrode (7.31%).

Suggested Citation

  • Yue, Gentian & Wu, Jihuai & Xiao, Yaoming & Lin, Jianming & Huang, Miaoliang & Lan, Zhang & Fan, Leqing, 2013. "Functionalized graphene/poly(3,4-ethylenedioxythiophene):polystyrenesulfonate as counter electrode catalyst for dye-sensitized solar cells," Energy, Elsevier, vol. 54(C), pages 315-321.
    • Handle: RePEc:eee:energy:v:54:y:2013:i:c:p:315-321
    DOI: 10.1016/j.energy.2013.01.037
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    References listed on IDEAS

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    1. Kaushika, N.D. & Rai, Anil K., 2007. "An investigation of mismatch losses in solar photovoltaic cell networks," Energy, Elsevier, vol. 32(5), pages 755-759.
    2. Francis, L. & Sreekumaran Nair, A. & Jose, R. & Ramakrishna, S. & Thavasi, V. & Marsano, E., 2011. "Fabrication and characterization of dye-sensitized solar cells from rutile nanofibers and nanorods," Energy, Elsevier, vol. 36(1), pages 627-632.
    3. Diker, Halide & Varlikli, Canan & Mizrak, Koray & Dana, Aykutlu, 2011. "Characterizations and photocatalytic activity comparisons of N-doped nc-TiO2 depending on synthetic conditions and structural differences of amine sources," Energy, Elsevier, vol. 36(2), pages 1243-1254.
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    Cited by:

    1. Han, Chaoling & Chen, Zhenqian, 2021. "Study on the synergism of thermal transport and electrochemical of PEMFC based on N, P co-doped graphene substrate electrode," Energy, Elsevier, vol. 214(C).
    2. Wang, Guanxi & Xiao, Wei & Yu, Jiaguo, 2015. "High-efficiency dye-sensitized solar cells based on electrospun TiO2 multi-layered composite film photoanodes," Energy, Elsevier, vol. 86(C), pages 196-203.
    3. Wang, Kai & Li, Liwei & Zhang, Tiezhu & Liu, Zaifei, 2014. "Nitrogen-doped graphene for supercapacitor with long-term electrochemical stability," Energy, Elsevier, vol. 70(C), pages 612-617.
    4. Yue, Gentian & Wang, Lei & Zhang, Xin'an & Wu, Jihuai & Jiang, Qiwei & Zhang, Weifeng & Huang, Miaoliang & Lin, Jianming, 2014. "Fabrication of high performance multi-walled carbon nanotubes/polypyrrole counter electrode for dye-sensitized solar cells," Energy, Elsevier, vol. 67(C), pages 460-467.

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