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A combination of acetic acid and deep eutectic solvent pretreatment on poplar for coproduction of bioethanol, bio-oil and energy recovery

Author

Listed:
  • Xu, Xiaojie
  • Zhang, Shiyu
  • Gai, Junming
  • Xie, Xinyu
  • Wu, Shufang
  • Hu, Jinguang
  • Song, Kai
  • Chu, Qiulu

Abstract

This work proposed an acetic acid (AC) pre-hydrolysis and a deep eutectic solvent (DES) post-delignification strategy for efficient fractionation of hemicellulose and lignin from lignocellulosic biomass, providing an easily hydrolyzed cellulose, which could be effectively converted to ethanol through semi-simultaneous saccharification and fermentation (SSSF) process. Results showed that, 11.20 kg xylo-oligosaccharides (XOSs), 19.91 kg ethanol and 25.89 kg lignin could be produced from lignocellulosic biorefinery based on the AC-DES pretreatment of 100 kg poplar. In addition, the lignin recovered from DES showed the potential as feedstock for production of hydrocarbon enriched bio-oil by pyrolysis. Higher heating values (HHV) of 27.19 MJ/kg and 31.56 MJ/kg for oil were measured, after pyrolysis of DES lignin and DES lignin/low-density polyethylene (LDPE) with ratio of 7:3, respectively. Finally, mass balance and energy analysis revealed that, lignocellulosic biorefinery based on AC-DES combined pretreatment to co-produce XOSs, bioerthanol and DES lignin could achieve an energy recovery of 78 %.

Suggested Citation

  • Xu, Xiaojie & Zhang, Shiyu & Gai, Junming & Xie, Xinyu & Wu, Shufang & Hu, Jinguang & Song, Kai & Chu, Qiulu, 2024. "A combination of acetic acid and deep eutectic solvent pretreatment on poplar for coproduction of bioethanol, bio-oil and energy recovery," Energy, Elsevier, vol. 313(C).
    • Handle: RePEc:eee:energy:v:313:y:2024:i:c:s0360544224037344
    DOI: 10.1016/j.energy.2024.133956
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    References listed on IDEAS

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    1. Veronika Jančíková & Michal Jablonský, 2024. "Exploiting Deep Eutectic Solvent-like Mixtures for Fractionation Biomass, and the Mechanism Removal of Lignin: A Review," Sustainability, MDPI, vol. 16(2), pages 1-22, January.
    2. Kim, Kwang Ho & Kim, Tae-Seung & Lee, Soo-Min & Choi, Donha & Yeo, Hwanmyeong & Choi, In-Gyu & Choi, Joon Weon, 2013. "Comparison of physicochemical features of biooils and biochars produced from various woody biomasses by fast pyrolysis," Renewable Energy, Elsevier, vol. 50(C), pages 188-195.
    3. Xu, Ling-Hua & Ma, Cheng-Ye & Zhang, Chen & Xu, Ying & Wen, Jia-Long & Yuan, Tong-Qi, 2022. "An integrated acetic acid-catalyzed hydrothermal-pretreatment (AAP) and rapid ball-milling for producing high-yield of xylo-oligosaccharides, fermentable glucose and lignin from poplar wood," Renewable Energy, Elsevier, vol. 201(P1), pages 691-699.
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