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Study of lead-free perovskite photoconverting structures by impedance spectroscopy

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  • Aleksandrova, M.P.

Abstract

In this paper, the impedance spectroscopy technique is applied to study the charge dynamics across the bulk and at the interfaces at elevated temperatures for a novel photoelectric element, consisting of the lead-free perovskite material. The results show that the device performance degrades at a temperature of 54 °C, but at a temperature of 35 °C traps are thermally activated in the perovskite layer. As a result, the charge transport resistance is dependent on the signal frequency and the interfacial capacitance associated with charge accumulation increases. At elevated temperatures, the high-frequency plots are related to the photon-induced charges, while at low frequencies the ions transfer and space charge accumulation affect the processes in the photoelectric element. Based on the measurements conducted, it is possible to propose an equivalent electric circuit that can be used to quantify important material parameters and to understand loss mechanisms for different solar cell architectures. New information was provided about the temperature limitations and critical thermal threshold where physical degradation of the lead-free perovskite occurred.

Suggested Citation

  • Aleksandrova, M.P., 2023. "Study of lead-free perovskite photoconverting structures by impedance spectroscopy," Energy, Elsevier, vol. 273(C).
    • Handle: RePEc:eee:energy:v:273:y:2023:i:c:s0360544223005352
    DOI: 10.1016/j.energy.2023.127141
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    References listed on IDEAS

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    1. Wolfgang Tress & Konrad Domanski & Brian Carlsen & Anand Agarwalla & Essa A. Alharbi & Michael Graetzel & Anders Hagfeldt, 2019. "Performance of perovskite solar cells under simulated temperature-illumination real-world operating conditions," Nature Energy, Nature, vol. 4(7), pages 568-574, July.
    2. Han Chen & Fei Ye & Wentao Tang & Jinjin He & Maoshu Yin & Yanbo Wang & Fengxian Xie & Enbing Bi & Xudong Yang & Michael Grätzel & Liyuan Han, 2017. "A solvent- and vacuum-free route to large-area perovskite films for efficient solar modules," Nature, Nature, vol. 550(7674), pages 92-95, October.
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