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Fouling propensity in reverse electrodialysis operated with hypersaline brine

Author

Listed:
  • Santoro, Sergio
  • Tufa, Ramato Ashu
  • Avci, Ahmet Halil
  • Fontananova, Enrica
  • Di Profio, Gianluca
  • Curcio, Efrem

Abstract

The impact of fouling on the performance of Reverse Electrodialysis operated with highly concentrated brine is a poorly investigated area. In this work, the fouling propensity and stability of Ion Exchange Membranes (IEMs), developed by Fujifilm Manufacturing Europe BV (The Netherlands), is investigated under the condition of seawater and brine. The fouling propensity of the IEMs was depicted by the determination of the Gibbs energy barrier of based-on the Classical Nucleation along with the Theoretical modeling of heterogeneous nucleation as a function of electrochemical (contact angle, permittivity, charge density) and morphological (roughness) membrane properties validated by CaCO3 precipitation. Results indicate that Cation Exchange Membranes (CEM) are more susceptible to the scaling due to the reduced energy barrier of heterogeneous nucleation. FTIR-ATR analysis on six months-aged membranes samples indicated a partial modification in the chemical structure of Anion Exchange Membranes (AEM) induced by the organic fouling associated with humic substances. The tensile tests demonstrated substantial mechanical stability of IEMs. Lab-scale RED tests operated with artificial brine over 30 days showed a significant increase in pressure drop through feed channels due to significant colloidal fouling along with a 23% reduction of maximum gross power density with consequent decrease of net power density.

Suggested Citation

  • Santoro, Sergio & Tufa, Ramato Ashu & Avci, Ahmet Halil & Fontananova, Enrica & Di Profio, Gianluca & Curcio, Efrem, 2021. "Fouling propensity in reverse electrodialysis operated with hypersaline brine," Energy, Elsevier, vol. 228(C).
    • Handle: RePEc:eee:energy:v:228:y:2021:i:c:s0360544221008124
    DOI: 10.1016/j.energy.2021.120563
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    1. Tufa, Ramato Ashu & Pawlowski, Sylwin & Veerman, Joost & Bouzek, Karel & Fontananova, Enrica & di Profio, Gianluca & Velizarov, Svetlozar & Goulão Crespo, João & Nijmeijer, Kitty & Curcio, Efrem, 2018. "Progress and prospects in reverse electrodialysis for salinity gradient energy conversion and storage," Applied Energy, Elsevier, vol. 225(C), pages 290-331.
    2. Karasu, Seçkin & Altan, Aytaç & Bekiros, Stelios & Ahmad, Wasim, 2020. "A new forecasting model with wrapper-based feature selection approach using multi-objective optimization technique for chaotic crude oil time series," Energy, Elsevier, vol. 212(C).
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