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Lab-scale experimental tests of power to gas-oxycombustion hybridization: System design and preliminary results

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  • Bailera, Manuel
  • Peña, Begoña
  • Lisbona, Pilar
  • Marín, Julián
  • Romeo, Luis M.

Abstract

Power-to-Gas (PtG) represents one of the most promising energy storage technologies. PtG converts electricity surplus into synthetic natural gas by combining water electrolysis and CO2 methanation. This technology valorises captured CO2 to produce a ‘carbon neutral’ natural gas, while allowing temporal displacement of renewable energy. PtG-Oxycombustion hybridization is proposed to integrate mass and energy flows of the global system. Oxygen, comburent under oxy-fuel combustion, is commonly produced in an air separation unit. This unit can be replaced by an electrolyser which by-produces O2 reducing the electrical consumption and the energy penalty of the carbon separation process. The aim of this work is to present the design, construction and testing of a methanation reactor at laboratory scale to increase the knowledge of the key component of this system. Experimental data are used to validate the theoretical kinetic model at different operating temperatures implemented in Aspen Plus. CO2 conversions about 60–80% are found for catalyst temperature between 350 and 550 °C. These values agree well with expected theoretical conversions from the kinetic model.

Suggested Citation

  • Bailera, Manuel & Peña, Begoña & Lisbona, Pilar & Marín, Julián & Romeo, Luis M., 2021. "Lab-scale experimental tests of power to gas-oxycombustion hybridization: System design and preliminary results," Energy, Elsevier, vol. 226(C).
    • Handle: RePEc:eee:energy:v:226:y:2021:i:c:s0360544221006241
    DOI: 10.1016/j.energy.2021.120375
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    References listed on IDEAS

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    1. Bailera, Manuel & Lisbona, Pilar & Romeo, Luis M. & Espatolero, Sergio, 2017. "Power to Gas projects review: Lab, pilot and demo plants for storing renewable energy and CO2," Renewable and Sustainable Energy Reviews, Elsevier, vol. 69(C), pages 292-312.
    2. Neubert, Michael & Hauser, Alexander & Pourhossein, Babak & Dillig, Marius & Karl, Juergen, 2018. "Experimental evaluation of a heat pipe cooled structured reactor as part of a two-stage catalytic methanation process in power-to-gas applications," Applied Energy, Elsevier, vol. 229(C), pages 289-298.
    3. Bailera, Manuel & Lisbona, Pilar & Romeo, Luis M. & Espatolero, Sergio, 2016. "Power to Gas–biomass oxycombustion hybrid system: Energy integration and potential applications," Applied Energy, Elsevier, vol. 167(C), pages 221-229.
    4. Götz, Manuel & Lefebvre, Jonathan & Mörs, Friedemann & McDaniel Koch, Amy & Graf, Frank & Bajohr, Siegfried & Reimert, Rainer & Kolb, Thomas, 2016. "Renewable Power-to-Gas: A technological and economic review," Renewable Energy, Elsevier, vol. 85(C), pages 1371-1390.
    5. Eveloy, Valerie, 2019. "Hybridization of solid oxide electrolysis-based power-to-methane with oxyfuel combustion and carbon dioxide utilization for energy storage," Renewable and Sustainable Energy Reviews, Elsevier, vol. 108(C), pages 550-571.
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    1. Katla, Daria & Węcel, Daniel & Jurczyk, Michał & Skorek-Osikowska, Anna, 2023. "Preliminary experimental study of a methanation reactor for conversion of H2 and CO2 into synthetic natural gas (SNG)," Energy, Elsevier, vol. 263(PD).
    2. Romeo, Luis M. & Cavana, Marco & Bailera, Manuel & Leone, Pierluigi & Peña, Begoña & Lisbona, Pilar, 2022. "Non-stoichiometric methanation as strategy to overcome the limitations of green hydrogen injection into the natural gas grid," Applied Energy, Elsevier, vol. 309(C).
    3. Máté Zavarkó & Attila R. Imre & Gábor Pörzse & Zoltán Csedő, 2021. "Past, Present and Near Future: An Overview of Closed, Running and Planned Biomethanation Facilities in Europe," Energies, MDPI, vol. 14(18), pages 1-27, September.
    4. Bailera, Manuel & Lisbona, Pilar & Peña, Begoña & Alarcón, Andreina & Guilera, Jordi & Perpiñán, Jorge & Romeo, Luis M., 2022. "Synthetic natural gas production in a 1 kW reactor using Ni–Ce/Al2O3 and Ru–Ce/Al2O3: Kinetics, catalyst degradation and process design," Energy, Elsevier, vol. 256(C).
    5. García-Luna, S. & Ortiz, C. & Carro, A. & Chacartegui, R. & Pérez-Maqueda, L.A., 2022. "Oxygen production routes assessment for oxy-fuel combustion," Energy, Elsevier, vol. 254(PB).

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