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Investigation of functionalized carbon nanotubes' performance on carbon dioxide hydrate formation

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  • Nashed, Omar
  • Partoon, Behzad
  • Lal, Bhajan
  • Sabil, Khalik M.
  • Shariff, Azmi Mohd

Abstract

In this work, the impact of functional group on the thermodynamics and kinetics of CO2 hydrates are investigated experimentally. The hydroxylated multi-wall carbon nanotubes (OH-MWCNT) and carboxylated carbon nanotubes (COOH-MWCNT) along with pristine carbon nanotubes (MWCNT) are selected for this study. The carbon nanotubes are suspended in a 0.03 wt% sodium dodecyl sulfate (SDS) aqueous solution and the results are compared with SDS aqueous solution at the same concentration of 0.03 wt% and deionized water. The CO2 hydrate phase boundary and kinetic parameters of CO2 hydrate formation including induction time, the initial rate and amount of gas consumed, gas uptake, storage capacity, and water to hydrates conversion are studied. The results show that the nanofluids studied do not affect the equilibrium conditions of CO2 hydrates. In addition, 0.01 and 0.05 wt% of COOH-MWCNT mixed with 0.03 wt% SDS showed highest initial hydrate formation rate and gas uptake. Furthermore, a comparison between SDS and COOH-MWCNT (without stabilizer SDS) at 0.03 wt% revealed that addition of COOH-MWCNT to the water enhance the initial hydrates formation rate compared to SDS.

Suggested Citation

  • Nashed, Omar & Partoon, Behzad & Lal, Bhajan & Sabil, Khalik M. & Shariff, Azmi Mohd, 2019. "Investigation of functionalized carbon nanotubes' performance on carbon dioxide hydrate formation," Energy, Elsevier, vol. 174(C), pages 602-610.
    • Handle: RePEc:eee:energy:v:174:y:2019:i:c:p:602-610
    DOI: 10.1016/j.energy.2019.02.193
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    References listed on IDEAS

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    Cited by:

    1. Zhang, Fengyuan & Wang, Xiaolin & Lou, Xia & Lipiński, Wojciech, 2021. "The effect of sodium dodecyl sulfate and dodecyltrimethylammonium chloride on the kinetics of CO2 hydrate formation in the presence of tetra-n-butyl ammonium bromide for carbon capture applications," Energy, Elsevier, vol. 227(C).
    2. Wang, Xiaolin & Zhang, Fengyuan & Lipiński, Wojciech, 2020. "Research progress and challenges in hydrate-based carbon dioxide capture applications," Applied Energy, Elsevier, vol. 269(C).
    3. Liu, Ni & Chen, Litao & Liu, Caixia & Yang, Liang & Liu, Daoping, 2020. "Experimental study of carbon dioxide hydrate formation in the presence of graphene oxide," Energy, Elsevier, vol. 211(C).
    4. Cheng, Chuanxiao & Lai, Zhengxiang & Jin, Tingxiang & Jing, Zhiyong & Geng, Wangning & Qi, Tian & Zhu, Shiquan & Zhang, Jun & Liu, Jianxiu & Wang, Fan & Dong, Hongsheng & Zhang, Lunxiang, 2022. "Rapid nucleation and growth of tetrafluoroethane hydrate in the cyclic process of boiling–condensation," Energy, Elsevier, vol. 256(C).
    5. Liu, Fa-Ping & Li, Ai-Rong & Qing, Sheng-Lan & Luo, Ze-Dong & Ma, Yu-Ling, 2022. "Formation kinetics, mechanism of CO2 hydrate and its applications," Renewable and Sustainable Energy Reviews, Elsevier, vol. 159(C).
    6. Nguyen, Ngoc N. & La, Vinh T. & Huynh, Chinh D. & Nguyen, Anh V., 2022. "Technical and economic perspectives of hydrate-based carbon dioxide capture," Applied Energy, Elsevier, vol. 307(C).

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