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Analysis of catalytic pyrolysis of municipal solid waste and paper sludge using TG-FTIR, Py-GC/MS and DAEM (distributed activation energy model)

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  • Fang, Shiwen
  • Yu, Zhaosheng
  • Ma, Xiaoqian
  • Lin, Yan
  • Chen, Lin
  • Liao, Yanfen

Abstract

In this work, an analysis of co-pyrolysis municipal solid waste and paper sludge with additive (MgO) were investigated by TG-FTIR and Py-GC/MS. The proportions of paper sludge in the blends were 10%, 30% and 50%, respectively. The pyrolysis characteristics, the yields of pollutants (CO, SO2, NO, HCl) and CO2, the products and chemical composition, the kinetic behaviors and the distribution activation energy model were investigated. After adding paper sludge, the sums of pollutants reduced, the amount of aliphatic hydrocarbons decreased and oxygenates compounds increased. After adding MgO, the results showed that the residue mass decreased, the emission of pollutants reduced, the ratio of aliphatic hydrocarbons became larger, the ratio of oxygenates compounds became smaller, and the activation energy reduced. According to the beforementioned results, the 30% percentage of paper sludge in the mixture with MgO might be the most suitable ratio for co-pyrolysis.

Suggested Citation

  • Fang, Shiwen & Yu, Zhaosheng & Ma, Xiaoqian & Lin, Yan & Chen, Lin & Liao, Yanfen, 2018. "Analysis of catalytic pyrolysis of municipal solid waste and paper sludge using TG-FTIR, Py-GC/MS and DAEM (distributed activation energy model)," Energy, Elsevier, vol. 143(C), pages 517-532.
    • Handle: RePEc:eee:energy:v:143:y:2018:i:c:p:517-532
    DOI: 10.1016/j.energy.2017.11.038
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    5. Kumar, Akash & Yan, Beibei & Tao, Junyu & Li, Jian & Kumari, Lata & Oba, Belay Tafa & Aborisade, Moses Akintayo & Chen, Guanyi, 2022. "Influence of waste plastic on pyrolysis of low-lipid microalgae: A study on thermokinetics, behaviors, evolved gas characteristics, and products distribution," Renewable Energy, Elsevier, vol. 185(C), pages 416-430.
    6. Kumar, Aman & Singh, Ekta & Mishra, Rahul & Lo, Shang Lien & Kumar, Sunil, 2023. "Global trends in municipal solid waste treatment technologies through the lens of sustainable energy development opportunity," Energy, Elsevier, vol. 275(C).
    7. Sun, Hao & Bi, Haobo & Jiang, Chunlong & Ni, Zhanshi & Tian, Junjian & Zhou, Wenliang & Qiu, Zhicong & Lin, Qizhao, 2022. "Experimental study of the co-pyrolysis of sewage sludge and wet waste via TG-FTIR-GC and artificial neural network model: Synergistic effect, pyrolysis kinetics and gas products," Renewable Energy, Elsevier, vol. 184(C), pages 1-14.
    8. Fang, Shiwen & Lin, Yousheng & Lin, Yan & Chen, Shu & Shen, Xiangyang & Zhong, Tianming & Ding, Lixing & Ma, Xiaoqian, 2020. "Influence of ultrasonic pretreatment on the co-pyrolysis characteristics and kinetic parameters of municipal solid waste and paper mill sludge," Energy, Elsevier, vol. 190(C).
    9. Gu, Tianbao & Fu, Zhufu & Berning, Torsten & Li, Xuantian & Yin, Chungen, 2021. "A simplified kinetic model based on a universal description for solid fuels pyrolysis: Theoretical derivation, experimental validation, and application demonstration," Energy, Elsevier, vol. 225(C).
    10. Fang, Shiwen & Deng, Zhengbing & Lin, Yan & Huang, Zhen & Ding, Lixing & Deng, Lisheng & Huang, Hongyu, 2021. "Nitrogen migration in sewage sludge chemical looping gasification using copper slag modified by NiO as an oxygen carrier," Energy, Elsevier, vol. 228(C).
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