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Hydrogenation improvement of TiFe by adding ZrMn2

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  • Lv, Peng
  • Huot, Jacques

Abstract

In this paper, we report the microstructure and hydrogen storage properties of TiFe + x wt.%ZrMn2 (x = 2, 4, 8, 12) alloys prepared by arc melting. Each alloy was made of two phases: a TiFe phase with very small amount of zirconium and manganese, and a second phase which has a higher proportion of zirconium and manganese. We found that the first hydrogenation kinetics increase with x. This is most likely due to the presence of zirconium-rich secondary phase that acts as a gateway for hydrogen to enter the main TiFe phase. Pressure-composition isotherms also show that increasing x decreases the absorption plateau pressure. Moreover, for x = 12, air exposure had a minimal impact on hydrogen absorption behaviour. Finally, we found that cold rolling has minimal effect on the activation kinetics of TiFe + x wt.%ZrMn2 (x = 4) alloy.

Suggested Citation

  • Lv, Peng & Huot, Jacques, 2017. "Hydrogenation improvement of TiFe by adding ZrMn2," Energy, Elsevier, vol. 138(C), pages 375-382.
    • Handle: RePEc:eee:energy:v:138:y:2017:i:c:p:375-382
    DOI: 10.1016/j.energy.2017.07.072
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    References listed on IDEAS

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    1. Yang, Tai & Wang, Peng & Li, Qiang & Xia, Chaoqun & Yin, Fuxing & Liang, Chunyong & Zhang, Yanghuan, 2018. "Hydrogen absorption and desorption behavior of Ni catalyzed Mg–Y–C–Ni nanocomposites," Energy, Elsevier, vol. 165(PA), pages 709-719.
    2. Liu, Jingjing & Cheng, Honghui & Han, Shumin & Liu, Hongfei & Huot, Jacques, 2020. "Hydrogen storage properties and cycling degradation of single-phase La0.60R0.15Mg0·25Ni3.45 alloys with A2B7-type superlattice structure," Energy, Elsevier, vol. 192(C).
    3. Chen, X.Y. & Chen, R.R. & Ding, X. & Fang, H.Z. & Li, X.Z. & Ding, H.S. & Su, Y.Q. & Guo, J.J. & Fu, H.Z., 2019. "Effect of phase formation on hydrogen storage properties in Ti-V-Mn alloys by zirconium substitution," Energy, Elsevier, vol. 166(C), pages 587-597.
    4. Wu, Zhen & Zhu, Pengfei & Yao, Jing & Tan, Peng & Xu, Haoran & Chen, Bin & Yang, Fusheng & Zhang, Zaoxiao & Ni, Meng, 2020. "Thermo-economic modeling and analysis of an NG-fueled SOFC-WGS-TSA-PEMFC hybrid energy conversion system for stationary electricity power generation," Energy, Elsevier, vol. 192(C).

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