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Atomic layer deposition of yttria-stabilized zirconia thin films for enhanced reactivity and stability of solid oxide fuel cells

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  • Park, Joonho
  • Lee, Yeageun
  • Chang, Ikwhang
  • Cho, Gu Young
  • Ji, Sanghoon
  • Lee, Wonyoung
  • Cha, Suk Won

Abstract

We report the advantages of atomic layer deposition (ALD) for the fabrication of yttria-stabilized zirconia (YSZ) electrolyte. The reactivity and stability of anodic aluminum oxide (AAO)-based thin-film solid oxide fuel cells (SOFCs) are improved by applying ALD YSZ electrolyte. The fuel cell fabricated by ALD shows a peak power density of 154.6 mW cm−2 at 450 °C, whereas the fuel cell fabricated by sputtering demonstrates a peak power density of 66.2 mW cm−2. The amorphous and nanogranular microstructure of the ALD YSZ film is ascribed for a significant improvement in the cathodic reactivity of the AAO-based thin-film fuel cells. Moreover, the smooth and uniform surface of the ALD YSZ electrolytes mitigates the agglomeration of the Pt cathode layer, and thus the thermal stability of the thin-film fuel cell is remarkably improved at 450 °C.

Suggested Citation

  • Park, Joonho & Lee, Yeageun & Chang, Ikwhang & Cho, Gu Young & Ji, Sanghoon & Lee, Wonyoung & Cha, Suk Won, 2016. "Atomic layer deposition of yttria-stabilized zirconia thin films for enhanced reactivity and stability of solid oxide fuel cells," Energy, Elsevier, vol. 116(P1), pages 170-176.
    • Handle: RePEc:eee:energy:v:116:y:2016:i:p1:p:170-176
    DOI: 10.1016/j.energy.2016.09.094
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    References listed on IDEAS

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    1. Zongping Shao & Sossina M. Haile, 2004. "A high-performance cathode for the next generation of solid-oxide fuel cells," Nature, Nature, vol. 431(7005), pages 170-173, September.
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    3. Paek, Jun Yeol & Chang, Ikwhang & Park, Joon Ho & Ji, Sanghoon & Cha, Suk Won, 2014. "A study on properties of yttrium-stabilized zirconia thin films fabricated by different deposition techniques," Renewable Energy, Elsevier, vol. 65(C), pages 202-206.
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    5. Chang, Ikwhang & Bae, Jiwoong & Park, Joonho & Lee, Sunho & Ban, Myeongseok & Park, Taehyun & Lee, Yoon Ho & Song, Han Ho & Kim, Young-Beom & Cha, Suk Won, 2016. "A thermally self-sustaining solid oxide fuel cell system at ultra-low operating temperature (319 °C)," Energy, Elsevier, vol. 104(C), pages 107-113.
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    Cited by:

    1. Lee, Yeageun & Park, Joonho & Yu, Wonjong & Tanveer, Waqas Hassan & Lee, Yoon Ho & Cho, Gu Young & Park, Taehyun & Zheng, Chunhua & Lee, Wonyoung & Cha, Suk Won, 2018. "Nickel-based bilayer thin-film anodes for low-temperature solid oxide fuel cells," Energy, Elsevier, vol. 161(C), pages 1133-1138.
    2. Cho, Gu Young & Lee, Yoon Ho & Yu, Wonjong & An, Jihwan & Cha, Suk Won, 2019. "Optimization of Y2O3 dopant concentration of yttria stabilized zirconia thin film electrolyte prepared by plasma enhanced atomic layer deposition for high performance thin film solid oxide fuel cells," Energy, Elsevier, vol. 173(C), pages 436-442.
    3. Lee, Sanghoon & Lee, Yeageun & Park, Joonho & Yu, Wonjong & Cho, Gu Young & Kim, Yusung & Cha, Suk Won, 2019. "Effect of plasma-enhanced atomic layer deposited YSZ inter-layer on cathode interface of GDC electrolyte in thin film solid oxide fuel cells," Renewable Energy, Elsevier, vol. 144(C), pages 123-128.

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