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Investigations of the temperature distribution in proton exchange membrane fuel cells

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  • Jung, Chi-Young
  • Shim, Hyo-Sub
  • Koo, Sang-Man
  • Lee, Sang-Hwan
  • Yi, Sung-Chul

Abstract

A two-dimensional, non-isothermal model of a proton exchange membrane fuel cell was implemented to elucidate heat balance through the membrane electrode assembly (MEA). To take local utilization of platinum catalyst into account, the model was presented by considering the formation of agglomerated catalyst structure in the electrodes. To estimate energy balance through the MEA, various modes of heat generation and depletion by reversible/irreversible heat release, ohmic heating and phase change of water were included in the present model. In addition, dual-pathway kinetics, that is a combination of Heyrovsky–Volmer and Tafel–Volmer kinetics, were employed to precisely describe the hydrogen oxidation reaction. The proposed model was validated with experimental cell polarization, resulting in excellent fit. The temperature distribution inside the MEA was analyzed by the model. Consequently, a thorough investigation was made of the relation between membrane thickness and the temperature distribution inside the MEA.

Suggested Citation

  • Jung, Chi-Young & Shim, Hyo-Sub & Koo, Sang-Man & Lee, Sang-Hwan & Yi, Sung-Chul, 2012. "Investigations of the temperature distribution in proton exchange membrane fuel cells," Applied Energy, Elsevier, vol. 93(C), pages 733-741.
    • Handle: RePEc:eee:appene:v:93:y:2012:i:c:p:733-741
    DOI: 10.1016/j.apenergy.2011.08.035
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    1. Trongchuankij, Wiruyn & Pruksathorn, Kejvalee & Hunsom, Mali, 2011. "Preparation of a high performance Pt-Co/C electrocatalyst for oxygen reduction in PEM fuel cell via a combined process of impregnation and seeding," Applied Energy, Elsevier, vol. 88(3), pages 974-980, March.
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    Cited by:

    1. Yang, Wonseok & Cha, Dowon & Kim, Yongchan, 2019. "Effects of flow direction on dynamic response and stability of nonhumidification PEM fuel cell," Energy, Elsevier, vol. 185(C), pages 386-395.
    2. Wang, Qianqian & Tang, Fumin & Li, Bing & Dai, Haifeng & Zheng, Jim P. & Zhang, Cunman & Ming, Pingwen, 2022. "Investigation of the thermal responses under gas channel and land inside proton exchange membrane fuel cell with assembly pressure," Applied Energy, Elsevier, vol. 308(C).
    3. Hwang, Jenn-Jiang, 2013. "Thermal control and performance assessment of a proton exchanger membrane fuel cell generator," Applied Energy, Elsevier, vol. 108(C), pages 184-193.
    4. Wan, Zhongmin & Liu, Jing & Luo, Zhiping & Tu, Zhengkai & Liu, Zhichun & Liu, Wei, 2013. "Evaluation of self-water-removal in a dead-ended proton exchange membrane fuel cell," Applied Energy, Elsevier, vol. 104(C), pages 751-757.
    5. Xuan, Jin & Leung, D.Y.C. & Wang, Huizhi & Leung, Michael K.H. & Wang, Bin & Ni, Meng, 2013. "Air-breathing membraneless laminar flow-based fuel cells: Do they breathe enough oxygen?," Applied Energy, Elsevier, vol. 104(C), pages 400-407.
    6. Hosseinzadeh, Elham & Rokni, Masoud & Rabbani, Abid & Mortensen, Henrik Hilleke, 2013. "Thermal and water management of low temperature Proton Exchange Membrane Fuel Cell in fork-lift truck power system," Applied Energy, Elsevier, vol. 104(C), pages 434-444.
    7. Wu, Horng-Wen, 2016. "A review of recent development: Transport and performance modeling of PEM fuel cells," Applied Energy, Elsevier, vol. 165(C), pages 81-106.
    8. Baik, Kyung Don & Kong, Im Mo & Hong, Bo Ki & Kim, Sae Hoon & Kim, Min Soo, 2013. "Local measurements of hydrogen crossover rate in polymer electrolyte membrane fuel cells," Applied Energy, Elsevier, vol. 101(C), pages 560-566.
    9. Kwan, Trevor Hocksun & Wu, Xiaofeng & Yao, Qinghe, 2018. "Multi-objective genetic optimization of the thermoelectric system for thermal management of proton exchange membrane fuel cells," Applied Energy, Elsevier, vol. 217(C), pages 314-327.
    10. Xing, Lei & Liu, Xiaoteng & Alaje, Taiwo & Kumar, Ravi & Mamlouk, Mohamed & Scott, Keith, 2014. "A two-phase flow and non-isothermal agglomerate model for a proton exchange membrane (PEM) fuel cell," Energy, Elsevier, vol. 73(C), pages 618-634.
    11. Wang, H.Y. & Yang, W.J. & Kim, Y.B., 2014. "Analyzing in-plane temperature distribution via a micro-temperature sensor in a unit polymer electrolyte membrane fuel cell," Applied Energy, Elsevier, vol. 124(C), pages 148-155.
    12. Nishimura, Akira & Yamamoto, Kohei & Okado, Tatsuya & Kojima, Yuya & Hirota, Masafumi & Kolhe, Mohan Lal, 2020. "Impact analysis of MPL and PEM thickness on temperature distribution within PEFC operating at relatively higher temperature," Energy, Elsevier, vol. 205(C).
    13. Liu, Dengcheng & Lin, Rui & Feng, Bowen & Han, Lihang & Zhang, Yu & Ni, Meng & Wu, Sai, 2019. "Localised electrochemical impedance spectroscopy investigation of polymer electrolyte membrane fuel cells using Print circuit board based interference-free system," Applied Energy, Elsevier, vol. 254(C).
    14. Ling, C.Y. & Cao, H. & Chen, Y. & Han, M. & Birgersson, E., 2016. "Compact open cathode feed system for PEMFCs," Applied Energy, Elsevier, vol. 164(C), pages 670-675.
    15. Singdeo, Debanand & Dey, Tapobrata & Gaikwad, Shrihari & Andreasen, Søren Juhl & Ghosh, Prakash C., 2017. "A new modified-serpentine flow field for application in high temperature polymer electrolyte fuel cell," Applied Energy, Elsevier, vol. 195(C), pages 13-22.

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