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Experimental validation of a multiphase flow model of a lab-scale fluidized-bed gasification unit

Author

Listed:
  • Porcu, Andrea
  • Xu, Yupeng
  • Mureddu, Mauro
  • Dessì, Federica
  • Shahnam, Mehrdad
  • Rogers, William A.
  • Sastri, Bhima S.
  • Pettinau, Alberto

Abstract

This paper presents the results of a combined experimental and computational characterization of a biomass gasification process as a carbon neutral technology for power generation and/or green hydrogen production. With the aim to set and validate a computational fluid dynamic (CFD) multiphase flow simulation model based on the MFiX suite – as a support for the design and optimization of advanced reactors for energy purposes – a wide experimental campaign has been carried out with cypress (Cupressus sempervirens) wood chips in a lab-scale bubbling fluidized-bed gasification unit in different operation modes: pyrolysis, air-blown gasification as well as steam gasification of char. In addition, pyrolysis kinetics have been experimentally assessed by thermogravimetric analysis (TGA). This study shows that biomass pyrolysis is characterized by a syngas yield of 0.65–0.66, whereas its gasification allows the production of a syngas (1.73–1.77 Nm3 per kilogram of fuel) characterized by a lower heating value of about 5 MJ/Nm3, with a hydrogen concentration between 11.4 and 14.3% by volume (depending on the equivalence ratio). In addition, model used is a good predictive tool that can successfully simulate the process and predict syngas composition with good accuracy, in particular for CO, H2 and CH4.

Suggested Citation

  • Porcu, Andrea & Xu, Yupeng & Mureddu, Mauro & Dessì, Federica & Shahnam, Mehrdad & Rogers, William A. & Sastri, Bhima S. & Pettinau, Alberto, 2021. "Experimental validation of a multiphase flow model of a lab-scale fluidized-bed gasification unit," Applied Energy, Elsevier, vol. 293(C).
    • Handle: RePEc:eee:appene:v:293:y:2021:i:c:s030626192100413x
    DOI: 10.1016/j.apenergy.2021.116933
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    as
    1. Ku, Xiaoke & Wang, Jin & Jin, Hanhui & Lin, Jianzhong, 2019. "Effects of operating conditions and reactor structure on biomass entrained-flow gasification," Renewable Energy, Elsevier, vol. 139(C), pages 781-795.
    2. Kan, Xiang & Chen, Xiaoping & Shen, Ye & Lapkin, Alexei A. & Kraft, Markus & Wang, Chi-Hwa, 2019. "Box-Behnken design based CO2 co-gasification of horticultural waste and sewage sludge with addition of ash from waste as catalyst," Applied Energy, Elsevier, vol. 242(C), pages 1549-1561.
    3. Andrea Porcu & Stefano Sollai & Davide Marotto & Mauro Mureddu & Francesca Ferrara & Alberto Pettinau, 2019. "Techno-Economic Analysis of a Small-Scale Biomass-to-Energy BFB Gasification-Based System," Energies, MDPI, vol. 12(3), pages 1-17, February.
    4. Ardolino, Filomena & Lodato, Concetta & Astrup, Thomas F. & Arena, Umberto, 2018. "Energy recovery from plastic and biomass waste by means of fluidized bed gasification: A life cycle inventory model," Energy, Elsevier, vol. 165(PB), pages 299-314.
    5. Rodriguez-Alejandro, David A. & Nam, Hyungseok & Maglinao, Amado L. & Capareda, Sergio C. & Aguilera-Alvarado, Alberto F., 2016. "Development of a modified equilibrium model for biomass pilot-scale fluidized bed gasifier performance predictions," Energy, Elsevier, vol. 115(P1), pages 1092-1108.
    6. Gambarotta, Agostino & Morini, Mirko & Zubani, Andrea, 2018. "A non-stoichiometric equilibrium model for the simulation of the biomass gasification process," Applied Energy, Elsevier, vol. 227(C), pages 119-127.
    7. Kulkarni, Avanti & Baker, Ryan & Abdoulmomine, Nourredine & Adhikari, Sushil & Bhavnani, Sushil, 2016. "Experimental study of torrefied pine as a gasification fuel using a bubbling fluidized bed gasifier," Renewable Energy, Elsevier, vol. 93(C), pages 460-468.
    8. Sansaniwal, S.K. & Rosen, M.A. & Tyagi, S.K., 2017. "Global challenges in the sustainable development of biomass gasification: An overview," Renewable and Sustainable Energy Reviews, Elsevier, vol. 80(C), pages 23-43.
    9. Ahmed, I.I. & Gupta, A.K., 2011. "Kinetics of woodchips char gasification with steam and carbon dioxide," Applied Energy, Elsevier, vol. 88(5), pages 1613-1619, May.
    10. Jin Wu & Jiangjiang Wang & Jing Wu & Chaofan Ma, 2019. "Exergy and Exergoeconomic Analysis of a Combined Cooling, Heating, and Power System Based on Solar Thermal Biomass Gasification," Energies, MDPI, vol. 12(12), pages 1-19, June.
    11. Situmorang, Yohanes Andre & Zhao, Zhongkai & Yoshida, Akihiro & Abudula, Abuliti & Guan, Guoqing, 2020. "Small-scale biomass gasification systems for power generation (<200 kW class): A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 117(C).
    12. Vakalis, Stergios & Moustakas, Konstantinos, 2019. "Modelling of advanced gasification systems (MAGSY): Simulation and validation for the case of the rising co-current reactor," Applied Energy, Elsevier, vol. 242(C), pages 526-533.
    13. Jeong, Hyo Jae & Seo, Dong Kyun & Hwang, Jungho, 2014. "CFD modeling for coal size effect on coal gasification in a two-stage commercial entrained-bed gasifier with an improved char gasification model," Applied Energy, Elsevier, vol. 123(C), pages 29-36.
    14. Kan, Tao & Strezov, Vladimir & Evans, Tim J., 2016. "Lignocellulosic biomass pyrolysis: A review of product properties and effects of pyrolysis parameters," Renewable and Sustainable Energy Reviews, Elsevier, vol. 57(C), pages 1126-1140.
    15. Motta, Ingrid Lopes & Miranda, Nahieh Toscano & Maciel Filho, Rubens & Wolf Maciel, Maria Regina, 2018. "Biomass gasification in fluidized beds: A review of biomass moisture content and operating pressure effects," Renewable and Sustainable Energy Reviews, Elsevier, vol. 94(C), pages 998-1023.
    16. Lu, Ding & Yoshikawa, Kunio & Ismail, Tamer M. & Abd El-Salam, M., 2018. "Assessment of the carbonized woody briquette gasification in an updraft fixed bed gasifier using the Euler-Euler model," Applied Energy, Elsevier, vol. 220(C), pages 70-86.
    17. Wang, Jiangjiang & Ma, Chaofan & Wu, Jing, 2019. "Thermodynamic analysis of a combined cooling, heating and power system based on solar thermal biomass gasification☆," Applied Energy, Elsevier, vol. 247(C), pages 102-115.
    18. Schulze, S. & Richter, A. & Vascellari, M. & Gupta, A. & Meyer, B. & Nikrityuk, P.A., 2016. "Novel intrinsic-based submodel for char particle gasification in entrained-flow gasifiers: Model development, validation and illustration," Applied Energy, Elsevier, vol. 164(C), pages 805-814.
    19. Khodaei, Hassan & Al-Abdeli, Yasir M. & Guzzomi, Ferdinando & Yeoh, Guan H., 2015. "An overview of processes and considerations in the modelling of fixed-bed biomass combustion," Energy, Elsevier, vol. 88(C), pages 946-972.
    20. Parrillo, Francesco & Ardolino, Filomena & Calì, Gabriele & Marotto, Davide & Pettinau, Alberto & Arena, Umberto, 2021. "Fluidized bed gasification of eucalyptus chips: Axial profiles of syngas composition in a pilot scale reactor," Energy, Elsevier, vol. 219(C).
    21. Dessì, Federica & Mureddu, Mauro & Ferrara, Francesca & Fermoso, Javier & Orsini, Alessandro & Sanna, Aimaro & Pettinau, Alberto, 2021. "Thermogravimetric characterisation and kinetic analysis of Nannochloropsis sp. and Tetraselmis sp. microalgae for pyrolysis, combustion and oxy-combustion," Energy, Elsevier, vol. 217(C).
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    2. Verma, Shivpal & Dregulo, Andrei Mikhailovich & Kumar, Vinay & Bhargava, Preeti Chaturvedi & Khan, Nawaz & Singh, Anuradha & Sun, Xinwei & Sindhu, Raveendran & Binod, Parameswaran & Zhang, Zengqiang &, 2023. "Reaction engineering during biomass gasification and conversion to energy," Energy, Elsevier, vol. 266(C).
    3. Cormos, Calin-Cristian, 2023. "Green hydrogen production from decarbonized biomass gasification: An integrated techno-economic and environmental analysis," Energy, Elsevier, vol. 270(C).
    4. Dessì, Federica & Mureddu, Mauro & Ferrara, Francesca & Pettinau, Alberto, 2022. "A comprehensive pathway on the determination of the kinetic triplet and the reaction mechanism of brewer's spent grain and beech wood chips pyrolysis," Renewable Energy, Elsevier, vol. 190(C), pages 548-559.
    5. Tian, Beile & Mao, Songbo & Guo, Feiqiang & Bai, Jiaming & Shu, Rui & Qian, Lin & Liu, Qi, 2022. "Monolithic biochar-supported cobalt-based catalysts with high-activity and superior-stability for biomass tar reforming," Energy, Elsevier, vol. 242(C).

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