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Fluidized bed gasification of eucalyptus chips: Axial profiles of syngas composition in a pilot scale reactor

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  • Parrillo, Francesco
  • Ardolino, Filomena
  • Calì, Gabriele
  • Marotto, Davide
  • Pettinau, Alberto
  • Arena, Umberto

Abstract

Air gasification tests have been carried out in a pilot scale bubbling fluidized bed gasifier, able to treat up to 100 kg/h of Eucalyptus wood chips, and operated, under chemical and thermal steady-state conditions, at different values of equivalence ratio. The results are reported in terms of the main process performance parameters and transfer coefficients, which indicate the fate of carbon in the different output streams (syngas, fines, tars). The results can be transferred to commercial scale reactors and confirm the technical feasibility of the air gasification of the biomass in the range 0.25–0.34 of equivalence ratio, yielding a good quality syngas, with a low heating value between 5000 and 6000 kJ/m3N,syngas. The measured axial syngas composition profiles along the reactor indicate a monotonic reduction of methane and carbon dioxide concentrations and an increase of that of hydrogen. This suggests that water gas shift and steam and dry reforming reactions play a significant role, together with a limited contribution of tar cracking reactions, probably enhanced by alkali and alkaline earth metallic species contained in the inorganic fraction of elutriated fines. Results can support the implementation of reliable numerical models of bubbling fluidized bed gasifiers and the optimisation of design/operating criteria.

Suggested Citation

  • Parrillo, Francesco & Ardolino, Filomena & Calì, Gabriele & Marotto, Davide & Pettinau, Alberto & Arena, Umberto, 2021. "Fluidized bed gasification of eucalyptus chips: Axial profiles of syngas composition in a pilot scale reactor," Energy, Elsevier, vol. 219(C).
    • Handle: RePEc:eee:energy:v:219:y:2021:i:c:s0360544220327110
    DOI: 10.1016/j.energy.2020.119604
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    References listed on IDEAS

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    1. Alauddin, Zainal Alimuddin Bin Zainal & Lahijani, Pooya & Mohammadi, Maedeh & Mohamed, Abdul Rahman, 2010. "Gasification of lignocellulosic biomass in fluidized beds for renewable energy development: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 14(9), pages 2852-2862, December.
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    3. Andrea Porcu & Stefano Sollai & Davide Marotto & Mauro Mureddu & Francesca Ferrara & Alberto Pettinau, 2019. "Techno-Economic Analysis of a Small-Scale Biomass-to-Energy BFB Gasification-Based System," Energies, MDPI, vol. 12(3), pages 1-17, February.
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    5. Arena, Umberto & Di Gregorio, Fabrizio, 2014. "Energy generation by air gasification of two industrial plastic wastes in a pilot scale fluidized bed reactor," Energy, Elsevier, vol. 68(C), pages 735-743.
    6. Parrillo, F. & Ruoppolo, G. & Arena, U., 2020. "The role of activated carbon size in the catalytic cracking of naphthalene," Energy, Elsevier, vol. 190(C).
    7. Anis, Samsudin & Zainal, Z.A., 2011. "Tar reduction in biomass producer gas via mechanical, catalytic and thermal methods: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 15(5), pages 2355-2377, June.
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    1. Dessì, Federica & Mureddu, Mauro & Ferrara, Francesca & Pettinau, Alberto, 2022. "A comprehensive pathway on the determination of the kinetic triplet and the reaction mechanism of brewer's spent grain and beech wood chips pyrolysis," Renewable Energy, Elsevier, vol. 190(C), pages 548-559.
    2. Giovanni Biancini & Barbara Marchetti & Luca Cioccolanti & Matteo Moglie, 2022. "Comprehensive Life Cycle Assessment Analysis of an Italian Composting Facility concerning Environmental Footprint Minimization and Renewable Energy Integration," Sustainability, MDPI, vol. 14(22), pages 1-21, November.
    3. Parrillo, Francesco & Ardolino, Filomena & Boccia, Carmine & Calì, Gabriele & Marotto, Davide & Pettinau, Alberto & Arena, Umberto, 2023. "Co-gasification of plastics waste and biomass in a pilot scale fluidized bed reactor," Energy, Elsevier, vol. 273(C).
    4. Porcu, Andrea & Xu, Yupeng & Mureddu, Mauro & Dessì, Federica & Shahnam, Mehrdad & Rogers, William A. & Sastri, Bhima S. & Pettinau, Alberto, 2021. "Experimental validation of a multiphase flow model of a lab-scale fluidized-bed gasification unit," Applied Energy, Elsevier, vol. 293(C).

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