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Process synthesis and analysis for catalytic conversion of lignocellulosic biomass to fuels: Separate conversion of cellulose and hemicellulose using 2-sec-butylphenol (SBP) solvent

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  • Byun, Jaewon
  • Han, Jeehoon

Abstract

We developed a strategy for the catalytic production of liquid hydrocarbon fuels (butene oligomers) from cellulose and hemicellulose, which are the major fractions of lignocellulosic biomass. In this strategy the cellulose and hemicellulose fractions are separated through a pretreatment step and then converted to levulinic acid (LA) by monophasic and biphasic reactions using 2-sec-butylphenol (SBP) solvent respectively. The LA is upgraded catalytically to γ-valerolactone (GVL), and subsequently to butene oligomers. To design the integrated strategy, we developed separation subsystems to satisfy the optimized feed concentration for catalytic conversions and to recycle solvents (SBP). To satisfy energy requirements for our process from combustion of biomass residues, we designed a heat exchanger network (HEN) for minimum energy consumption by maximizing heat recovery from the process streams. Our technoeconomic evaluation shows that the integrated strategy using corn stover feedstock results in a minimum selling price of $3.71 per gallon of gasoline equivalent for butene oligomers if using the best possible parameters.

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  • Byun, Jaewon & Han, Jeehoon, 2016. "Process synthesis and analysis for catalytic conversion of lignocellulosic biomass to fuels: Separate conversion of cellulose and hemicellulose using 2-sec-butylphenol (SBP) solvent," Applied Energy, Elsevier, vol. 171(C), pages 483-490.
    • Handle: RePEc:eee:appene:v:171:y:2016:i:c:p:483-490
    DOI: 10.1016/j.apenergy.2016.03.088
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    Cited by:

    1. Kim, Juyeon & Han, Jeehoon, 2021. "Bio-based process for the catalytic production of ethyl levulinate from cellulose," Applied Energy, Elsevier, vol. 300(C).
    2. Kwon, Oseok & Han, Jeehoon, 2021. "Supply chain management of butyric acid-derived butanol: Stochastic approach," Applied Energy, Elsevier, vol. 297(C).
    3. Kim, Juyeon & Byun, Jaewon & Han, Jeehoon, 2022. "Process integration and economics of gamma-valerolactone using a cellulose-derived ethyl levulinate intermediate and ethanol solvent," Energy, Elsevier, vol. 239(PA).
    4. Kim, Juyeon & Han, Jeehoon, 2018. "Simulation study of a strategy to produce gamma-valerolactone from ethyl levulinate," Energy, Elsevier, vol. 163(C), pages 986-991.
    5. Cho, Seong-Heon & Kim, Juyeon & Han, Jeehoon & Lee, Daewon & Kim, Hyung Ju & Kim, Yong Tae & Cheng, Xun & Xu, Ye & Lee, Jechan & Kwon, Eilhann E., 2019. "Bioalcohol production from acidogenic products via a two-step process: A case study of butyric acid to butanol," Applied Energy, Elsevier, vol. 252(C), pages 1-1.
    6. Kwon, Oseok & Kim, Juyeon & Han, Jeehoon, 2022. "Organic waste derived biodiesel supply chain network: Deterministic multi-period planning model," Applied Energy, Elsevier, vol. 305(C).
    7. Byun, Jaewon & Han, Jeehoon, 2020. "Economic feasible strategy of cellulosic biofuels: Co-production of pentanediols," Energy, Elsevier, vol. 193(C).
    8. Park, Hoyoung & Byun, Jaewon & Han, Jeehoon, 2021. "Economically feasible thermochemical process for methanol production from kenaf," Energy, Elsevier, vol. 230(C).
    9. Xu, Jikun & Hou, Huijie & Hu, Jingping & Liu, Bingchuan, 2018. "Coupling of hydrothermal and ionic liquid pretreatments for sequential biorefinery of Tamarix austromongolica," Applied Energy, Elsevier, vol. 229(C), pages 745-755.
    10. Byun, Jaewon & Han, Jeehoon, 2021. "Economically feasible production of green methane from vegetable and fruit-rich food waste," Energy, Elsevier, vol. 235(C).

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