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Observation of phonon Stark effect

Author

Listed:
  • Zhiheng Huang

    (Chinese Academy of Sciences
    University of Chinese Academy of Sciences)

  • Yunfei Bai

    (Chinese Academy of Sciences
    University of Chinese Academy of Sciences)

  • Yanchong Zhao

    (Chinese Academy of Sciences
    University of Chinese Academy of Sciences)

  • Le Liu

    (Chinese Academy of Sciences
    University of Chinese Academy of Sciences)

  • Xuan Zhao

    (Chinese Academy of Sciences
    University of Chinese Academy of Sciences)

  • Jiangbin Wu

    (Chinese Academy of Sciences)

  • Kenji Watanabe

    (National Institute for Materials Science)

  • Takashi Taniguchi

    (National Institute for Materials Science)

  • Wei Yang

    (Chinese Academy of Sciences
    University of Chinese Academy of Sciences)

  • Dongxia Shi

    (Chinese Academy of Sciences
    University of Chinese Academy of Sciences)

  • Yang Xu

    (Chinese Academy of Sciences
    University of Chinese Academy of Sciences)

  • Tiantian Zhang

    (Chinese Academy of Sciences)

  • Qingming Zhang

    (Chinese Academy of Sciences
    University of Chinese Academy of Sciences
    Lanzhou University)

  • Ping-Heng Tan

    (Chinese Academy of Sciences)

  • Zhipei Sun

    (Aalto University)

  • Sheng Meng

    (Chinese Academy of Sciences
    University of Chinese Academy of Sciences
    Songshan Lake Materials Laboratory)

  • Yaxian Wang

    (Chinese Academy of Sciences)

  • Luojun Du

    (Chinese Academy of Sciences
    University of Chinese Academy of Sciences)

  • Guangyu Zhang

    (Chinese Academy of Sciences
    University of Chinese Academy of Sciences
    Songshan Lake Materials Laboratory)

Abstract

Stark effect, the electric-field analogue of magnetic Zeeman effect, is one of the celebrated phenomena in modern physics and appealing for emergent applications in electronics, optoelectronics, as well as quantum technologies. While in condensed matter it has prospered only for excitons, whether other collective excitations can display Stark effect remains elusive. Here, we report the observation of phonon Stark effect in a two-dimensional quantum system of bilayer 2H-MoS2. The longitudinal acoustic phonon red-shifts linearly with applied electric fields and can be tuned over ~1 THz, evidencing giant Stark effect of phonons. Together with many-body ab initio calculations, we uncover that the observed phonon Stark effect originates fundamentally from the strong coupling between phonons and interlayer excitons (IXs). In addition, IX-mediated electro-phonon intensity modulation up to ~1200% is discovered for infrared-active phonon A2u. Our results unveil the exotic phonon Stark effect and effective phonon engineering by IX-mediated mechanism, promising for a plethora of exciting many-body physics and potential technological innovations.

Suggested Citation

  • Zhiheng Huang & Yunfei Bai & Yanchong Zhao & Le Liu & Xuan Zhao & Jiangbin Wu & Kenji Watanabe & Takashi Taniguchi & Wei Yang & Dongxia Shi & Yang Xu & Tiantian Zhang & Qingming Zhang & Ping-Heng Tan , 2024. "Observation of phonon Stark effect," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    • Handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-48992-w
    DOI: 10.1038/s41467-024-48992-w
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    References listed on IDEAS

    as
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