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Long-range transport of 2D excitons with acoustic waves

Author

Listed:
  • Ruoming Peng

    (University of Washington)

  • Adina Ripin

    (University of Washington)

  • Yusen Ye

    (University of Washington)

  • Jiayi Zhu

    (University of Washington)

  • Changming Wu

    (University of Washington)

  • Seokhyeong Lee

    (University of Washington)

  • Huan Li

    (University of Washington
    Zhejiang University)

  • Takashi Taniguchi

    (Research Center for Functional Materials, National Institute for Materials Science)

  • Kenji Watanabe

    (Research Center for Functional Materials, National Institute for Materials Science)

  • Ting Cao

    (University of Washington)

  • Xiaodong Xu

    (University of Washington
    University of Washington)

  • Mo Li

    (University of Washington
    University of Washington)

Abstract

Excitons are elementary optical excitation in semiconductors. The ability to manipulate and transport these quasiparticles would enable excitonic circuits and devices for quantum photonic technologies. Recently, interlayer excitons in 2D semiconductors have emerged as a promising candidate for engineering excitonic devices due to their long lifetime, large exciton binding energy, and gate tunability. However, the charge-neutral nature of the excitons leads to weak response to the in-plane electric field and thus inhibits transport beyond the diffusion length. Here, we demonstrate the directional transport of interlayer excitons in bilayer WSe2 driven by the propagating potential traps induced by surface acoustic waves (SAW). We show that at 100 K, the SAW-driven excitonic transport is activated above a threshold acoustic power and reaches 20 μm, a distance at least ten times longer than the diffusion length and only limited by the device size. Temperature-dependent measurement reveals the transition from the diffusion-limited regime at low temperature to the acoustic field-driven regime at elevated temperature. Our work shows that acoustic waves are an effective, contact-free means to control exciton dynamics and transport, promising for realizing 2D materials-based excitonic devices such as exciton transistors, switches, and transducers up to room temperature.

Suggested Citation

  • Ruoming Peng & Adina Ripin & Yusen Ye & Jiayi Zhu & Changming Wu & Seokhyeong Lee & Huan Li & Takashi Taniguchi & Kenji Watanabe & Ting Cao & Xiaodong Xu & Mo Li, 2022. "Long-range transport of 2D excitons with acoustic waves," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
  • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-29042-9
    DOI: 10.1038/s41467-022-29042-9
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    1. Sanfeng Wu & Sonia Buckley & John R. Schaibley & Liefeng Feng & Jiaqiang Yan & David G. Mandrus & Fariba Hatami & Wang Yao & Jelena Vučković & Arka Majumdar & Xiaodong Xu, 2015. "Monolayer semiconductor nanocavity lasers with ultralow thresholds," Nature, Nature, vol. 520(7545), pages 69-72, April.
    2. Zefang Wang & Daniel A. Rhodes & Kenji Watanabe & Takashi Taniguchi & James C. Hone & Jie Shan & Kin Fai Mak, 2019. "Evidence of high-temperature exciton condensation in two-dimensional atomic double layers," Nature, Nature, vol. 574(7776), pages 76-80, October.
    3. Pasqual Rivera & John R. Schaibley & Aaron M. Jones & Jason S. Ross & Sanfeng Wu & Grant Aivazian & Philip Klement & Kyle Seyler & Genevieve Clark & Nirmal J. Ghimire & Jiaqiang Yan & D. G. Mandrus & , 2015. "Observation of long-lived interlayer excitons in monolayer MoSe2–WSe2 heterostructures," Nature Communications, Nature, vol. 6(1), pages 1-6, May.
    4. Jessica Lindlau & Malte Selig & Andre Neumann & Léo Colombier & Jonathan Förste & Victor Funk & Michael Förg & Jonghwan Kim & Gunnar Berghäuser & Takashi Taniguchi & Kenji Watanabe & Feng Wang & Ermin, 2018. "The role of momentum-dark excitons in the elementary optical response of bilayer WSe2," Nature Communications, Nature, vol. 9(1), pages 1-7, December.
    5. Kha Tran & Galan Moody & Fengcheng Wu & Xiaobo Lu & Junho Choi & Kyounghwan Kim & Amritesh Rai & Daniel A. Sanchez & Jiamin Quan & Akshay Singh & Jacob Embley & André Zepeda & Marshall Campbell & Trav, 2019. "Evidence for moiré excitons in van der Waals heterostructures," Nature, Nature, vol. 567(7746), pages 71-75, March.
    6. Kyle L. Seyler & Pasqual Rivera & Hongyi Yu & Nathan P. Wilson & Essance L. Ray & David G. Mandrus & Jiaqiang Yan & Wang Yao & Xiaodong Xu, 2019. "Signatures of moiré-trapped valley excitons in MoSe2/WSe2 heterobilayers," Nature, Nature, vol. 567(7746), pages 66-70, March.
    7. Nils Lundt & Sebastian Klembt & Evgeniia Cherotchenko & Simon Betzold & Oliver Iff & Anton V. Nalitov & Martin Klaas & Christof P. Dietrich & Alexey V. Kavokin & Sven Höfling & Christian Schneider, 2016. "Room-temperature Tamm-plasmon exciton-polaritons with a WSe2 monolayer," Nature Communications, Nature, vol. 7(1), pages 1-6, December.
    8. Long Zhang & Fengcheng Wu & Shaocong Hou & Zhe Zhang & Yu-Hsun Chou & Kenji Watanabe & Takashi Taniguchi & Stephen R. Forrest & Hui Deng, 2021. "Van der Waals heterostructure polaritons with moiré-induced nonlinearity," Nature, Nature, vol. 591(7848), pages 61-65, March.
    9. Chenhao Jin & Emma C. Regan & Aiming Yan & M. Iqbal Bakti Utama & Danqing Wang & Sihan Zhao & Ying Qin & Sijie Yang & Zhiren Zheng & Shenyang Shi & Kenji Watanabe & Takashi Taniguchi & Sefaattin Tonga, 2019. "Observation of moiré excitons in WSe2/WS2 heterostructure superlattices," Nature, Nature, vol. 567(7746), pages 76-80, March.
    10. Long Zhang & Rahul Gogna & Will Burg & Emanuel Tutuc & Hui Deng, 2018. "Photonic-crystal exciton-polaritons in monolayer semiconductors," Nature Communications, Nature, vol. 9(1), pages 1-8, December.
    11. Wei Fu & Zhen Shen & Yuntao Xu & Chang-Ling Zou & Risheng Cheng & Xu Han & Hong X. Tang, 2019. "Phononic integrated circuitry and spin–orbit interaction of phonons," Nature Communications, Nature, vol. 10(1), pages 1-7, December.
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    1. Hassan Lamsaadi & Dorian Beret & Ioannis Paradisanos & Pierre Renucci & Delphine Lagarde & Xavier Marie & Bernhard Urbaszek & Ziyang Gan & Antony George & Kenji Watanabe & Takashi Taniguchi & Andrey T, 2023. "Kapitza-resistance-like exciton dynamics in atomically flat MoSe2-WSe2 lateral heterojunction," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    2. Arjun Iyer & Yadav P. Kandel & Wendao Xu & John M. Nichol & William H. Renninger, 2024. "Coherent optical coupling to surface acoustic wave devices," Nature Communications, Nature, vol. 15(1), pages 1-9, December.

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