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Real-Time Source Dynamics of PM 2.5 During Winter Haze Episodes Resolved by SPAMS: A Case Study in Yinchuan, Northwest China

Author

Listed:
  • Huihui Du

    (Yinchuan Ecological Environment Monitoring Station, Yinchuan 750001, China)

  • Tantan Tan

    (School of Water and Environment, Chang’an University, Xi’an 710054, China)

  • Jiaying Pan

    (Yinchuan Ecological Environment Monitoring Station, Yinchuan 750001, China)

  • Meng Xu

    (Yinchuan Ecological Environment Monitoring Station, Yinchuan 750001, China)

  • Aidong Liu

    (Yinchuan Ecological Environment Monitoring Station, Yinchuan 750001, China)

  • Yanpeng Li

    (School of Water and Environment, Chang’an University, Xi’an 710054, China
    Key Laboratory of Subsurface Hydrology and Ecological Effect in Arid Region of the Ministry of Education, Chang’an University, Xi’an 710054, China)

Abstract

The occurrence of haze pollution significantly deteriorates air quality and threatens human health, yet persistent knowledge gaps in real-time source apportionment of fine particulate matter (PM 2.5 ) hinder sustained improvements in atmospheric pollution conditions. Thus, this study employed single-particle aerosol mass spectrometry (SPAMS) to investigate PM 2.5 sources and dynamics during winter haze episodes in Yinchuan, Northwest China. Results showed that the average PM 2.5 concentration was 57 μg·m −3 , peaking at 218 μg·m −3 . PM 2.5 was dominated by organic carbon (OC, 17.3%), mixed carbonaceous particles (ECOC, 17.0%), and elemental carbon (EC, 14.3%). The primary sources were coal combustion (26.4%), fugitive dust (25.8%), and vehicle emissions (19.1%). Residential coal burning dominated coal emissions (80.9%), highlighting inefficient decentralized heating. Source contributions showed distinct diurnal patterns: coal combustion peaked nocturnally (29.3% at 09:00) due to heating and inversions, fugitive dust rose at night (28.6% at 19:00) from construction and low winds, and vehicle emissions aligned with traffic (17.5% at 07:00). Haze episodes were driven by synergistic increases in local coal (+4.0%), dust (+2.7%), and vehicle (+2.1%) emissions, compounded by regional transport (10.1–36.7%) of aged particles from northwestern zones. Fugitive dust correlated with sulfur dioxide (SO 2 ) and ozone (O 3 ) ( p < 0.01), suggesting roles as carriers and reactive interfaces. Findings confirm local emission dominance with spatiotemporal heterogeneity and regional transport influence. SPAMS effectively resolved short-term pollution dynamics, providing critical insights for targeted air quality management in arid regions.

Suggested Citation

  • Huihui Du & Tantan Tan & Jiaying Pan & Meng Xu & Aidong Liu & Yanpeng Li, 2025. "Real-Time Source Dynamics of PM 2.5 During Winter Haze Episodes Resolved by SPAMS: A Case Study in Yinchuan, Northwest China," Sustainability, MDPI, vol. 17(14), pages 1-20, July.
    • Handle: RePEc:gam:jsusta:v:17:y:2025:i:14:p:6627-:d:1705889
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    References listed on IDEAS

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    1. Yun Liu & Ruoshui Wang & Tingning Zhao & Jun Gao & Chenghao Zheng & Mengwei Wang, 2025. "Spatiotemporal Distribution of Atmospheric Particulate Matters and Correlations Among Them in Different Functional Areas of a Typical Mining City in Northwestern China," Sustainability, MDPI, vol. 17(13), pages 1-19, June.
    2. Zhang, Zongxi & Zhou, Yuguang & Zhao, Nan & Li, Huan & Tohniyaz, Bahargul & Mperejekumana, Philbert & Hong, Quan & Wu, Rucong & Li, Gang & Sultan, Muhammad & Zayan, Ali Mohammed Ibrahim & Cao, Jinxin , 2021. "Clean heating during winter season in Northern China: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 149(C).
    3. Ru-Jin Huang & Yanlin Zhang & Carlo Bozzetti & Kin-Fai Ho & Jun-Ji Cao & Yongming Han & Kaspar R. Daellenbach & Jay G. Slowik & Stephen M. Platt & Francesco Canonaco & Peter Zotter & Robert Wolf & Sim, 2014. "High secondary aerosol contribution to particulate pollution during haze events in China," Nature, Nature, vol. 514(7521), pages 218-222, October.
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