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Recent Developments in Ceria-Driven Solar Thermochemical Water and Carbon Dioxide Splitting Redox Cycle

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  • Rahul R. Bhosale

    (Department of Civil and Chemical Engineering, University of Tennessee at Chattanooga, 615 Mccallie Ave., Chattanooga, TN 37403, USA)

Abstract

Metal oxide (MO) based solar thermochemical H 2 O (WS) and CO 2 splitting (CDS) is one of the most promising and potential-containing processes that can be used to produce H 2 and syngas (liquid fuel precursor). Several non-volatile and volatile MOs were considered redox materials for the solar-driven WS and CDS operation. Among all the examined redox materials, based on their high O 2 storage capacity, faster oxidation kinetics, and good stability, ceria and doped ceria materials are deemed to be one of the best alternatives for the operation of the thermochemical redox reactions associated with the WS and CDS. Pure ceria was used for solar fuel production for the first time in 2006. A review paper highlighting the work done on the ceria-based solar thermochemical redox WS and CDS cycle from 2006 until 2016 is already published elsewhere by the author. This review paper presents all the significant findings reported in applying pure ceria and doped ceria materials for the WS and CDS by research teams worldwide.

Suggested Citation

  • Rahul R. Bhosale, 2023. "Recent Developments in Ceria-Driven Solar Thermochemical Water and Carbon Dioxide Splitting Redox Cycle," Energies, MDPI, vol. 16(16), pages 1-30, August.
    • Handle: RePEc:gam:jeners:v:16:y:2023:i:16:p:5949-:d:1215713
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    References listed on IDEAS

    as
    1. Wang, Bo & Li, Xian & Zhu, Xuancan & Wang, Yuesen & Tian, Tian & Dai, Yanjun & Wang, Chi-Hwa, 2023. "An epitrochoidal rotary reactor for solar-driven hydrogen production based on the redox cycling of ceria: Thermodynamic analysis and geometry optimization," Energy, Elsevier, vol. 270(C).
    2. Koepf, E. & Alxneit, I. & Wieckert, C. & Meier, A., 2017. "A review of high temperature solar driven reactor technology: 25years of experience in research and development at the Paul Scherrer Institute," Applied Energy, Elsevier, vol. 188(C), pages 620-651.
    3. Stéphane Abanades, 2022. "Redox Cycles, Active Materials, and Reactors Applied to Water and Carbon Dioxide Splitting for Solar Thermochemical Fuel Production: A Review," Energies, MDPI, vol. 15(19), pages 1-28, September.
    4. Haeussler, Anita & Abanades, Stéphane & Julbe, Anne & Jouannaux, Julien & Cartoixa, Bruno, 2020. "Solar thermochemical fuel production from H2O and CO2 splitting via two-step redox cycling of reticulated porous ceria structures integrated in a monolithic cavity-type reactor," Energy, Elsevier, vol. 201(C).
    5. Thanda, V.K. & Fend, Th. & Laaber, D. & Lidor, A. & von Storch, H. & Säck, J.P. & Hertel, J. & Lampe, J. & Menz, S. & Piesche, G. & Berger, S. & Lorentzou, S. & Syrigou, M. & Denk, Th. & Gonzales-Pard, 2022. "Experimental investigation of the applicability of a 250 kW ceria receiver/reactor for solar thermochemical hydrogen generation," Renewable Energy, Elsevier, vol. 198(C), pages 389-398.
    6. Lucía Arribas & José González-Aguilar & Manuel Romero, 2018. "Solar-Driven Thermochemical Water-Splitting by Cerium Oxide: Determination of Operational Conditions in a Directly Irradiated Fixed Bed Reactor," Energies, MDPI, vol. 11(9), pages 1-15, September.
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