IDEAS home Printed from https://ideas.repec.org/a/gam/jeners/v15y2022i18p6751-d915798.html
   My bibliography  Save this article

Gasification Characteristics of High Moisture Content Lignite under CO 2 and Auto-Generated Steam Atmosphere in a Moving Bed Tubular Reactor

Author

Listed:
  • Haojie Gao

    (School of Automotive Engineering, Yancheng Institution of Technology, Yancheng 224051, China)

  • Zhisong Wen

    (School of Automotive Engineering, Yancheng Institution of Technology, Yancheng 224051, China)

  • Lizhu Jin

    (School of Automotive Engineering, Yancheng Institution of Technology, Yancheng 224051, China)

  • Xin Xiong

    (School of Automotive Engineering, Yancheng Institution of Technology, Yancheng 224051, China)

  • Yuezhao Zhu

    (School of Mechanical and Power Engineering, Nanjing Tech University, Nanjing 211816, China)

Abstract

An external thermal high-temperature continuous feed moving bed tubular reactor was used for the gasification of high moisture content lignite (30.41 wt.%) under CO 2 and an auto-generated steam atmosphere. The objectives of this study are to illustrate the synergistic gasification characteristics of high moisture content lignite and CO 2 in the tubular reactor; CO 2 and auto-generated steam (steam released from the lignite) were used as gasification agents for lignite gasification. The effects of temperature and CO 2 flow rate were also investigated. Experimental results showed that when the gasification temperature increased from 800 °C to 1000 °C, the H 2 yield also increased from 8.45 mol kg −1 to 17.86 mol kg −1 . This may indicate that the H 2 O-CO 2 gasification of semi-coke was enhanced with the rise in temperature. At 900 °C, the gas yield increased with the increase in CO 2 flow rate, while the yield of char and liquid product showed an opposite trend. The lower heating value of the H 2 -rich syngas varied from 11.73 MJ m −3 to 12.77 MJ Nm −3 . The experimental results proved that the high moisture content lignite in-situ CO 2 gasification process is an effective methodology for the clean and efficient utilization of lignite.

Suggested Citation

  • Haojie Gao & Zhisong Wen & Lizhu Jin & Xin Xiong & Yuezhao Zhu, 2022. "Gasification Characteristics of High Moisture Content Lignite under CO 2 and Auto-Generated Steam Atmosphere in a Moving Bed Tubular Reactor," Energies, MDPI, vol. 15(18), pages 1-10, September.
  • Handle: RePEc:gam:jeners:v:15:y:2022:i:18:p:6751-:d:915798
    as

    Download full text from publisher

    File URL: https://www.mdpi.com/1996-1073/15/18/6751/pdf
    Download Restriction: no

    File URL: https://www.mdpi.com/1996-1073/15/18/6751/
    Download Restriction: no
    ---><---

    References listed on IDEAS

    as
    1. Özdenkçi, Karhan & Prestipino, Mauro & Björklund-Sänkiaho, Margareta & Galvagno, Antonio & De Blasio, Cataldo, 2020. "Alternative energy valorization routes of black liquor by stepwise supercritical water gasification: Effect of process parameters on hydrogen yield and energy efficiency," Renewable and Sustainable Energy Reviews, Elsevier, vol. 134(C).
    2. Liu, Rongtang & Liu, Ming & Fan, Peipei & Zhao, Yongliang & Yan, Junjie, 2018. "Thermodynamic study on a novel lignite poly-generation system of electricity-gas-tar integrated with pre-drying and pyrolysis," Energy, Elsevier, vol. 165(PB), pages 140-152.
    3. Kumari, Geeta & Vairakannu, Prabu, 2018. "CO2-air based two stage gasification of low ash and high ash Indian coals in the context of underground coal gasification," Energy, Elsevier, vol. 143(C), pages 822-832.
    4. He, Xiao & Zeng, Kuo & Xie, Yingpu & Flamant, Gilles & Yang, Haiping & Yang, Xinyi & Nzihou, Ange & Zheng, Anqing & Ding, Zhi & Chen, Hanping, 2019. "The effects of temperature and molten salt on solar pyrolysis of lignite," Energy, Elsevier, vol. 181(C), pages 407-416.
    5. Liu, Jia & Hu, Nan & Fan, Li-Wu, 2022. "Optimal design and thermodynamic analysis on the hydrogen oxidation reactor in a combined hydrogen production and power generation system based on coal gasification in supercritical water," Energy, Elsevier, vol. 238(PB).
    Full references (including those not matched with items on IDEAS)

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Zhao, Jingyu & Deng, Jun & Wang, Tao & Song, Jiajia & Zhang, Yanni & Shu, Chi-Min & Zeng, Qiang, 2019. "Assessing the effectiveness of a high-temperature-programmed experimental system for simulating the spontaneous combustion properties of bituminous coal through thermokinetic analysis of four oxidatio," Energy, Elsevier, vol. 169(C), pages 587-596.
    2. Arnob Das & Susmita Datta Peu, 2022. "A Comprehensive Review on Recent Advancements in Thermochemical Processes for Clean Hydrogen Production to Decarbonize the Energy Sector," Sustainability, MDPI, vol. 14(18), pages 1-42, September.
    3. Bei, Lijing & Ge, Zhiwei & Ren, Changyifan & Su, Di & Shang, Fei & Wang, Yu & Guo, Liejin, 2023. "Numerical study on supercritical water partial oxidation of ethanol with auto-thermal operation," Energy, Elsevier, vol. 264(C).
    4. Wei, Yi & Lu, Licong & Zhang, Xudong & Ji, Jianbing, 2022. "Hydrogen produced at low temperatures by electrochemically assisted pyrolysis of cellulose in molten carbonate," Energy, Elsevier, vol. 254(PC).
    5. Zeng, Kuo & Li, Rui & Minh, Doan Pham & Weiss-Hortala, Elsa & Nzihou, Ange & Zhong, Dian & Flamant, Gilles, 2020. "Characterization of char generated from solar pyrolysis of heavy metal contaminated biomass," Energy, Elsevier, vol. 206(C).
    6. Zeng, Kuo & Li, Jun & Xie, Yingpu & Yang, Haiping & Yang, Xinyi & Zhong, Dian & Zhen, Wanxin & Flamant, Gilles & Chen, Hanping, 2020. "Molten salt pyrolysis of biomass: The mechanism of volatile reforming and pyrolysis," Energy, Elsevier, vol. 213(C).
    7. Feng, Lele & Zhou, Sibo & Xu, Xiangcen & Qin, Botao, 2022. "Importance evaluation for influencing factors of underground coal gasification through ex-situ experiment and analytic hierarchy process," Energy, Elsevier, vol. 261(PA).
    8. Li, Hong & Zhou, Hao & Liu, Kailong & Gao, Xin & Li, Xingang, 2021. "Retrofit application of traditional petroleum chemical technologies to coal chemical industry for sustainable energy-efficiency production," Energy, Elsevier, vol. 218(C).
    9. Chen, Yi-Feng & Su, Sheng & Zhang, Liang-Ping & Jiang, Long & Qing, Meng-Xia & Chi, Huan-Ying & Ling, Peng & Han, Heng-Da & Xu, Kai & Wang, Yi & Hu, Song & Xiang, Jun, 2021. "Insights into evolution mechanism of PAHs in coal thermal conversion: A combined experimental and DFT study," Energy, Elsevier, vol. 222(C).
    10. Liu, Rongtang & Liu, Ming & Zhao, Yongliang & Ma, Yuegeng & Yan, Junjie, 2021. "Thermodynamic study of a novel lignite poly-generation system driven by solar energy," Energy, Elsevier, vol. 214(C).
    11. Fan, Yuyang & Li, Luwei & Tippayawong, Nakorn & Xia, Shengpeng & Cao, Fengzhu & Yang, Xingwei & Zheng, Anqing & Zhao, Zengli & Li, Haibin, 2019. "Quantitative structure-reactivity relationships for pyrolysis and gasification of torrefied xylan," Energy, Elsevier, vol. 188(C).
    12. Xin, Lin & An, Mingyu & Feng, Mingze & Li, Kaixuan & Cheng, Weimin & Liu, Weitao & Hu, Xiangming & Wang, Zhigang & Han, Limin, 2021. "Study on pyrolysis characteristics of lump coal in the context of underground coal gasification," Energy, Elsevier, vol. 237(C).
    13. Zhao, Yongliang & Liu, Ming & Wang, Chaoyang & Wang, Zhu & Chong, Daotong & Yan, Junjie, 2019. "Exergy analysis of the regulating measures of operational flexibility in supercritical coal-fired power plants during transient processes," Applied Energy, Elsevier, vol. 253(C), pages 1-1.
    14. Backer, Michael & Gladen, Adam, 2023. "Impact of salt composition and temperature on low-temperature torrefaction of pine in molten nitrate salts," Energy, Elsevier, vol. 263(PE).
    15. Xu, Jialing & Rong, Siqi & Sun, Jingli & Peng, Zhiyong & Jin, Hui & Guo, Liejin & Zhang, Xiang & Zhou, Teng, 2022. "Optimal design of non-isothermal supercritical water gasification reactor: From biomass to hydrogen," Energy, Elsevier, vol. 244(PB).
    16. Shen, Ye & Li, Xian & Yao, Zhiyi & Cui, Xiaoqiang & Wang, Chi-Hwa, 2019. "CO2 gasification of woody biomass: Experimental study from a lab-scale reactor to a small-scale autothermal gasifier," Energy, Elsevier, vol. 170(C), pages 497-506.
    17. Huang, Yingfei & Zhang, Fengming & Liang, Zhaojian & Li, Yufeng & Wu, Tong, 2023. "Effect of hydrothermal flame generation methods on energy consumption and economic performance of supercritical water oxidation systems," Energy, Elsevier, vol. 266(C).
    18. Huo, Hailong & Liu, Xunliang & Wen, Zhi & Lou, Guofeng & Dou, Ruifeng & Su, Fuyong & Zhou, Wenning & Jiang, Zeyi, 2021. "Case study of a novel low rank coal to calcium carbide process based on techno-economic assessment," Energy, Elsevier, vol. 228(C).

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:gam:jeners:v:15:y:2022:i:18:p:6751-:d:915798. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: MDPI Indexing Manager (email available below). General contact details of provider: https://www.mdpi.com .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.