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Modelling Carbon Corrosion during a PEMFC Startup: Simulation of Mitigation Strategies

Author

Listed:
  • Bolahaga Randrianarizafy

    (LITEN, CEA, Univ. Grenoble Alpes, F-38054 Grenoble, France)

  • Pascal Schott

    (LITEN, CEA, Univ. Grenoble Alpes, F-38054 Grenoble, France)

  • Mathias Gerard

    (LITEN, CEA, Univ. Grenoble Alpes, F-38054 Grenoble, France)

  • Yann Bultel

    (LEPMI, Grenoble INP, CNRS, Univ. Savoie Mont Blanc, F-38000 Grenoble, France)

Abstract

This paper presents a study of the carbon support corrosion and mitigation strategies through the use of a pseudo-3D model. This model consists in coupling a 2D model along the channel with another model perpendicular to the flow at the rib/channel scale. Simulations offer a deeper understanding of the corrosion through the analysis of the local conditions. Rib/channel heterogeneities show the higher degradation in the zones facing the anodic rib. These results are validated qualitatively on literature data by analysis of SEM images and carbon dioxide concentration at the cathode outlet. Three mitigation strategies are studied using the model. The first one consists in speeding up the hydrogen filling of the cell. The second strategy involves an external electrical resistance to create a current leak during the startup. Third, a design study of the rib/channel is performed to minimize the cathode degradation. Whatever the mitigation strategy, it consists in reducing either the duration or the magnitude of the high cathode electrode potential.

Suggested Citation

  • Bolahaga Randrianarizafy & Pascal Schott & Mathias Gerard & Yann Bultel, 2020. "Modelling Carbon Corrosion during a PEMFC Startup: Simulation of Mitigation Strategies," Energies, MDPI, vol. 13(9), pages 1-17, May.
    • Handle: RePEc:gam:jeners:v:13:y:2020:i:9:p:2338-:d:355239
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    References listed on IDEAS

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    1. Zhang, Tong & Wang, Peiqi & Chen, Huicui & Pei, Pucheng, 2018. "A review of automotive proton exchange membrane fuel cell degradation under start-stop operating condition," Applied Energy, Elsevier, vol. 223(C), pages 249-262.
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    1. Sim, Jaebong & Kang, Minsoo & Min, Kyoungdoug & Lee, Eunsook & Jyoung, Jy-Young, 2022. "Effects of carbon corrosion on proton exchange membrane fuel cell performance using two durability evaluation methods," Renewable Energy, Elsevier, vol. 190(C), pages 959-970.
    2. Ahmed Mohmed Dafalla & Lin Wei & Bereket Tsegai Habte & Jian Guo & Fangming Jiang, 2022. "Membrane Electrode Assembly Degradation Modeling of Proton Exchange Membrane Fuel Cells: A Review," Energies, MDPI, vol. 15(23), pages 1-26, December.

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