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The Zr-Doped CaO CO 2 Sorbent Fabricated by Wet High-Energy Milling

Author

Listed:
  • Vyacheslav V. Rodaev

    (Institute for Nanotechnology and Nanomaterials, Derzhavin Tambov State University, Internatsionalnaya Street 33, 392000 Tambov, Russia)

  • Svetlana S. Razlivalova

    (Institute for Nanotechnology and Nanomaterials, Derzhavin Tambov State University, Internatsionalnaya Street 33, 392000 Tambov, Russia)

Abstract

We fabricated the Zr-doped CaO sorbent for high-temperature CO 2 capture by the wet high-energy co-milling of calcium carbonate and natural zirconium dioxide (baddeleyite) for the first time. The morphology of the material was examined by scanning electron microscopy, energy-dispersive X-ray analysis and X-ray diffraction. Its CO 2 uptake capacity was determined using thermogravimetric analysis. After 50 carbonation–calcination cycles, the Zr-doped CaO sorbent characterized by a high enough CO 2 uptake capacity of 8.6 mmol/g and unchanged microstructure due to CaZrO 3 nanoparticles uniformly distributed in the CaO matrix to prevent CaCO 3 sintering under carbonation. The proposed easy-to-implement CaO-based sorbents fabrication technique is promising for industrial application.

Suggested Citation

  • Vyacheslav V. Rodaev & Svetlana S. Razlivalova, 2020. "The Zr-Doped CaO CO 2 Sorbent Fabricated by Wet High-Energy Milling," Energies, MDPI, vol. 13(16), pages 1-7, August.
    • Handle: RePEc:gam:jeners:v:13:y:2020:i:16:p:4110-:d:396371
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    References listed on IDEAS

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    1. Antzara, Andy & Heracleous, Eleni & Lemonidou, Angeliki A., 2015. "Improving the stability of synthetic CaO-based CO2 sorbents by structural promoters," Applied Energy, Elsevier, vol. 156(C), pages 331-343.
    2. Najmus S. Sifat & Yousef Haseli, 2019. "A Critical Review of CO 2 Capture Technologies and Prospects for Clean Power Generation," Energies, MDPI, vol. 12(21), pages 1-33, October.
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