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Study of MgO-based dry regenerable sorbent for sorption enhanced water gas shift reaction

Author

Listed:
  • Choi, Dong-Hyeok
  • Lee, Joong Beom
  • Eom, Tae Hyoung
  • Baek, Jeom In
  • Jegarl, Seong
  • Ryu, Chong Kul

Abstract

CO2 sorption capacities and physical properties of the MgO-based sorbent, and the effect of steam during the sorbent regeneration were studied. Four MgO-based dry regenerable sorbents (P-A ∼ D) were prepared by spray drying method for the application to pre-combustion CO2 capture. Physical properties of the sorbents were measured by standard ASTM methods. MgO-based sorbents satisfied with most of the physical requirements for commercial fluidized-bed process. All sorbents had a spherical shape and an average size of 106 ± 10 μm. Most of the attrition index (AI) of the sorbents except for P-D was below 12%, which was superior, compared to commercial fluidized catalytic cracking (FCC) catalysts. CO2 sorption capacities were evaluated by multi-cycle test in a high pressure bubbling fluidized-bed reactor at 473 K and 20 bar with 37% CO2. The sorption capacities of the sorbents showed 3.3–14.5 wt% during 3 cycle. Particularly, P-A showed a high CO2 sorption capacity of more than 14 wt%. In this study, CO2 sorption capacity of steam-treated sorbent was higher than non-treated sorbent. This result can be explained by the presence of Mg(OH)2 formed by hydroxylation by MgO and increasing surface area of steam-treated sorbent.

Suggested Citation

  • Choi, Dong-Hyeok & Lee, Joong Beom & Eom, Tae Hyoung & Baek, Jeom In & Jegarl, Seong & Ryu, Chong Kul, 2013. "Study of MgO-based dry regenerable sorbent for sorption enhanced water gas shift reaction," Renewable Energy, Elsevier, vol. 54(C), pages 144-149.
    • Handle: RePEc:eee:renene:v:54:y:2013:i:c:p:144-149
    DOI: 10.1016/j.renene.2012.08.044
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    References listed on IDEAS

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    1. Barelli, L. & Bidini, G. & Gallorini, F. & Servili, S., 2008. "Hydrogen production through sorption-enhanced steam methane reforming and membrane technology: A review," Energy, Elsevier, vol. 33(4), pages 554-570.
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    1. Gao, Wanlin & Zhou, Tuantuan & Gao, Yanshan & Wang, Qiang, 2019. "Enhanced water gas shift processes for carbon dioxide capture and hydrogen production," Applied Energy, Elsevier, vol. 254(C).

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