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Carbon nanofiber-supported tantalum oxides as durable catalyst for the oxygen evolution reaction in alkaline media

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  • Ruiz-Cornejo, J.C.
  • Vivo-Vilches, J.F.
  • Sebastián, D.
  • Martínez-Huerta, M.V.
  • Lázaro, M.J.

Abstract

Active and durable electrocatalysts for the oxygen evolution reaction (OER), capable of replacing noble metal catalysts, are required to develop efficient and competitive devices within the frame of the water electrolysis technology for hydrogen production. In this work, we have investigated tantalum based catalysts supported on carbon nanofibers (CNF) for the first time. The effect of CNF characteristics and the catalyst annealing temperature on the electrochemical response for the OER have been analyzed in alkaline environment using a rotating ring disc electrode (RRDE). The best OER activity and oxygen efficiency were found with a highly graphitic CNF, despite its lower surface area, synthesized at 700 °C, and upon a catalyst annealing temperature of 800 °C. The ordering degree of carbon nanofibers favors the production of oxygen in combination with a low oxygen content in tantalum oxides. The most active catalyst exhibited also an excellent durability.

Suggested Citation

  • Ruiz-Cornejo, J.C. & Vivo-Vilches, J.F. & Sebastián, D. & Martínez-Huerta, M.V. & Lázaro, M.J., 2021. "Carbon nanofiber-supported tantalum oxides as durable catalyst for the oxygen evolution reaction in alkaline media," Renewable Energy, Elsevier, vol. 178(C), pages 307-317.
    • Handle: RePEc:eee:renene:v:178:y:2021:i:c:p:307-317
    DOI: 10.1016/j.renene.2021.06.076
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    References listed on IDEAS

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    1. Luque-Centeno, J.M. & Martínez-Huerta, M.V. & Sebastián, D. & Lemes, G. & Pastor, E. & Lázaro, M.J., 2018. "Bifunctional N-doped graphene Ti and Co nanocomposites for the oxygen reduction and evolution reactions," Renewable Energy, Elsevier, vol. 125(C), pages 182-192.
    2. Mark K. Debe, 2012. "Electrocatalyst approaches and challenges for automotive fuel cells," Nature, Nature, vol. 486(7401), pages 43-51, June.
    3. Hosseini, Seyed Ehsan & Wahid, Mazlan Abdul, 2016. "Hydrogen production from renewable and sustainable energy resources: Promising green energy carrier for clean development," Renewable and Sustainable Energy Reviews, Elsevier, vol. 57(C), pages 850-866.
    4. Ching-Wei Tung & Ying-Ya Hsu & Yen-Ping Shen & Yixin Zheng & Ting-Shan Chan & Hwo-Shuenn Sheu & Yuan-Chung Cheng & Hao Ming Chen, 2015. "Reversible adapting layer produces robust single-crystal electrocatalyst for oxygen evolution," Nature Communications, Nature, vol. 6(1), pages 1-9, November.
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