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Integrating chromium-based ceramic and acid catalysis to convert glucose into 5-hydroxymethylfurfural

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  • Cui, Mei
  • Wu, Zhongjie
  • Huang, Renliang
  • Qi, Wei
  • Su, Rongxin
  • He, Zhimin

Abstract

5-Hydroxymethylfurfural is an important bio-based chemical that shows broad application potential. In the present study, the use of chitosan nanoparticles was proposed to adsorb and recycle chromium ions from aqueous solution with Cr(III) and Cr(VI) removal rates of up to 97.5% and 81.2%, respectively. A chromium-based ceramic powder catalyst was designed and synthesized, the structural properties of the catalyst were characterized, and the catalytic performances of the catalyst were evaluated. The results showed that after chromium was doped into the blank ceramic, the main lattice structure of the ceramic was preserved. Both the specific surface area and pore diameter decreased, and a portion of the Cr(VI) was transformed to Cr(III). The chromium-based ceramic powder and sulfuric acid co-catalyzed the one-pot synthesis of 5-hydroxymethylfurfural from glucose in the water/dimethyl sulfoxide system, with the product yield reaching 64.7%. After the catalyst was reused 5 times, the product yield was still close to 60%. Thus, the catalyst exhibited good recyclability. The results of this study provide a good example of the one-step synthesis of 5-hydroxymethylfurfural from glucose.

Suggested Citation

  • Cui, Mei & Wu, Zhongjie & Huang, Renliang & Qi, Wei & Su, Rongxin & He, Zhimin, 2018. "Integrating chromium-based ceramic and acid catalysis to convert glucose into 5-hydroxymethylfurfural," Renewable Energy, Elsevier, vol. 125(C), pages 327-333.
    • Handle: RePEc:eee:renene:v:125:y:2018:i:c:p:327-333
    DOI: 10.1016/j.renene.2018.02.085
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    References listed on IDEAS

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    1. Argun, Hidayet & Onaran, Gülizar, 2016. "Glucose and 5-hydroxymethylfurfural production from cellulosic waste by sequential alkaline and acid hydrolysis," Renewable Energy, Elsevier, vol. 96(PA), pages 442-449.
    2. Yuriy Román-Leshkov & Christopher J. Barrett & Zhen Y. Liu & James A. Dumesic, 2007. "Production of dimethylfuran for liquid fuels from biomass-derived carbohydrates," Nature, Nature, vol. 447(7147), pages 982-985, June.
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    Cited by:

    1. Cai, Bo & Kang, Rui & Guo, Dayi & Feng, Junfeng & Ma, Tianyi & Pan, Hui, 2022. "An eco-friendly acidic catalyst phosphorus-doped graphitic carbon nitride for efficient conversion of fructose to 5-Hydroxymethylfurfural," Renewable Energy, Elsevier, vol. 199(C), pages 1629-1638.
    2. Yang, Fengli & Weng, Jushi & Ding, Jiajing & Zhao, Zhiyan & Qin, Lizhen & Xia, Feifei, 2020. "Effective conversion of saccharides into hydroxymethylfurfural catalyzed by a natural clay, attapulgite," Renewable Energy, Elsevier, vol. 151(C), pages 829-836.
    3. Li, Chao & Sun, Yifan & Li, Qingyang & Zhang, Lijun & Zhang, Shu & Wang, Huaisheng & Hu, Guangzhi & Hu, Xun, 2022. "Effects of volatiles on properties of char during sequential pyrolysis of PET and cellulose," Renewable Energy, Elsevier, vol. 189(C), pages 139-151.

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