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A study of the inhibition properties of gallic acid/lignin-modified hydrogel inhibitor prepared via graft copolymerization

Author

Listed:
  • Huang, Zhian
  • Hu, Zhidan
  • Zhou, Zhengqing
  • Zhang, Yinghua
  • Liu, Qianming
  • Wang, Hongsheng
  • Ding, Hao
  • Di, Xiaoche
  • Jameel, Danish
  • Ren, Jiaze
  • Wang, Pengfei

Abstract

In view of the shortcomings of pure hydrogels, such as a single inhibition effect and poor stability at high temperatures, this study aims to develop a new composite hydrogel inhibitor and to study its inhibition mechanism. To this end, gallic acid and lignin were added to modify the hydrogel, and a gallic acid/lignin-modified hydrogel (GA/LG-PAA) inhibitor was prepared. By scanning electron microscope, it was discovered that inhibited coal samples treated with gallic acid hydrogel (GA-PAA) and GA/LG-PAA had bigger particles. By using thermogravimetric analysis, it was found that after the inhibition treatment with GA/LG-PAA, the coal samples’ characteristic temperature points have increased to different degrees. Among these, the dry cracking temperature was increased by 53.87 °C, the ignition temperature was increased by 20.23 °C, and the burnout temperature was increased by 19.79 °C. Thermogravimetric experiments therefore showed that GA/LG-PAA had the best inhibition effect. Through infrared diffuse reflection experiments, it was found that the peak areas of methylene, carbonyl, carbon-carbon double bond, ether bond and other functional groups were all increased in coal samples after inhibition. The GA/LG-PAA inhibited spontaneous combustion by forming ether bonds. The results show that GA/LG-PAA can effectively inhibit coal spontaneous combustion.

Suggested Citation

  • Huang, Zhian & Hu, Zhidan & Zhou, Zhengqing & Zhang, Yinghua & Liu, Qianming & Wang, Hongsheng & Ding, Hao & Di, Xiaoche & Jameel, Danish & Ren, Jiaze & Wang, Pengfei, 2024. "A study of the inhibition properties of gallic acid/lignin-modified hydrogel inhibitor prepared via graft copolymerization," Energy, Elsevier, vol. 294(C).
    • Handle: RePEc:eee:energy:v:294:y:2024:i:c:s0360544224006376
    DOI: 10.1016/j.energy.2024.130865
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    References listed on IDEAS

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    1. Xu, Xiaoxue & Yuan, Shujie & Li, Jinhu & Guo, Shengli & Yan, Zhuo, 2023. "Preparation of lignin-based intumescent nanogel and its mechanism of inhibiting coal spontaneous combustion," Energy, Elsevier, vol. 275(C).
    2. Fan, Xin-li & Ma, Li & Sheng, You-jie & Liu, Xi-xi & Wei, Gao-ming & Liu, Shang-ming, 2023. "Experimental investigation on the characteristics of XG/GG/HPAM gel foam and prevention of coal spontaneous combustion," Energy, Elsevier, vol. 284(C).
    3. Xi, Xian & Jiang, Shuguang & Shi, Quanlin & Yin, Chenchen, 2023. "Experimental investigation on the leakage plugging and fire extinguishment characteristics of industrial solid waste-based composite foam slurry materials," Energy, Elsevier, vol. 269(C).
    4. Abbasi, Kashif Raza & Shahbaz, Muhammad & Zhang, Jinjun & Irfan, Muhammad & Alvarado, Rafael, 2022. "Analyze the environmental sustainability factors of China: The role of fossil fuel energy and renewable energy," Renewable Energy, Elsevier, vol. 187(C), pages 390-402.
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