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Staged pyrolysis of biomass to probe the evolution of fractions of bio-oil

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  • Li, Chao
  • Li, Yuannian
  • Jiang, Yuchen
  • Zhang, Lijun
  • Zhang, Shu
  • Ding, Kuan
  • Li, Bin
  • Wang, Shuang
  • Hu, Xun

Abstract

Bio-oil is a complex mixture of organics and each group of chemicals has a varied response to pyrolysis temperatures. This was investigated via the staged pyrolysis of poplar sawdust, cellulose, and lignin by consecutively increasing temperature to 250, 350, 450, and 550 °C, respectively. The results showed that 350 °C was the boundary temperature for formation of majority of organics from sawdust and cellulose and more than half of organics from lignin. The further increase of temperature to 550 °C mainly promoted the aromatization of reaction intermediates from aliphatic components. The staged pyrolysis also facilitated the charring reactions, generating the bio-oil with more light organics including anhydrate sugars, ketones, aldehydes, and phenolics. The enhanced charring reactions promoted the carbonization reactions via deoxygenation, making biochar carbon-rich and thermally more stable. Additionally, the staged pyrolysis also impacted the morphologies and evolution of the functionalities of biochar via influencing the volatile-char interactions.

Suggested Citation

  • Li, Chao & Li, Yuannian & Jiang, Yuchen & Zhang, Lijun & Zhang, Shu & Ding, Kuan & Li, Bin & Wang, Shuang & Hu, Xun, 2023. "Staged pyrolysis of biomass to probe the evolution of fractions of bio-oil," Energy, Elsevier, vol. 263(PD).
    • Handle: RePEc:eee:energy:v:263:y:2023:i:pd:s0360544222027591
    DOI: 10.1016/j.energy.2022.125873
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    1. Ren, Xueyong & Shanb Ghazani, Mohammad & Zhu, Hui & Ao, Wenya & Zhang, Han & Moreside, Emma & Zhu, Jinjiao & Yang, Pu & Zhong, Na & Bi, Xiaotao, 2022. "Challenges and opportunities in microwave-assisted catalytic pyrolysis of biomass: A review," Applied Energy, Elsevier, vol. 315(C).
    2. Ge, Shengbo & Yek, Peter Nai Yuh & Cheng, Yoke Wang & Xia, Changlei & Wan Mahari, Wan Adibah & Liew, Rock Keey & Peng, Wanxi & Yuan, Tong-Qi & Tabatabaei, Meisam & Aghbashlo, Mortaza & Sonne, Christia, 2021. "Progress in microwave pyrolysis conversion of agricultural waste to value-added biofuels: A batch to continuous approach," Renewable and Sustainable Energy Reviews, Elsevier, vol. 135(C).
    3. Zhang, Chenting & Chao, Li & Zhang, Zhanming & Zhang, Lijun & Li, Qingyin & Fan, Huailin & Zhang, Shu & Liu, Qing & Qiao, Yingyun & Tian, Yuanyu & Wang, Yi & Hu, Xun, 2021. "Pyrolysis of cellulose: Evolution of functionalities and structure of bio-char versus temperature," Renewable and Sustainable Energy Reviews, Elsevier, vol. 135(C).
    4. Zhong, Dian & Zeng, Kuo & Li, Jun & Qiu, Yi & Flamant, Gilles & Nzihou, Ange & Vladimirovich, Vasilevich Sergey & Yang, Haiping & Chen, Hanping, 2022. "Characteristics and evolution of heavy components in bio-oil from the pyrolysis of cellulose, hemicellulose and lignin," Renewable and Sustainable Energy Reviews, Elsevier, vol. 157(C).
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    1. Ali Abdulkhani & Zahra Echresh Zadeh & Solomon Gajere Bawa & Fubao Sun & Meysam Madadi & Xueming Zhang & Basudeb Saha, 2023. "Comparative Production of Bio-Oil from In Situ Catalytic Upgrading of Fast Pyrolysis of Lignocellulosic Biomass," Energies, MDPI, vol. 16(6), pages 1-19, March.

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