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Characteristics and kinetic analysis of pyrolysis of forestry waste promoted by microwave-metal interaction

Author

Listed:
  • Li, Longzhi
  • Tan, Yongdong
  • Sun, Jifu
  • Zhang, Yue
  • Zhang, Lianjie
  • Deng, Yue
  • Cai, Dongqiang
  • Song, Zhanlong
  • Zou, Guifu
  • Bai, Yonghui

Abstract

In the present work, a method of pyrolyzing forestry waste (FW) under microwave-metal interaction was proposed. The kinetic analysis of the process was carried out using a microwave thermogravimetric analyzer. The mechanism of FW pyrolysis under microwave-metal interaction was discussed from the perspective of microwave-induced metal discharge and non-discharge processes. The initial pyrolysis temperature Ti reduced, and the maximum pyrolysis rate Rm and pyrolysis characteristic index S increased by employing a method where microwave and metal were coupled. The number of metals inserted also significantly affected the pyrolysis behavior. Rm in the presence of one metal was 92.3% higher than that recorded in the absence of metal. The results of kinetic analysis revealed in the presence of metal, the activation energies at 400 W and 560 W were 51.7% and 57.5% lower, respectively, than the activation energy recorded in the absence of metal. Multiple effects of light, heat, and plasma produced by microwave-induced discharge caused the local pyrolysis of FW. The promotion of FW pyrolysis in the non-discharge stage was primarily caused by the microwave absorption of carbon into heat and the conversion of current on the metal surface into Joule heat.

Suggested Citation

  • Li, Longzhi & Tan, Yongdong & Sun, Jifu & Zhang, Yue & Zhang, Lianjie & Deng, Yue & Cai, Dongqiang & Song, Zhanlong & Zou, Guifu & Bai, Yonghui, 2021. "Characteristics and kinetic analysis of pyrolysis of forestry waste promoted by microwave-metal interaction," Energy, Elsevier, vol. 232(C).
    • Handle: RePEc:eee:energy:v:232:y:2021:i:c:s0360544221013438
    DOI: 10.1016/j.energy.2021.121095
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    References listed on IDEAS

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    1. Li, Longzhi & Cao, Kangqi & Cai, Dongqiang & Zhang, Zhonglei & Zhao, Zhiyang & Yu, Miao & Zhang, Lianjie & Zhang, Qiang & Zou, Guifu & Wang, Cuiping, 2023. "Influences of iron additives on microwave-assisted pyrolysis of woody biomass and microwave-induced discharge with spherical bio-char," Energy, Elsevier, vol. 276(C).
    2. Zhang, Lianjie & Tan, Yongdong & Cai, Dongqiang & Sun, Jifu & Zhang, Yue & Li, Longzhi & Zhang, Qiang & Zou, Guifu & Song, Zhanlong & Bai, Yonghui, 2022. "Enhanced pyrolysis of woody biomass under interaction of microwave and needle-shape metal and its production properties," Energy, Elsevier, vol. 249(C).
    3. Li, Longzhi & Cai, Dongqiang & Zhang, Lianjie & Zhang, Yue & Zhao, Zhiyang & Zhang, Zhonglei & Sun, Jifu & Tan, Yongdong & Zou, Guifu, 2023. "Synergistic effects during pyrolysis of binary mixtures of biomass components using microwave-assisted heating coupled with iron base tip-metal," Renewable Energy, Elsevier, vol. 203(C), pages 312-322.

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