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Kinetic parameters of petroleum coke gasification for modelling chemical-looping combustion systems

Author

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  • Korus, Agnieszka
  • Klimanek, Adam
  • Sładek, Sławomir
  • Szlęk, Andrzej
  • Tilland, Airy
  • Bertholin, Stéphane
  • Haugen, Nils Erland L.

Abstract

One of the best low-cost approaches for capturing carbon dioxide from the combustion of solid fuels is chemical looping combustion (CLC) technology, where the processes of fuel oxidation and extraction of oxygen from the air are split in two separate reactors. In order to model the petroleum coke (petcoke) conversion in a CLC method, detailed knowledge about the reactions of pet-coke with O2, CO2, and H2O at temperatures between 750 and 1100 °C is required. Due to the lack of sufficient literature data, in this paper, the reactivity of these reactions is investigated in a custom-built test rig that enabled measurements of the mass loss of the fuel sample and the composition of the released gases. The Avrami, Random Pore, Shrinking Core, and Hybrid models were applied to the experimental results to determine the kinetic parameters of petcoke gasification. At temperatures up to 1000 °C, the reaction with CO2 was found to be negligibly slow. An activation energy of 103.91 kJ/mol was obtained for petcoke gasification in 10–40 vol% of H2O, while a value of 15.87 kJ/mol was found for oxidation in 2–4 vol% O2, as described by best-fitting models, i.e. Hybrid and Random Pore models, respectively.

Suggested Citation

  • Korus, Agnieszka & Klimanek, Adam & Sładek, Sławomir & Szlęk, Andrzej & Tilland, Airy & Bertholin, Stéphane & Haugen, Nils Erland L., 2021. "Kinetic parameters of petroleum coke gasification for modelling chemical-looping combustion systems," Energy, Elsevier, vol. 232(C).
    • Handle: RePEc:eee:energy:v:232:y:2021:i:c:s036054422101183x
    DOI: 10.1016/j.energy.2021.120935
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    References listed on IDEAS

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    1. Wei, Juntao & Guo, Qinghua & Gong, Yan & Ding, Lu & Yu, Guangsuo, 2020. "Effect of biomass leachates on structure evolution and reactivity characteristic of petroleum coke gasification," Renewable Energy, Elsevier, vol. 155(C), pages 111-120.
    2. Zhan, Xiuli & Zhou, ZhiJie & Wang, Fuchen, 2010. "Catalytic effect of black liquor on the gasification reactivity of petroleum coke," Applied Energy, Elsevier, vol. 87(5), pages 1710-1715, May.
    3. Karasu, Seçkin & Altan, Aytaç & Bekiros, Stelios & Ahmad, Wasim, 2020. "A new forecasting model with wrapper-based feature selection approach using multi-objective optimization technique for chaotic crude oil time series," Energy, Elsevier, vol. 212(C).
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    1. Ding, Haoran & Tong, Sirui & Qi, Zhifu & Liu, Fei & Sun, Shien & Han, Long, 2023. "Syngas production from chemical-looping steam methane reforming: The effect of channel geometry on BaCoO3/CeO2 monolithic oxygen carriers," Energy, Elsevier, vol. 263(PE).
    2. Gao, Zhuwei & Li, Chengxin & Qi, Xinyu & Wei, Yaodong & Liu, Zhongxin, 2022. "Flow analysis on carbonaceous deposition of heavy oil droplets and catalyst particles for coking formation process," Energy, Elsevier, vol. 260(C).
    3. Liyan Sun & Junjie Lin & Dali Kong & Kun Luo & Jianren Fan, 2022. "Numerical Simulation of a 10 kW Gas-Fueled Chemical Looping Combustion Unit," Energies, MDPI, vol. 15(6), pages 1-11, March.

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