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CeO2-modified CaO/Ca12Al14O33 bi-functional material for CO2 capture and H2 production in sorption-enhanced steam gasification of biomass

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  • Yan, Xianyao
  • Li, Yingjie
  • Ma, Xiaotong
  • Bian, Zhiguo
  • Zhao, Jianli
  • Wang, Zeyan

Abstract

A novel CeO2-modified CaO/Ca12Al14O33 bi-functional material fabricated by wet-mixing method was used in sorption-enhanced steam gasification of biomass for H2 production. The CO2 capture performance of the bi-functional material was investigated during the multiple carbonation/calcination cycles in a dual fixed-bed reactor. H2 production from the sorption-enhanced steam gasification of bagasse char using CeO2-modified CaO/Ca12Al14O33 was studied. When the mass ratio of CaO/Ca12Al14O33/CeO2 is 75:10:15, CO2 capture capacity of CeO2-modified CaO/Ca12Al14O33 reaches 0.48 g/g after 20 cycles under the realistic calcination condition, which is 30% higher than that of CaO/Ca12Al14O33. The average H2 concentration and yield using CeO2-modified CaO/Ca12Al14O33 during 10 cycles achieve 81.1 vol% and 0.124 L/g, which are 17.4% and 47.3% higher than those using CaO/Ca12Al14O33, respectively. CeO2 in CeO2-modified CaO/Ca12Al14O33 enhances water gas shift and steam methane reforming reactions. CeO2-modified CaO/Ca12Al14O33 possesses stronger basicity, and Ce3+ in the surface creates oxygen vacancies and promotes the conductivity of lattice oxygen, which are favorable for CO2 capture. CeO2 improves the cyclic stability of CaO/Ca12Al14O33 and stabilizes pores in 10–100 nm in diameter, which facilitates CO2 capture and H2 production. Thus, CeO2-modified CaO/Ca12Al14O33 appears promising for H2 production from the sorption-enhanced steam gasification of biomass.

Suggested Citation

  • Yan, Xianyao & Li, Yingjie & Ma, Xiaotong & Bian, Zhiguo & Zhao, Jianli & Wang, Zeyan, 2020. "CeO2-modified CaO/Ca12Al14O33 bi-functional material for CO2 capture and H2 production in sorption-enhanced steam gasification of biomass," Energy, Elsevier, vol. 192(C).
    • Handle: RePEc:eee:energy:v:192:y:2020:i:c:s036054421932359x
    DOI: 10.1016/j.energy.2019.116664
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    Cited by:

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    2. Arnob Das & Susmita Datta Peu, 2022. "A Comprehensive Review on Recent Advancements in Thermochemical Processes for Clean Hydrogen Production to Decarbonize the Energy Sector," Sustainability, MDPI, vol. 14(18), pages 1-42, September.
    3. Xiao Liang & Huichao Chen, 2021. "Utilization of biomass to promote calcium‐based sorbents for CO2 capture," Greenhouse Gases: Science and Technology, Blackwell Publishing, vol. 11(5), pages 837-855, October.
    4. Wang, Chao & Liao, Mingzheng & Jiang, Zhiqiang & Liang, Bo & Weng, Jiahong & Song, Qingbin & Zhao, Ming & Chen, Ying & Lei, Libin, 2022. "Sorption-enhanced propane partial oxidation hydrogen production for solid oxide fuel cell (SOFC) applications," Energy, Elsevier, vol. 247(C).
    5. Liu, Rui & Li, Chongcong & Zheng, Jinhao & Xue, Feilong & Yang, Mingjun & Zhang, Yan, 2023. "Hydrogen-rich syngas production via sorption-enhanced steam gasification of biomass using FexNiyCaO bi-functional materials," Energy, Elsevier, vol. 281(C).
    6. Xiaoquan Zhou & Liguo Yang & Xiaoxu Fan & Xuanyou Li, 2023. "Experimental Study on the Preparation of Hydrogen-Rich Gas by Gasifying of Traditional Chinese Medicine Residue in a DFB Based on Calcium Looping," Energies, MDPI, vol. 16(11), pages 1-13, May.
    7. Yan, Xianyao & Li, Yingjie & Sun, Chaoying & Zhang, Chunxiao & Yang, Liguo & Fan, Xiaoxu & Chu, Leizhe, 2022. "Enhanced H2 production from steam gasification of biomass by red mud-doped Ca-Al-Ce bi-functional material," Applied Energy, Elsevier, vol. 312(C).

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    More about this item

    Keywords

    Sorption-enhanced steam gasification; Bagasse char; CO2 capture; H2 production; Bi-functional material; CeO2-Modified CaO/Ca12Al14O33;
    All these keywords.

    JEL classification:

    • H2 - Public Economics - - Taxation, Subsidies, and Revenue

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