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Enhanced stability of Ni/SiO2 catalyst for CO2 methanation: Derived from nickel phyllosilicate with strong metal-support interactions

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Listed:
  • Ye, Run-Ping
  • Gong, Weibo
  • Sun, Zhao
  • Sheng, Qingtao
  • Shi, Xiufeng
  • Wang, Tongtong
  • Yao, Yi
  • Razink, Joshua J.
  • Lin, Ling
  • Zhou, Zhangfeng
  • Adidharma, Hertanto
  • Tang, Jinke
  • Fan, Maohong
  • Yao, Yuan-Gen

Abstract

Nowadays more and more significant technologies have been developing to save energy and reduce emissions. CO2 methanation has been an attractive process to reduce CO2-emissions since it consumes CO2 with H2 derived from renewable energy sources to produce CH4. However, the poor stability of Ni-based catalyst for CO2 methanation is still challenging. Herein, two Ni/SiO2 catalysts with different structure and catalytic properties were prepared by different methods. The Ni/SiO2-AEM nanocatalyst with a lamellar structure of nickel phyllosilicate was synthesized by a facile ammonia-evaporation method (AEM), which can conveniently and uniformly disperse nickel species on SiO2. Upon reduction of nickel phyllosilicate, it can disperse and confine small sized Ni particles (4.2 nm) in the silica support with a high surface area of 446.3 m2/g, leading to the Ni/SiO2-AEM catalyst achieving a high yield of methane with long-term stability of 100 h under the GHSV of 10,000 mL/(gcat h) and another 60 h with the GHSV increased to 30,000 mL/(gcat h) at 370 °C. In comparison, the Ni/SiO2-IM catalyst prepared by the impregnation method obtained lower yield of methane and worse stability under identical conditions. The results indicate that the catalyst with high surface area and strong metal-support interactions can improve stability.

Suggested Citation

  • Ye, Run-Ping & Gong, Weibo & Sun, Zhao & Sheng, Qingtao & Shi, Xiufeng & Wang, Tongtong & Yao, Yi & Razink, Joshua J. & Lin, Ling & Zhou, Zhangfeng & Adidharma, Hertanto & Tang, Jinke & Fan, Maohong &, 2019. "Enhanced stability of Ni/SiO2 catalyst for CO2 methanation: Derived from nickel phyllosilicate with strong metal-support interactions," Energy, Elsevier, vol. 188(C).
  • Handle: RePEc:eee:energy:v:188:y:2019:i:c:s0360544219317542
    DOI: 10.1016/j.energy.2019.116059
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    References listed on IDEAS

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    1. Yang, Yu & Liu, Jing & Shen, Weifeng & Li, Jie & Chien, I-Lung, 2018. "High-efficiency utilization of CO2 in the methanol production by a novel parallel-series system combining steam and dry methane reforming," Energy, Elsevier, vol. 158(C), pages 820-829.
    2. Veselovskaya, Janna V. & Parunin, Pavel D. & Netskina, Olga V. & Kibis, Lidiya S. & Lysikov, Anton I. & Okunev, Aleksey G., 2018. "Catalytic methanation of carbon dioxide captured from ambient air," Energy, Elsevier, vol. 159(C), pages 766-773.
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    Cited by:

    1. Soohyun Kim & Yunxia Yang & Renata Lippi & Hokyung Choi & Sangdo Kim & Donghyuk Chun & Hyuk Im & Sihyun Lee & Jiho Yoo, 2021. "Low-Rank Coal Supported Ni Catalysts for CO 2 Methanation," Energies, MDPI, vol. 14(8), pages 1-13, April.
    2. Nam, Hyungseok & Kim, Jung Hwan & Kim, Hana & Kim, Min Jae & Jeon, Sang-Goo & Jin, Gyoung-Tae & Won, Yooseob & Hwang, Byung Wook & Lee, Seung-Yong & Baek, Jeom-In & Lee, Doyeon & Seo, Myung Won & Ryu,, 2021. "CO2 methanation in a bench-scale bubbling fluidized bed reactor using Ni-based catalyst and its exothermic heat transfer analysis," Energy, Elsevier, vol. 214(C).
    3. Martyna Przydacz & Marcin Jędrzejczyk & Jacek Rogowski & Małgorzata Szynkowska-Jóźwik & Agnieszka M. Ruppert, 2020. "Highly Efficient Production of DMF from Biomass-Derived HMF on Recyclable Ni-Fe/TiO 2 Catalysts," Energies, MDPI, vol. 13(18), pages 1-14, September.
    4. Ahmed Aheed Ali Mohammed & Mohammed Ali H Saleh Saad & Anand Kumar & Mohammed J Al‐Marri, 2020. "Synthesis of fumed silica supported Ni catalyst for carbon dioxide conversion to methane," Greenhouse Gases: Science and Technology, Blackwell Publishing, vol. 10(4), pages 715-724, August.
    5. Alves, Luís & Pereira, Vítor & Lagarteira, Tiago & Mendes, Adélio, 2021. "Catalytic methane decomposition to boost the energy transition: Scientific and technological advancements," Renewable and Sustainable Energy Reviews, Elsevier, vol. 137(C).

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