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Computational model of a sulfur-iodine thermochemical water splitting system coupled to a VHTR for nuclear hydrogen production

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  • González Rodríguez, Daniel
  • Brayner de Oliveira Lira, Carlos Alberto
  • García Parra, Lázaro Roger
  • García Hernández, Carlos Rafael
  • de la Torre Valdés, Raciel

Abstract

Sulfur-Iodine thermochemical water splitting cycle coupled is one of the most promising methods for hydrogen production using a nuclear reactor as the primary energy source. However, there are not references in the scientific publications of a test facility that allow to evaluate the efficiency of the overall process. A computational model for the evaluation and optimization of the sulfur-iodine cycle coupled to a very high temperature reactor for nuclear hydrogen production was developed using a chemical process simulator Aspen HYSYS®. Some operational and design parameters of the cycle sections can be optimized in order to obtain the maximum hydrogen production and higher efficiency. The optimized sections of the flowsheet are coupled to a very high temperature nuclear system (TADSEA) through a Brayton gas cycle for power cogeneration. It is proposed a closed flowsheet for the sulfur-iodine thermochemical water splitting cycle coupled to an accelerator driven system, considering a Brayton cycle for the energy production. It is obtained an acceptable value of global efficiency for the initial operating condition. Several parametric studies are conducted using the flowsheet proposed to evaluate important operating parameters in the overall process efficiency.

Suggested Citation

  • González Rodríguez, Daniel & Brayner de Oliveira Lira, Carlos Alberto & García Parra, Lázaro Roger & García Hernández, Carlos Rafael & de la Torre Valdés, Raciel, 2018. "Computational model of a sulfur-iodine thermochemical water splitting system coupled to a VHTR for nuclear hydrogen production," Energy, Elsevier, vol. 147(C), pages 1165-1176.
    • Handle: RePEc:eee:energy:v:147:y:2018:i:c:p:1165-1176
    DOI: 10.1016/j.energy.2017.12.031
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    References listed on IDEAS

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    Cited by:

    1. Wang, Qi & Macián-Juan, Rafael, 2022. "Thermodynamic analysis of two novel very high temperature gas-cooled reactor-based hydrogen-electricity cogeneration systems using sulfur-iodine cycle and gas-steam combined cycle," Energy, Elsevier, vol. 256(C).
    2. Kumar, Dinesh & Bahauddin Alam, Syed & Ridwan, Tuhfatur & Goodwin, Cameron S., 2021. "Quantitative risk assessment of a high power density small modular reactor (SMR) core using uncertainty and sensitivity analyses," Energy, Elsevier, vol. 227(C).
    3. Ni, Hang & Qu, Xinhe & Zhao, Gang & Zhang, Ping & Peng, Wei, 2024. "Research on two novel hydrogen-electricity-heat polygeneration systems using very-high-temperature gas-cooled reactor and hybrid-sulfur cycle," Energy, Elsevier, vol. 290(C).
    4. Benim, Ali Cemal & Pfeiffelmann, Björn & Ocłoń, Paweł & Taler, Jan, 2019. "Computational investigation of a lifted hydrogen flame with LES and FGM," Energy, Elsevier, vol. 173(C), pages 1172-1181.
    5. Ni, Hang & Peng, Wei & Qu, Xinhe & Zhao, Gang & Zhang, Ping & Wang, Jie, 2022. "Thermodynamic analysis of a novel hydrogen–electricity–heat polygeneration system based on a very high-temperature gas-cooled reactor," Energy, Elsevier, vol. 249(C).
    6. Ni, Hang & Qu, Xinhe & Peng, Wei & Zhao, Gang & Zhang, Ping, 2023. "Study of two innovative hydrogen and electricity co-production systems based on very-high-temperature gas-cooled reactors," Energy, Elsevier, vol. 273(C).

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