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Nickel catalytic graphitized porous carbon as electrode material for high performance supercapacitors

Author

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  • Wang, Keliang
  • Cao, Yuhe
  • Wang, Xiaomin
  • Kharel, Parashu Ram
  • Gibbons, William
  • Luo, Bing
  • Gu, Zhengrong
  • Fan, Qihua
  • Metzger, Lloyd

Abstract

Whey-protein-derived nitrogen-doped porous carbon has been prepared by preliminary carbonization at 400 °C and final KOH activation at 700 °C combined with catalytic graphitization. Physical characterization indicated that the nitrogen-doped activated electrode material had a large specific surface area (2536 m2 g−1) and plenty of interconnected cavities, which greatly improved the performance of supercapacitors. Electrochemical measurements demonstrated that the as-prepared activated electrode material had exceptionally high capacitance of 248 F g−1 at charge/discharge current density of 0.1 A g−1. Moreover, the prepared supercapacitors exhibited ideal capacitive behavior with nearly no capacitance loss in 6 mol L−1 KOH at different charge/discharge current densities ranging from 0.1 to 5 A g−1 after 1000 charge/discharge cycles. The derived energy density was 12.4 Wh kg−1 at a power density of 495 W kg−1 under operational conditions. These results suggested that the whey-protein-derived porous carbon is a promising supercapacitor electrode material.

Suggested Citation

  • Wang, Keliang & Cao, Yuhe & Wang, Xiaomin & Kharel, Parashu Ram & Gibbons, William & Luo, Bing & Gu, Zhengrong & Fan, Qihua & Metzger, Lloyd, 2016. "Nickel catalytic graphitized porous carbon as electrode material for high performance supercapacitors," Energy, Elsevier, vol. 101(C), pages 9-15.
    • Handle: RePEc:eee:energy:v:101:y:2016:i:c:p:9-15
    DOI: 10.1016/j.energy.2016.01.059
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    References listed on IDEAS

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    1. Shao, Zhou & Li, Hongji & Li, Mingji & Li, Cuiping & Qu, Changqing & Yang, Baohe, 2015. "Fabrication of polyaniline nanowire/TiO2 nanotube array electrode for supercapacitors," Energy, Elsevier, vol. 87(C), pages 578-585.
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    1. Xu, Le & Zhao, Yan & Lian, Jiabiao & Xu, Yuanguo & Bao, Jian & Qiu, Jingxia & Xu, Li & Xu, Hui & Hua, Mingqing & Li, Huaming, 2017. "Morphology controlled preparation of ZnCo2O4 nanostructures for asymmetric supercapacitor with ultrahigh energy density," Energy, Elsevier, vol. 123(C), pages 296-304.
    2. Zhang, Shuping & Yin, Haoxin & Wang, Jiaxing & Zhu, Shuguang & Xiong, Yuanquan, 2021. "Catalytic cracking of biomass tar using Ni nanoparticles embedded carbon nanofiber/porous carbon catalysts," Energy, Elsevier, vol. 216(C).
    3. Zhang, Jijun & Chen, Zexiang & Wang, Yan & Li, Hai, 2016. "Morphology-controllable synthesis of 3D CoNiO2 nano-networks as a high-performance positive electrode material for supercapacitors," Energy, Elsevier, vol. 113(C), pages 943-948.
    4. Yoon, Sang Jun & Kim, Sangwon & Kim, Dong Kyu, 2019. "Optimization of local porosity in the electrode as an advanced channel for all-vanadium redox flow battery," Energy, Elsevier, vol. 172(C), pages 26-35.

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