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Aqueous phase reforming of sorbitol to bio-gasoline over Ni/HZSM-5 catalysts

Author

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  • Zhang, Qing
  • Wang, Tiejun
  • Li, Bing
  • Jiang, Ting
  • Ma, Longlong
  • Zhang, Xinghua
  • Liu, Qiying

Abstract

Liquid fuel such as bio-gasoline derived from biomass is widely recognized as a potential substitution for the diminishing fossil fuels due to its abundance of raw materials and lower greenhouse gas emissions. In this work, Ni/HZSM-5 catalysts were developed by incipient impregnation method and applied in the bio-gasoline production by aqueous phase reforming of sorbitol. The effects of reaction temperature, hydrogen pressure and calcination temperature of the catalysts on the catalytic performance were investigated. The activity test results showed that the catalyst calcined at 500°C had the maximal activity with 47.6% of the bio-gasoline yield and 76.4% of the total selectivity of lighter alkanes (C5C6) at 240°C and 4.0MPa. The catalysts were characterized by N2 physical adsorption, H2 temperature-programmed reduction (H2TPR), H2 temperature-programmed desorption (H2TPD), and infrared spectroscopy (IR) techniques. The characterization results revealed that the catalyst calcined at 500°C can provide optimum surface area and pore volume for the reaction. Moreover, 100% of the reducibility of Ni species was detected on the surface of HZSM-5, following by more nickel active sites, which led to a visible increase in the yield of bio-gasoline.

Suggested Citation

  • Zhang, Qing & Wang, Tiejun & Li, Bing & Jiang, Ting & Ma, Longlong & Zhang, Xinghua & Liu, Qiying, 2012. "Aqueous phase reforming of sorbitol to bio-gasoline over Ni/HZSM-5 catalysts," Applied Energy, Elsevier, vol. 97(C), pages 509-513.
    • Handle: RePEc:eee:appene:v:97:y:2012:i:c:p:509-513
    DOI: 10.1016/j.apenergy.2011.12.044
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    Cited by:

    1. Zhang, Xiaowen & Liu, Helei & Liang, Zhiwu & Idem, Raphael & Tontiwachwuthikul, Paitoon & Jaber Al-Marri, Mohammed & Benamor, Abdelbaki, 2018. "Reducing energy consumption of CO2 desorption in CO2-loaded aqueous amine solution using Al2O3/HZSM-5 bifunctional catalysts," Applied Energy, Elsevier, vol. 229(C), pages 562-576.
    2. Xu, Chunping & Paone, Emilia & Rodríguez-Padrón, Daily & Luque, Rafael & Mauriello, Francesco, 2020. "Reductive catalytic routes towards sustainable production of hydrogen, fuels and chemicals from biomass derived polyols," Renewable and Sustainable Energy Reviews, Elsevier, vol. 127(C).
    3. Shamsul, N.S. & Kamarudin, S.K. & Rahman, N.A., 2017. "Conversion of bio-oil to bio gasoline via pyrolysis and hydrothermal: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 80(C), pages 538-549.
    4. Wang, Tiejun & Qiu, Songbai & Weng, Yujing & Chen, Lungang & Liu, Qiying & Long, Jinxing & Tan, Jin & Zhang, Qing & Zhang, Qi & Ma, Longlong, 2015. "Liquid fuel production by aqueous phase catalytic transformation of biomass for aviation," Applied Energy, Elsevier, vol. 160(C), pages 329-335.
    5. Balasundram, Vekes & Ibrahim, Norazana & Kasmani, Rafiziana Md. & Isha, Ruzinah & Hamid, Mohd. Kamaruddin Abd. & Hasbullah, Hasrinah & Ali, Roshafima Rasit, 2018. "Catalytic upgrading of sugarcane bagasse pyrolysis vapours over rare earth metal (Ce) loaded HZSM-5: Effect of catalyst to biomass ratio on the organic compounds in pyrolysis oil," Applied Energy, Elsevier, vol. 220(C), pages 787-799.
    6. Wang, Tiejun & Yang, Yong & Ding, Mingyue & Liu, Qiying & Ma, Longlong, 2013. "Auto-thermal reforming of biomass raw fuel gas to syngas in a novel reformer: Promotion of hot-electron," Applied Energy, Elsevier, vol. 112(C), pages 448-453.

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