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Evaluation of a novel multibed heat-integrated vacuum and temperature swing adsorption post-combustion CO2 capture process

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  • Plaza, M.G.
  • Rubiera, F.

Abstract

A novel multibed heat-integrated vacuum and temperature swing adsorption process has been designed to capture 85% of the CO2 emitted by an advanced supercritical coal fired power plant of 820 MWe taken as reference, and to produce a concentrated product with 95% of CO2 using a microporous carbon obtained from olive stones. The overall performance of the post-combustion CO2 capture process has been evaluated from the results of the dynamic simulation of the process at cyclic steady state, using a detailed non-isothermal non-equilibrium dynamic fixed-bed adsorption model that takes into consideration competitive adsorption between the main flue gas components: N2, CO2 and H2O. The proposed process operates between 30 °C and 1.05 bar and 80 °C and 0.05 bar. The specific heat duty of the process, 2.41MJth kg−1 CO2, which is lower than the benchmark amine absorption technology, can be satisfied using waste heat. On the other hand, its electricity consumption, 1.15MJekg−1CO2, is higher. Increasing the pressure of the production step reduces significantly the energy demand of the process, but also its capture rate. Substantial improvements in performance can be expected from adsorbent development. Adsorption is an environmentally benign technology with great potential to mitigate CO2 emissions from industrial processes with unused waste heat sources.

Suggested Citation

  • Plaza, M.G. & Rubiera, F., 2019. "Evaluation of a novel multibed heat-integrated vacuum and temperature swing adsorption post-combustion CO2 capture process," Applied Energy, Elsevier, vol. 250(C), pages 916-925.
    • Handle: RePEc:eee:appene:v:250:y:2019:i:c:p:916-925
    DOI: 10.1016/j.apenergy.2019.05.079
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    References listed on IDEAS

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    Citations

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    2. Yuannan Zheng & Qingzhao Li & Guiyun Zhang & Yang Zhao & Xinxin Liu, 2021. "Evaluation of separation effect for CH4 enrichment from coalbed methane (CBM) under the synergistic action of temperature and pressure based on IAST theory," Greenhouse Gases: Science and Technology, Blackwell Publishing, vol. 11(3), pages 590-605, June.
    3. Xie, Heping & Gao, Xiaolin & Liu, Tao & Chen, Bin & Wu, Yifan & Jiang, Wenchuan, 2020. "Electricity generation by a novel CO2 mineralization cell based on organic proton-coupled electron transfer," Applied Energy, Elsevier, vol. 261(C).
    4. Wilkes, Mathew Dennis & Brown, Solomon, 2022. "Flexible CO2 capture for open-cycle gas turbines via vacuum-pressure swing adsorption: A model-based assessment," Energy, Elsevier, vol. 250(C).
    5. Yang, Chuanruo & Du, Zhilin & Jin, Junsu & Chen, Jian & Mi, Jianguo, 2020. "Epoxide-functionalized tetraethylenepentamine encapsulated into porous copolymer spheres for CO2 capture with superior stability," Applied Energy, Elsevier, vol. 260(C).
    6. Akinola, Toluleke E. & Bonilla Prado, Phebe L. & Wang, Meihong, 2022. "Experimental studies, molecular simulation and process modelling\simulation of adsorption-based post-combustion carbon capture for power plants: A state-of-the-art review," Applied Energy, Elsevier, vol. 317(C).
    7. Liu, W. & Ji, Y. & Wang, R.Q. & Zhang, X.J. & Jiang, L., 2023. "Analysis on temperature vacuum swing adsorption integrated with heat pump for efficient carbon capture," Applied Energy, Elsevier, vol. 335(C).

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    Keywords

    CO2 capture; Adsorption; Simulation; Post-combustion;
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