IDEAS home Printed from https://ideas.repec.org/a/eee/appene/v237y2019icp314-325.html
   My bibliography  Save this article

Simulation of elevated temperature solid sorbent CO2 capture for pre-combustion applications using computational fluid dynamics

Author

Listed:
  • Chen, Qin
  • Rosner, Fabian
  • Rao, Ashok
  • Samuelsen, Scott
  • Jayaraman, Ambal
  • Alptekin, Gokhan

Abstract

CO2 adsorption is one of the warm gas cleanup technologies under development for integrated gasification combined cycle (IGCC) applications. Computational Fluid Dynamics (CFD) can be a practical and powerful tool for reactor design for and optimization of the CO2 adsorption process. In this present work, CFD simulation was developed in commercially available ANSYS Fluent software and validated for solid sorbent CO2 capture to investigate pressure swing adsorption (PSA) for CO2 separation from syngas with all the auxiliary operating steps. The adsorption equilibrium and kinetics were incorporated into ANSYS by user defined functions (UDFs) for source terms in Navier–Stokes equations. The CFD model well predicted the CO2 breakthrough curve and temperature change. It was shown that in demo reactor operation, at the end of adsorption step, only half of the sorbent was loaded with CO2, while most of the loaded CO2 was released during the desorption step. Further optimization of sorbent packing and cycle operation can be done with assistance of this CFD model to maximize bed loading, and used to design the commercial size reactors.

Suggested Citation

  • Chen, Qin & Rosner, Fabian & Rao, Ashok & Samuelsen, Scott & Jayaraman, Ambal & Alptekin, Gokhan, 2019. "Simulation of elevated temperature solid sorbent CO2 capture for pre-combustion applications using computational fluid dynamics," Applied Energy, Elsevier, vol. 237(C), pages 314-325.
    • Handle: RePEc:eee:appene:v:237:y:2019:i:c:p:314-325
    DOI: 10.1016/j.apenergy.2019.01.042
    as

    Download full text from publisher

    File URL: http://www.sciencedirect.com/science/article/pii/S030626191930042X
    Download Restriction: Full text for ScienceDirect subscribers only
    File URL: https://libkey.io/10.1016/j.apenergy.2019.01.042?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    As the access to this document is restricted, you may want to search for a different version of it.

    References listed on IDEAS

    as
    1. Chen, Qin & Rao, Ashok & Samuelsen, Scott, 2015. "Coproduction of transportation fuels in advanced IGCCs via coal and biomass mixtures," Applied Energy, Elsevier, vol. 157(C), pages 851-860.
    2. Chen, Qin & Rao, Ashok & Samuelsen, Scott, 2014. "H2 coproduction in IGCC with CCS via coal and biomass mixture using advanced technologies," Applied Energy, Elsevier, vol. 118(C), pages 258-270.
    3. Hedin, Niklas & Andersson, Linnéa & Bergström, Lennart & Yan, Jinyue, 2013. "Adsorbents for the post-combustion capture of CO2 using rapid temperature swing or vacuum swing adsorption," Applied Energy, Elsevier, vol. 104(C), pages 418-433.
    Full references (including those not matched with items on IDEAS)

    Citations

    Citations are extracted by the CitEc Project, subscribe to its RSS feed for this item.
    as


    Cited by:

    1. Chi, Changyun & Li, Yingjie & Zhang, Wan & Wang, Zeyan, 2019. "Synthesis of a hollow microtubular Ca/Al sorbent with high CO2 uptake by hard templating," Applied Energy, Elsevier, vol. 251(C), pages 1-1.
    2. Zhao, Haitao & Ezeh, Collins I. & Ren, Weijia & Li, Wentao & Pang, Cheng Heng & Zheng, Chenghang & Gao, Xiang & Wu, Tao, 2019. "Integration of machine learning approaches for accelerated discovery of transition-metal dichalcogenides as Hg0 sensing materials," Applied Energy, Elsevier, vol. 254(C).
    3. Rosner, Fabian & Chen, Qin & Rao, Ashok & Samuelsen, Scott, 2020. "Thermo-economic analyses of isothermal water gas shift reactor integrations into IGCC power plant," Applied Energy, Elsevier, vol. 277(C).
    4. Rosner, Fabian & Chen, Qin & Rao, Ashok & Samuelsen, Scott & Jayaraman, Ambal & Alptekin, Gokhan, 2019. "Thermo-economic analyses of IGCC power plants employing warm gas CO2 separation technology," Energy, Elsevier, vol. 185(C), pages 541-553.
    5. Chen, Qin & Rosner, Fabian & Rao, Ashok & Samuelsen, Scott & Bonnema, Michael & Jayaraman, Ambal & Alptekin, Gokhan, 2020. "Simulation of elevated temperature combined water gas shift and solid sorbent CO2 capture for pre-combustion applications using computational fluid dynamics," Applied Energy, Elsevier, vol. 267(C).
    6. Yang, Shiliang & Zhou, Tao & Wei, Yonggang & Hu, Jianhang & Wang, Hua, 2020. "Dynamical and thermal property of rising bubbles in the bubbling fluidized biomass gasifier with wide particle size distribution," Applied Energy, Elsevier, vol. 259(C).
    7. Pashchenko, Dmitry, 2023. "Hydrogen-rich gas as a fuel for the gas turbines: A pathway to lower CO2 emission," Renewable and Sustainable Energy Reviews, Elsevier, vol. 173(C).
    8. Subraveti, Sai Gokul & Pai, Kasturi Nagesh & Rajagopalan, Ashwin Kumar & Wilkins, Nicholas Stiles & Rajendran, Arvind & Jayaraman, Ambalavan & Alptekin, Gokhan, 2019. "Cycle design and optimization of pressure swing adsorption cycles for pre-combustion CO2 capture," Applied Energy, Elsevier, vol. 254(C).

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Rosner, Fabian & Chen, Qin & Rao, Ashok & Samuelsen, Scott & Jayaraman, Ambal & Alptekin, Gokhan, 2019. "Thermo-economic analyses of IGCC power plants employing warm gas CO2 separation technology," Energy, Elsevier, vol. 185(C), pages 541-553.
    2. Chen, Qin & Rosner, Fabian & Rao, Ashok & Samuelsen, Scott & Bonnema, Michael & Jayaraman, Ambal & Alptekin, Gokhan, 2020. "Simulation of elevated temperature combined water gas shift and solid sorbent CO2 capture for pre-combustion applications using computational fluid dynamics," Applied Energy, Elsevier, vol. 267(C).
    3. Bassani, Andrea & Pirola, Carlo & Maggio, Enrico & Pettinau, Alberto & Frau, Caterina & Bozzano, Giulia & Pierucci, Sauro & Ranzi, Eliseo & Manenti, Flavio, 2016. "Acid Gas to Syngas (AG2S™) technology applied to solid fuel gasification: Cutting H2S and CO2 emissions by improving syngas production," Applied Energy, Elsevier, vol. 184(C), pages 1284-1291.
    4. Zhang, Minkai & Guo, Yincheng, 2013. "Rate based modeling of absorption and regeneration for CO2 capture by aqueous ammonia solution," Applied Energy, Elsevier, vol. 111(C), pages 142-152.
    5. Dang, Chengxiong & Xia, Huanhuan & Yuan, Shuting & Wei, Xingchuan & Cai, Weiquan, 2022. "Green hydrogen production from sorption-enhanced steam reforming of biogas over a Pd/Ni–CaO-mayenite multifunctional catalyst," Renewable Energy, Elsevier, vol. 201(P1), pages 314-322.
    6. Prabu, V., 2015. "Integration of in-situ CO2-oxy coal gasification with advanced power generating systems performing in a chemical looping approach of clean combustion," Applied Energy, Elsevier, vol. 140(C), pages 1-13.
    7. Zhang, Xiaowen & Zhang, Xin & Liu, Helei & Li, Wensheng & Xiao, Min & Gao, Hongxia & Liang, Zhiwu, 2017. "Reduction of energy requirement of CO2 desorption from a rich CO2-loaded MEA solution by using solid acid catalysts," Applied Energy, Elsevier, vol. 202(C), pages 673-684.
    8. Choi, Munkyoung & Cho, Minki & Lee, J.W., 2016. "Empirical formula for the mass flux in chemical absorption of CO2 with ammonia droplets," Applied Energy, Elsevier, vol. 164(C), pages 1-9.
    9. Qin, Shiyue & Chang, Shiyan & Yao, Qiang, 2018. "Modeling, thermodynamic and techno-economic analysis of coal-to-liquids process with different entrained flow coal gasifiers," Applied Energy, Elsevier, vol. 229(C), pages 413-432.
    10. Wei, Ning & Li, Xiaochun & Wang, Yan & Zhu, Qianlin & Liu, Shengnan & Liu, Naizhong & Su, Xuebing, 2015. "Geochemical impact of aquifer storage for impure CO2 containing O2 and N2: Tongliao field experiment," Applied Energy, Elsevier, vol. 145(C), pages 198-210.
    11. Wang, Weilong & Li, Jiang & Wei, Xiaolan & Ding, Jing & Feng, Haijun & Yan, Jinyue & Yang, Jianping, 2015. "Carbon dioxide adsorption thermodynamics and mechanisms on MCM-41 supported polyethylenimine prepared by wet impregnation method," Applied Energy, Elsevier, vol. 142(C), pages 221-228.
    12. Alexander García-Mariaca & Eva Llera-Sastresa, 2021. "Review on Carbon Capture in ICE Driven Transport," Energies, MDPI, vol. 14(21), pages 1-30, October.
    13. Zhu, Xuancan & Shi, Yixiang & Cai, Ningsheng, 2016. "Integrated gasification combined cycle with carbon dioxide capture by elevated temperature pressure swing adsorption," Applied Energy, Elsevier, vol. 176(C), pages 196-208.
    14. Huang, Yu-Fong & Cheng, Pei-Hsin & Chiueh, Pei-Te & Lo, Shang-Lien, 2017. "Leucaena biochar produced by microwave torrefaction: Fuel properties and energy efficiency," Applied Energy, Elsevier, vol. 204(C), pages 1018-1025.
    15. Taufiq, Bin Nur & Kikuchi, Yasunori & Ishimoto, Takayoshi & Honda, Kuniaki & Koyama, Michihisa, 2015. "Conceptual design of light integrated gasification fuel cell based on thermodynamic process simulation," Applied Energy, Elsevier, vol. 147(C), pages 486-499.
    16. Li, Shuangjun & Yuan, Xiangzhou & Deng, Shuai & Zhao, Li & Lee, Ki Bong, 2021. "A review on biomass-derived CO2 adsorption capture: Adsorbent, adsorber, adsorption, and advice," Renewable and Sustainable Energy Reviews, Elsevier, vol. 152(C).
    17. van der Spek, Mijndert & Ramirez, Andrea & Faaij, André, 2017. "Challenges and uncertainties of ex ante techno-economic analysis of low TRL CO2 capture technology: Lessons from a case study of an NGCC with exhaust gas recycle and electric swing adsorption," Applied Energy, Elsevier, vol. 208(C), pages 920-934.
    18. Bartela, Łukasz & Skorek-Osikowska, Anna & Kotowicz, Janusz, 2015. "An analysis of the investment risk related to the integration of a supercritical coal-fired combined heat and power plant with an absorption installation for CO2 separation," Applied Energy, Elsevier, vol. 156(C), pages 423-435.
    19. Kong, Yong & Shen, Xiaodong & Cui, Sheng & Fan, Maohong, 2015. "Development of monolithic adsorbent via polymeric sol–gel process for low-concentration CO2 capture," Applied Energy, Elsevier, vol. 147(C), pages 308-317.
    20. Liu, Xuetao & Saren, Sagar & Chen, Haonan & Jeong, Ji Hwan & Li, Minxia & Dang, Chaobin & Miyazaki, Takahiko & Thu, Kyaw, 2024. "Open adsorption system for atmospheric CO2 capture: Scaling and sensitivity analysis," Energy, Elsevier, vol. 294(C).

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:eee:appene:v:237:y:2019:i:c:p:314-325. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Catherine Liu (email available below). General contact details of provider: http://www.elsevier.com/wps/find/journaldescription.cws_home/405891/description#description .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.