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Investigation on model compound of biomass gasification tar cracking in microwave furnace: Comparative research

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  • Chen, Guanyi
  • Li, Jian
  • Cheng, Zhanjun
  • Yan, Beibei
  • Ma, Wenchao
  • Yao, Jingang

Abstract

Tar is a major concern for advancing biomass gasification in industrial application due to its risk to downstream pipes/equipment and tar-contaminated environmental issue. Meanwhile, tar also leads to energy loss. Thermal cracking with or without catalyst is a widely used method for removing tar during biomass gasification. Microwave thermal cracking is a lately developed method of removing tar and only a few literatures are available on its reaction parameters and catalytic effect. A microwave tube furnace was designed for investigating tar cracking in our lab. Toluene as biomass tar model compound was cracked under various operating conditions assisted by three different bed materials (SiC, biochar, and biochar-Ni). The results showed that microwave heating is effective for toluene cracking, and biochar can act as a bi-functional catalyst for toluene cracking. Toluene cracking rate reached 95.12% under reaction temperature of 800 °C, catalyst particle size of 40–60 meshes and Ni loading of 4 wt%. Hydrogen concentration was higher than 92 vol%. The mechanism of toluene cracking, effect of microwave and efficiency of energy conversion were also carefully discussed, and the applied potential of microwave tar cracking technology was proved.

Suggested Citation

  • Chen, Guanyi & Li, Jian & Cheng, Zhanjun & Yan, Beibei & Ma, Wenchao & Yao, Jingang, 2018. "Investigation on model compound of biomass gasification tar cracking in microwave furnace: Comparative research," Applied Energy, Elsevier, vol. 217(C), pages 249-257.
    • Handle: RePEc:eee:appene:v:217:y:2018:i:c:p:249-257
    DOI: 10.1016/j.apenergy.2018.02.028
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    References listed on IDEAS

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    Cited by:

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    4. Li, Jian & Tao, Junyu & Yan, Beibei & Cheng, Kexin & Chen, Guanyi & Hu, Jianli, 2020. "Microwave reforming with char-supported Nickel-Cerium catalysts: A potential approach for thorough conversion of biomass tar model compound," Applied Energy, Elsevier, vol. 261(C).
    5. Cheng Yang & Kanfeng Ying & Fan Yang & Huanghu Peng & Zezhou Chen, 2022. "Simulation on the Electric and Thermal Fields of a Microwave Reactor for Ex Situ Biomass Tar Elimination," Energies, MDPI, vol. 15(11), pages 1-12, June.
    6. Li, Jian & Tao, Junyu & Yan, Beibei & Jiao, Liguo & Chen, Guanyi & Hu, Jianli, 2021. "Review of microwave-based treatments of biomass gasification tar," Renewable and Sustainable Energy Reviews, Elsevier, vol. 150(C).
    7. Li, Longzhi & Meng, Bo & Qin, Xiaomin & Yang, Zhijuan & Chen, Jian & Yan, Keshuo & Wang, Fumao, 2020. "Toluene microwave cracking and reforming over bio-char with in-situ activation and ex-situ impregnation of metal," Renewable Energy, Elsevier, vol. 149(C), pages 1205-1213.
    8. Li, Jian & Jiao, Liguo & Tao, Junyu & Chen, Guanyi & Hu, Jianli & Yan, Beibei & Mansour, Mohy & Guo, Yaoyu & Ye, Peiwen & Ding, Zheng & Yu, Tianxiao, 2020. "Can microwave treat biomass tar? A comprehensive study based on experimental and net energy analysis," Applied Energy, Elsevier, vol. 272(C).
    9. Li, Longzhi & Yang, Zhijuan & Qin, Xiaomin & Chen, Jian & Yan, Keshuo & Zou, Guifu & Peng, Zhuoyan & Wang, Fumao & Song, Zhanlong & Ma, Chunyuan, 2019. "Toluene microwave-assisted reforming with CO2 or a mixed agent of CO2-H2O on Fe-doped activated biochar," Energy, Elsevier, vol. 177(C), pages 358-366.
    10. Zhang, Xiaosong & Pan, Jiawei & Wang, Liang & Qian, Tianle & Zhu, Yuezhao & Sun, Hongqi & Gao, Jian & Chen, Haijun & Gao, Ying & Liu, Chang, 2019. "COSMO-based solvent selection and Aspen Plus process simulation for tar absorptive removal," Applied Energy, Elsevier, vol. 251(C), pages 1-1.
    11. Fan, Liangliang & Liu, Lei & Xiao, Zhiguo & Su, Zheyang & Huang, Pei & Peng, Hongyu & Lv, Sen & Jiang, Haiwei & Ruan, Roger & Chen, Paul & Zhou, Wenguang, 2021. "Comparative study of continuous-stirred and batch microwave pyrolysis of linear low-density polyethylene in the presence/absence of HZSM-5," Energy, Elsevier, vol. 228(C).
    12. Tian, Beile & Mao, Songbo & Guo, Feiqiang & Bai, Jiaming & Shu, Rui & Qian, Lin & Liu, Qi, 2022. "Monolithic biochar-supported cobalt-based catalysts with high-activity and superior-stability for biomass tar reforming," Energy, Elsevier, vol. 242(C).

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