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A high-performance carbon nanoparticle-decorated graphite felt electrode for vanadium redox flow batteries

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  • Wei, L.
  • Zhao, T.S.
  • Zhao, G.
  • An, L.
  • Zeng, L.

Abstract

Increasing the performance of vanadium redox flow batteries (VRFBs), especially the energy efficiency and power density, is critically important to reduce the system cost to a level for widespread commercialization. Unlike conventional VRFBs with flow-through structure, in this work we create a VRFB featuring a flow-field structure with a carbon nanoparticle-decorated graphite felt electrode for the battery. This novel structure, exhibiting a significantly reduced ohmic loss through reducing electrode thickness, an increased surface area and improved electrocatalytic activity by coating carbon nanoparticles, allows the energy efficiency up to 84.8% at a current density of as high as 100mAcm−2 and the peak power density to reach a value of 508mWcm−2. In addition, it is demonstrated that the battery with this proposed structure exhibits a substantially improved rate capability and capacity retention as opposed to conventional flow-through structured battery with thick graphite felt electrodes.

Suggested Citation

  • Wei, L. & Zhao, T.S. & Zhao, G. & An, L. & Zeng, L., 2016. "A high-performance carbon nanoparticle-decorated graphite felt electrode for vanadium redox flow batteries," Applied Energy, Elsevier, vol. 176(C), pages 74-79.
    • Handle: RePEc:eee:appene:v:176:y:2016:i:c:p:74-79
    DOI: 10.1016/j.apenergy.2016.05.048
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    References listed on IDEAS

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    Cited by:

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    2. Sun, J. & Jiang, H.R. & Zhang, B.W. & Chao, C.Y.H. & Zhao, T.S., 2020. "Towards uniform distributions of reactants via the aligned electrode design for vanadium redox flow batteries," Applied Energy, Elsevier, vol. 259(C).
    3. Wei, L. & Zeng, L. & Wu, M.C. & Fan, X.Z. & Zhao, T.S., 2019. "Seawater as an alternative to deionized water for electrolyte preparations in vanadium redox flow batteries," Applied Energy, Elsevier, vol. 251(C), pages 1-1.
    4. Bates, Alex M. & Paxton, William F. & Spurgeon, Joshua M. & Park, Sam D. & Sunkara, Mahendra K., 2021. "Earth-abundant redox couples using durable boron doped diamond electrodes: Beyond vanadium redox couples," Applied Energy, Elsevier, vol. 282(PB).
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    6. Kim, Jungmyung & Park, Heesung, 2018. "Impact of nanofluidic electrolyte on the energy storage capacity in vanadium redox flow battery," Energy, Elsevier, vol. 160(C), pages 192-199.
    7. Zeng, Y.K. & Zhao, T.S. & Zhou, X.L. & Zeng, L. & Wei, L., 2016. "The effects of design parameters on the charge-discharge performance of iron-chromium redox flow batteries," Applied Energy, Elsevier, vol. 182(C), pages 204-209.
    8. Mehboob, Sheeraz & Ali, Ghulam & Shin, Hyun-Jin & Hwang, Jinyeon & Abbas, Saleem & Chung, Kyung Yoon & Ha, Heung Yong, 2018. "Enhancing the performance of all-vanadium redox flow batteries by decorating carbon felt electrodes with SnO2 nanoparticles," Applied Energy, Elsevier, vol. 229(C), pages 910-921.
    9. Ren, Y.X. & Zhao, T.S. & Tan, P. & Wei, Z.H. & Zhou, X.L., 2017. "Modeling of an aprotic Li-O2 battery incorporating multiple-step reactions," Applied Energy, Elsevier, vol. 187(C), pages 706-716.
    10. Kim, Jungmyung & Park, Heesung, 2017. "Experimental analysis of discharge characteristics in vanadium redox flow battery," Applied Energy, Elsevier, vol. 206(C), pages 451-457.
    11. Wei, L. & Zhao, T.S. & Zeng, L. & Zhou, X.L. & Zeng, Y.K., 2016. "Copper nanoparticle-deposited graphite felt electrodes for all vanadium redox flow batteries," Applied Energy, Elsevier, vol. 180(C), pages 386-391.
    12. Zhou, X.L. & Zhao, T.S. & An, L. & Zeng, Y.K. & Zhu, X.B., 2016. "Performance of a vanadium redox flow battery with a VANADion membrane," Applied Energy, Elsevier, vol. 180(C), pages 353-359.

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