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Development of sodium/lithium/fly ash sorbents for high temperature post-combustion CO2 capture

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  • Sanna, Aimaro
  • Ramli, Ili
  • Mercedes Maroto-Valer, M.

Abstract

CO2 capture from combustion processes faces several challenges including high energy penalty, low CO2 partial pressure, high flow rates and presence of water vapours. Absorption of CO2 at high temperature is recently attracting increasingly attention. Alkali metal based sorbents present clear advantages compared to other high temperature sorbents, such as high CO2 capture capacity, lower regeneration temperatures (<750°C) and excellent stability. In this work, Na/Li-silicates prepared by mixing Na/Li carbonates with fly ash (FA) in various molar ratios were evaluated for their capacity to chemisorb CO2 at 500–700°C and in presence of H2O (2–12vol%), diluted CO2 (14vol%) and CO2 sorption promoters.

Suggested Citation

  • Sanna, Aimaro & Ramli, Ili & Mercedes Maroto-Valer, M., 2015. "Development of sodium/lithium/fly ash sorbents for high temperature post-combustion CO2 capture," Applied Energy, Elsevier, vol. 156(C), pages 197-206.
    • Handle: RePEc:eee:appene:v:156:y:2015:i:c:p:197-206
    DOI: 10.1016/j.apenergy.2015.07.008
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    References listed on IDEAS

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    Cited by:

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    3. Craig, Christopher A., 2016. "Energy consumption, energy efficiency, and consumer perceptions: A case study for the Southeast United States," Applied Energy, Elsevier, vol. 165(C), pages 660-669.
    4. Wang, Ke & Zhou, Zhongyun & Zhao, Pengfei & Yin, Zeguang & Su, Zhen & Sun, Ji, 2016. "Synthesis of a highly efficient Li4SiO4 ceramic modified with a gluconic acid-based carbon coating for high-temperature CO2 capture," Applied Energy, Elsevier, vol. 183(C), pages 1418-1427.
    5. Theo, Wai Lip & Lim, Jeng Shiun & Hashim, Haslenda & Mustaffa, Azizul Azri & Ho, Wai Shin, 2016. "Review of pre-combustion capture and ionic liquid in carbon capture and storage," Applied Energy, Elsevier, vol. 183(C), pages 1633-1663.
    6. Wang, Ke & Zhou, Zhongyun & Zhao, Pengfei & Yin, Zeguang & Su, Zhen & Sun, Ji, 2017. "Molten sodium-fluoride-promoted high-performance Li4SiO4-based CO2 sorbents at low CO2 concentrations," Applied Energy, Elsevier, vol. 204(C), pages 403-412.
    7. Li, Xiangyu & Wang, Zhiqing & Feng, Ru & Huang, Jiejie & Fang, Yitian, 2021. "CO2 capture on aminosilane functionalized alumina-extracted residue of catalytic gasification coal ash," Energy, Elsevier, vol. 221(C).
    8. Craig, Christopher A. & Feng, Song, 2016. "An examination of electricity generation by utility organizations in the Southeast United States," Energy, Elsevier, vol. 116(P1), pages 601-608.
    9. Al-Kalbani, Haitham & Xuan, Jin & García, Susana & Wang, Huizhi, 2016. "Comparative energetic assessment of methanol production from CO2: Chemical versus electrochemical process," Applied Energy, Elsevier, vol. 165(C), pages 1-13.

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    Keywords

    Absorption; Fly ash; CO2 sorbents; Alkali metal silicates;
    All these keywords.

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