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CO2 absorption/regeneration enhancement in DI water with suspended nanoparticles for energy conversion application

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  • Lee, Jong Sung
  • Lee, Jae Won
  • Kang, Yong Tae

Abstract

The integrated gasification combined cycle (IGCC) is getting much more attention due to the rich reserves of coal around the world. In general, the absorption rate of a physical method such as the IGCC system is weaker than that of a chemical method, but it needs much less energy during the regeneration process. In this study, the main objective is to estimate the performance enhancement for CO2 gas absorption and regeneration by using SiO2/DI water and Al2O3/DI water nanofluids. The key parameters are the concentrations of SiO2 and Al2O3 nanoparticles and the system pressure during the regeneration process. It is found that the maximum CO2 absorption and regeneration performance enhancements are 23.5% and 11.8% at 0.01vol% of SiO2 nanoparticles, respectively. However, in the case of Al2O3 nanoparticles, the CO2 absorption performance increases 23.5% at 0.01vol%, but the regeneration performance decreases 11.2% at 0.01vol%, respectively. The enhancement mechanisms for CO2 absorption and regeneration by nanoparticles are summarized and proposed in this study.

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  • Lee, Jong Sung & Lee, Jae Won & Kang, Yong Tae, 2015. "CO2 absorption/regeneration enhancement in DI water with suspended nanoparticles for energy conversion application," Applied Energy, Elsevier, vol. 143(C), pages 119-129.
    • Handle: RePEc:eee:appene:v:143:y:2015:i:c:p:119-129
    DOI: 10.1016/j.apenergy.2015.01.020
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    1. Amaris, Carlos & Bourouis, Mahmoud & Vallès, Manel, 2014. "Passive intensification of the ammonia absorption process with NH3/LiNO3 using carbon nanotubes and advanced surfaces in a tubular bubble absorber," Energy, Elsevier, vol. 68(C), pages 519-528.
    2. Sundar, L. Syam & Sharma, K.V. & Naik, M.T. & Singh, Manoj K., 2013. "Empirical and theoretical correlations on viscosity of nanofluids: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 25(C), pages 670-686.
    3. Lee, Jae Won & Kang, Yong Tae, 2013. "CO2 absorption enhancement by Al2O3 nanoparticles in NaCl aqueous solution," Energy, Elsevier, vol. 53(C), pages 206-211.
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    1. Zhang, Xiaowen & Liu, Helei & Liang, Zhiwu & Idem, Raphael & Tontiwachwuthikul, Paitoon & Jaber Al-Marri, Mohammed & Benamor, Abdelbaki, 2018. "Reducing energy consumption of CO2 desorption in CO2-loaded aqueous amine solution using Al2O3/HZSM-5 bifunctional catalysts," Applied Energy, Elsevier, vol. 229(C), pages 562-576.
    2. Zarei, Fariba & Bagherzadeh Jahromi, Farideh & Elhambakhsh, Abbas & Keshavarz, Peyman, 2023. "Enhanced CO2 absorption and reduced regeneration energy consumption using modified magnetic NPs," Energy, Elsevier, vol. 278(C).
    3. Liu, Changhui & Qiao, Yu & Du, Peixing & Zhang, Jiahao & Zhao, Jiateng & Liu, Chenzhen & Huo, Yutao & Qi, Cong & Rao, Zhonghao & Yan, Yuying, 2021. "Recent advances of nanofluids in micro/nano scale energy transportation," Renewable and Sustainable Energy Reviews, Elsevier, vol. 149(C).
    4. Zhang, Xiaowen & Zhang, Rui & Liu, Helei & Gao, Hongxia & Liang, Zhiwu, 2018. "Evaluating CO2 desorption performance in CO2-loaded aqueous tri-solvent blend amines with and without solid acid catalysts," Applied Energy, Elsevier, vol. 218(C), pages 417-429.
    5. Zhang, Xiaowen & Zhang, Xin & Liu, Helei & Li, Wensheng & Xiao, Min & Gao, Hongxia & Liang, Zhiwu, 2017. "Reduction of energy requirement of CO2 desorption from a rich CO2-loaded MEA solution by using solid acid catalysts," Applied Energy, Elsevier, vol. 202(C), pages 673-684.
    6. Siti Aishah Mohd Rozaiddin & Kok Keong Lau, 2022. "A Review on Enhancing Solvent Regeneration in CO 2 Absorption Process Using Nanoparticles," Sustainability, MDPI, vol. 14(8), pages 1-33, April.
    7. Chen, Yifeng & Song, Shuailong & Li, Ning & Wu, Jian & Lu, Xiaohua & Ji, Xiaoyan, 2022. "Developing hybrid 1-hexyl-3-methylimidazolium bis(trifluoromethylsulfonyl)imide/titanium dioxide/water absorbent for CO2 separation," Applied Energy, Elsevier, vol. 326(C).
    8. Ali Saleh Bairq, Zain & Gao, Hongxia & Huang, Yufei & Zhang, Haiyan & Liang, Zhiwu, 2019. "Enhancing CO2 desorption performance in rich MEA solution by addition of SO42−/ZrO2/SiO2 bifunctional catalyst," Applied Energy, Elsevier, vol. 252(C), pages 1-1.
    9. Lee, Jae Won & Kim, Seonggon & Torres Pineda, Israel & Kang, Yong Tae, 2021. "Review of nanoabsorbents for capture enhancement of CO2 and its industrial applications with design criteria," Renewable and Sustainable Energy Reviews, Elsevier, vol. 138(C).
    10. Zhang, Zhien & Cai, Jianchao & Chen, Feng & Li, Hao & Zhang, Wenxiang & Qi, Wenjie, 2018. "Progress in enhancement of CO2 absorption by nanofluids: A mini review of mechanisms and current status," Renewable Energy, Elsevier, vol. 118(C), pages 527-535.
    11. Arshadi, M. & Taghvaei, H. & Abdolmaleki, M.K. & Lee, M. & Eskandarloo, H. & Abbaspourrad, A., 2019. "Carbon dioxide absorption in water/nanofluid by a symmetric amine-based nanodendritic adsorbent," Applied Energy, Elsevier, vol. 242(C), pages 1562-1572.
    12. Lee, Jae Won & Torres Pineda, Israel & Lee, Jung Hun & Kang, Yong Tae, 2016. "Combined CO2 absorption/regeneration performance enhancement by using nanoabsorbents," Applied Energy, Elsevier, vol. 178(C), pages 164-176.

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    Keywords

    Absorption; Al2O3; CO2; Nanoparticle; Regeneration; SiO2;
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