IDEAS home Printed from https://ideas.repec.org/a/nat/natcom/v13y2022i1d10.1038_s41467-022-32699-x.html
   My bibliography  Save this article

Flexible iontronics based on 2D nanofluidic material

Author

Listed:
  • Di Wei

    (Chinese Academy of Sciences)

  • Feiyao Yang

    (Chinese Academy of Sciences)

  • Zhuoheng Jiang

    (Chinese Academy of Sciences)

  • Zhonglin Wang

    (Chinese Academy of Sciences
    Georgia Institute of Technology)

Abstract

Iontronics focuses on the interactions between electrons and ions, playing essential roles in most processes across physics, chemistry and life science. Osmotic power source as an example of iontronics, could transform ion gradient into electrical energy, however, it generates low power, sensitive to humidity and can’t operate under freezing point. Herein, based on 2D nanofluidic graphene oxide material, we demonstrate an ultrathin (∼10 µm) osmotic power source with voltage of 1.5 V, volumetric specific energy density of 6 mWh cm−3 and power density of 28 mW cm−3, achieving the highest values so far. Coupled with triboelectric nanogenerator, it could form a self-charged conformable triboiontronic device. Furthermore, the 3D aerogel scales up areal power density up to 1.3 mW cm−2 purely from ion gradient based on nanoconfined enhancement from graphene oxide that can operate under −40 °C and overcome humidity limitations, enabling to power the future implantable electronics in human-machine interface.

Suggested Citation

  • Di Wei & Feiyao Yang & Zhuoheng Jiang & Zhonglin Wang, 2022. "Flexible iontronics based on 2D nanofluidic material," Nature Communications, Nature, vol. 13(1), pages 1-11, December.
  • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-32699-x
    DOI: 10.1038/s41467-022-32699-x
    as

    Download full text from publisher

    File URL: https://www.nature.com/articles/s41467-022-32699-x
    File Function: Abstract
    Download Restriction: no

    File URL: https://libkey.io/10.1038/s41467-022-32699-x?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    References listed on IDEAS

    as
    1. Jiandong Feng & Michael Graf & Ke Liu & Dmitry Ovchinnikov & Dumitru Dumcenco & Mohammad Heiranian & Vishal Nandigana & Narayana R. Aluru & Andras Kis & Aleksandra Radenovic, 2016. "Single-layer MoS2 nanopores as nanopower generators," Nature, Nature, vol. 536(7615), pages 197-200, August.
    2. Yaxin Huang & Huhu Cheng & Ce Yang & Panpan Zhang & Qihua Liao & Houze Yao & Gaoquan Shi & Liangti Qu, 2018. "Interface-mediated hygroelectric generator with an output voltage approaching 1.5 volts," Nature Communications, Nature, vol. 9(1), pages 1-8, December.
    3. Weiwen Xin & Zhen Zhang & Xiaodong Huang & Yuhao Hu & Teng Zhou & Congcong Zhu & Xiang-Yu Kong & Lei Jiang & Liping Wen, 2019. "High-performance silk-based hybrid membranes employed for osmotic energy conversion," Nature Communications, Nature, vol. 10(1), pages 1-10, December.
    4. Ryan C. Rollings & Aaron T. Kuan & Jene A. Golovchenko, 2016. "Ion selectivity of graphene nanopores," Nature Communications, Nature, vol. 7(1), pages 1-7, September.
    5. Alessandro Siria & Philippe Poncharal & Anne-Laure Biance & Rémy Fulcrand & Xavier Blase & Stephen T. Purcell & Lydéric Bocquet, 2013. "Giant osmotic energy conversion measured in a single transmembrane boron nitride nanotube," Nature, Nature, vol. 494(7438), pages 455-458, February.
    6. Dmitriy A. Dikin & Sasha Stankovich & Eric J. Zimney & Richard D. Piner & Geoffrey H. B. Dommett & Guennadi Evmenenko & SonBinh T. Nguyen & Rodney S. Ruoff, 2007. "Preparation and characterization of graphene oxide paper," Nature, Nature, vol. 448(7152), pages 457-460, July.
    7. Mengchen Zhang & Kecheng Guan & Yufan Ji & Gongping Liu & Wanqin Jin & Nanping Xu, 2019. "Controllable ion transport by surface-charged graphene oxide membrane," Nature Communications, Nature, vol. 10(1), pages 1-8, December.
    8. Zhong–Shuai Wu & Khaled Parvez & Xinliang Feng & Klaus Müllen, 2013. "Graphene-based in-plane micro-supercapacitors with high power and energy densities," Nature Communications, Nature, vol. 4(1), pages 1-8, December.
    Full references (including those not matched with items on IDEAS)

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Mai, Van-Phung & Yang, Ruey-Jen, 2020. "Boosting power generation from salinity gradient on high-density nanoporous membrane using thermal effect," Applied Energy, Elsevier, vol. 274(C).
    2. Ce Yang & Haiyan Wang & Jiaxin Bai & Tiancheng He & Huhu Cheng & Tianlei Guang & Houze Yao & Liangti Qu, 2022. "Transfer learning enhanced water-enabled electricity generation in highly oriented graphene oxide nanochannels," Nature Communications, Nature, vol. 13(1), pages 1-12, December.
    3. Ren, Qinlong & Zhu, Huangyi & Chen, Kelei & Zhang, J.F. & Qu, Z.G., 2022. "Similarity principle based multi-physical parameter unification and comparison in salinity-gradient osmotic energy conversion," Applied Energy, Elsevier, vol. 307(C).
    4. Weipeng Xian & Xiuhui Zuo & Changjia Zhu & Qing Guo & Qing-Wei Meng & Xincheng Zhu & Sai Wang & Shengqian Ma & Qi Sun, 2022. "Anomalous thermo-osmotic conversion performance of ionic covalent-organic-framework membranes in response to charge variations," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    5. Rezakazemi, Mashallah & Arabi Shamsabadi, Ahmad & Lin, Haiqing & Luis, Patricia & Ramakrishna, Seeram & Aminabhavi, Tejraj M., 2021. "Sustainable MXenes-based membranes for highly energy-efficient separations," Renewable and Sustainable Energy Reviews, Elsevier, vol. 143(C).
    6. Zhang, X.F. & Zhang, X. & Qu, Z.G. & Pu, J.Q. & Wang, Q., 2022. "Thermal-enhanced nanofluidic osmotic energy conversion with the interfacial photothermal method," Applied Energy, Elsevier, vol. 326(C).
    7. Nawapong Unsuree & Sorasak Phanphak & Pongthep Prajongtat & Aritsa Bunpheng & Kulpavee Jitapunkul & Pornpis Kongputhon & Pannaree Srinoi & Pawin Iamprasertkun & Wisit Hirunpinyopas, 2021. "A Review: Ion Transport of Two-Dimensional Materials in Novel Technologies from Macro to Nanoscopic Perspectives," Energies, MDPI, vol. 14(18), pages 1-38, September.
    8. Chen, Xi & Wang, Lu & Zhou, Ruhong & Long, Rui & Liu, Zhichun & Liu, Wei, 2023. "pH-depended behaviors of electrolytes in nanofluidic salinity gradient energy harvesting," Renewable Energy, Elsevier, vol. 211(C), pages 31-41.
    9. Zhen Zhang & Preeti Bhauriyal & Hafeesudeen Sahabudeen & Zhiyong Wang & Xiaohui Liu & Mike Hambsch & Stefan C. B. Mannsfeld & Renhao Dong & Thomas Heine & Xinliang Feng, 2022. "Cation-selective two-dimensional polyimine membranes for high-performance osmotic energy conversion," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    10. Kecheng Guan & Yanan Guo & Zhan Li & Yuandong Jia & Qin Shen & Keizo Nakagawa & Tomohisa Yoshioka & Gongping Liu & Wanqin Jin & Hideto Matsuyama, 2023. "Deformation constraints of graphene oxide nanochannels under reverse osmosis," Nature Communications, Nature, vol. 14(1), pages 1-12, December.
    11. Wang, Y. & Wang, H. & Wan, C.Q., 2018. "The effect of colloids on nanofluidic power generation," Energy, Elsevier, vol. 160(C), pages 863-867.
    12. Song, Dongxing & Li, Lu & Huang, Ce & Wang, Ke, 2023. "Synergy between ionic thermoelectric conversion and nanofluidic reverse electrodialysis for high power density generation," Applied Energy, Elsevier, vol. 334(C).
    13. Chen, Xi & Luo, Zuoqing & Long, Rui & Liu, Zhichun & Liu, Wei, 2022. "Impacts of transmembrane pH gradient on nanofluidic salinity gradient energy conversion," Renewable Energy, Elsevier, vol. 187(C), pages 440-449.
    14. Shihao Su & Yifan Zhang & Shengyuan Peng & Linxin Guo & Yong Liu & Engang Fu & Huijun Yao & Jinlong Du & Guanghua Du & Jianming Xue, 2022. "Multifunctional graphene heterogeneous nanochannel with voltage-tunable ion selectivity," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    15. Li, Yong & Song, Jian & Yang, Jie, 2015. "Graphene models and nano-scale characterization technologies for fuel cell vehicle electrodes," Renewable and Sustainable Energy Reviews, Elsevier, vol. 42(C), pages 66-77.
    16. Park, Seung-Keun & Seong, Chae-Yong & Yoo, Suyeon & Piao, Yuanzhe, 2016. "Porous Mn3O4 nanorod/reduced graphene oxide hybrid paper as a flexible and binder-free anode material for lithium ion battery," Energy, Elsevier, vol. 99(C), pages 266-273.
    17. Jin Wang & Zheng Cui & Shangzhen Li & Zeyuan Song & Miaolu He & Danxi Huang & Yuan Feng & YanZheng Liu & Ke Zhou & Xudong Wang & Lei Wang, 2024. "Unlocking osmotic energy harvesting potential in challenging real-world hypersaline environments through vermiculite-based hetero-nanochannels," Nature Communications, Nature, vol. 15(1), pages 1-12, December.
    18. Dasari, Bhagya Lakshmi & Nouri, Jamshid M. & Brabazon, Dermot & Naher, Sumsun, 2017. "Graphene and derivatives – Synthesis techniques, properties and their energy applications," Energy, Elsevier, vol. 140(P1), pages 766-778.
    19. Kuichang Zuo & Xiang Zhang & Xiaochuan Huang & Eliezer F. Oliveira & Hua Guo & Tianshu Zhai & Weipeng Wang & Pedro J. J. Alvarez & Menachem Elimelech & Pulickel M. Ajayan & Jun Lou & Qilin Li, 2022. "Ultrahigh resistance of hexagonal boron nitride to mineral scale formation," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    20. Jiayue Tang & Yuanyuan Zhao & Mi Wang & Dianyu Wang & Xuan Yang & Ruiran Hao & Mingzhan Wang & Yanlei Wang & Hongyan He & John H. Xin & Shuang Zheng, 2022. "Circadian humidity fluctuation induced capillary flow for sustainable mobile energy," Nature Communications, Nature, vol. 13(1), pages 1-9, December.

    More about this item

    Statistics

    Access and download statistics

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-32699-x. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Sonal Shukla or Springer Nature Abstracting and Indexing (email available below). General contact details of provider: http://www.nature.com .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.