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CO2 Fixation by Membrane Separated NaCl Electrolysis

Author

Listed:
  • Hyun Sic Park

    (Department of Chemical and Biomolecular Engineering, Yonsei University, 262 Seongsanno, Seodaemun-gu, Seoul 120-749, Korea)

  • Ju Sung Lee

    (Department of Chemical and Biomolecular Engineering, Yonsei University, 262 Seongsanno, Seodaemun-gu, Seoul 120-749, Korea)

  • JunYoung Han

    (Proton Conductors Section, Department of Energy Conversion and Storage, Technical University of Denmark, Kemitorvet 207, Kgs. Lyngby DK-2800, Denmark)

  • Sangwon Park

    (CO2 Sequestration Department, Korea Institute of Geoscience and Mineral Resources (KIGAM), 124 Gwahak-ro, Yuseong-gu, Daejeon 305-350, Korea)

  • Jinwon Park

    (Department of Chemical and Biomolecular Engineering, Yonsei University, 262 Seongsanno, Seodaemun-gu, Seoul 120-749, Korea)

  • Byoung Ryul Min

    (Department of Chemical and Biomolecular Engineering, Yonsei University, 262 Seongsanno, Seodaemun-gu, Seoul 120-749, Korea)

Abstract

Atmospheric concentrations of carbon dioxide (CO2), a major cause of global warming, have been rising due to industrial development. Carbon capture and storage (CCS), which is regarded as the most effective way to reduce such atmospheric CO2 concentrations, has several environmental and technical disadvantages. Carbon capture and utilization (CCU), which has been introduced to cover such disadvantages, makes it possible to capture CO2, recycling byproducts as resources. However, CCU also requires large amounts of energy in order to induce reactions. Among existing CCU technologies, the process for converting CO2 into CaCO3 requires high temperature and high pressure as reaction conditions. This study proposes a method to fixate CaCO3 stably by using relatively less energy than existing methods. After forming NaOH absorbent solution through electrolysis of NaCl in seawater, CaCO3 was precipitated at room temperature and pressure. Following the experiment, the resulting product CaCO3 was analyzed with Fourier transform infrared spectroscopy (FT-IR); field emission scanning electron microscopy (FE-SEM) image and X-ray diffraction (XRD) patterns were also analyzed. The results showed that the CaCO3 crystal product was high-purity calcite. The study shows a successful method for fixating CO2 by reducing carbon dioxide released into the atmosphere while forming high-purity CaCO3.

Suggested Citation

  • Hyun Sic Park & Ju Sung Lee & JunYoung Han & Sangwon Park & Jinwon Park & Byoung Ryul Min, 2015. "CO2 Fixation by Membrane Separated NaCl Electrolysis," Energies, MDPI, vol. 8(8), pages 1-12, August.
    • Handle: RePEc:gam:jeners:v:8:y:2015:i:8:p:8704-8715:d:54222
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    References listed on IDEAS

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    1. Siefert, Nicholas S. & Litster, Shawn, 2013. "Exergy and economic analyses of advanced IGCC–CCS and IGFC–CCS power plants," Applied Energy, Elsevier, vol. 107(C), pages 315-328.
    2. Holloway, S., 2005. "Underground sequestration of carbon dioxide—a viable greenhouse gas mitigation option," Energy, Elsevier, vol. 30(11), pages 2318-2333.
    3. Fagerlund, Johan & Nduagu, Experience & Romão, Inês & Zevenhoven, Ron, 2012. "CO2 fixation using magnesium silicate minerals part 1: Process description and performance," Energy, Elsevier, vol. 41(1), pages 184-191.
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    Cited by:

    1. José Luis Míguez & Jacobo Porteiro & Raquel Pérez-Orozco & Miguel Ángel Gómez, 2018. "Technology Evolution in Membrane-Based CCS," Energies, MDPI, vol. 11(11), pages 1-18, November.
    2. Liang, Zhuoran & Tian, Zhan & Sun, Laixiang & Feng, Kuishuang & Zhong, Honglin & Gu, Tingting & Liu, Xiaochen, 2016. "Heat wave, electricity rationing, and trade-offs between environmental gains and economic losses: The example of Shanghai," Applied Energy, Elsevier, vol. 184(C), pages 951-959.
    3. Hyun Sic Park & JunYoung Han & Ju Sung Lee & Kwang-Mo Kim & Hyung Jun Jo & Byoung Ryul Min, 2016. "Comparison of Two Processes Forming CaCO 3 Precipitates by Electrolysis," Energies, MDPI, vol. 9(12), pages 1-8, December.
    4. Schmitt, Stephan & Wissner, Matthias, 2016. "Kapazitätsmechanismen – Internationale Erfahrungen," WIK Discussion Papers 406, WIK Wissenschaftliches Institut für Infrastruktur und Kommunikationsdienste GmbH.

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    Keywords

    CCU; CO2 fixation; CaCO3-(Calcite); electrolysis;
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