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Simulation of Triple-Cation Perovskite Solar Cells: Key Design Factors for Efficiency Promotion

Author

Listed:
  • Tarek I. Alanazi

    (Department of Physics, College of Science, Northern Border University, Arar 73222, Saudi Arabia)

  • Omer I. Eid

    (Department of Physics, College of Science, Northern Border University, Arar 73222, Saudi Arabia
    Department of Physics, Faculty of Science, University of Khartoum, Khartoum 11115, Sudan)

Abstract

Compositional engineering is considered one of the recent interesting techniques used in the field of perovskite solar cells (PSCs). In this method, more than one material was used in a specific cation in the perovskite structure. This work aims to simulate the cesium-containing triple-cation perovskite (TCP) via the SCAPS-1D simulation program with a device structure of ITO/SnO 2 /TCP/Spiro-OMeTAD/Au. First, we studied the effect of interface defects on the PCSs with respect to experimental results and found that when no interface defects occur, the power conversion efficiency (PCE) reaches a value of 22.16% which is higher than the reported PCE, implying that the fabricated cell suffers from the interface defects as a main effect on cell degradation. Incorporating interface defects into the simulation results in a very good match between the experimental and simulated data with a PCE of 17.92%. Further, to provide possible routes to enhance the performance of the solar cell under investigation, impacts of absorber layer thickness, conduction band offset (CBO), surface recombination velocity, and light intensity were explored. In addition, hole transport layer (HTL)-free design was investigated to alleviate the instability issues associated to the organic HTL, leading to a PCE of 18.28%, for a surface velocity of 10 4 cm/s, which is interestingly higher than the initial cell. The provided study reveals the critical role of interface defects and other key design factors and suggests potential solutions to alleviate the subsequent degradation mechanisms, thereby enhancing the overall cell performance.

Suggested Citation

  • Tarek I. Alanazi & Omer I. Eid, 2023. "Simulation of Triple-Cation Perovskite Solar Cells: Key Design Factors for Efficiency Promotion," Energies, MDPI, vol. 16(6), pages 1-14, March.
    • Handle: RePEc:gam:jeners:v:16:y:2023:i:6:p:2717-:d:1097329
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    References listed on IDEAS

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    1. Marwa. S. Salem & Ahmed Shaker & Abdelhalim Zekry & Mohamed Abouelatta & Adwan Alanazi & Mohammad T. Alshammari & Christian Gontand, 2021. "Analysis of Hybrid Hetero-Homo Junction Lead-Free Perovskite Solar Cells by SCAPS Simulator," Energies, MDPI, vol. 14(18), pages 1-22, September.
    2. Kunta Yoshikawa & Hayato Kawasaki & Wataru Yoshida & Toru Irie & Katsunori Konishi & Kunihiro Nakano & Toshihiko Uto & Daisuke Adachi & Masanori Kanematsu & Hisashi Uzu & Kenji Yamamoto, 2017. "Silicon heterojunction solar cell with interdigitated back contacts for a photoconversion efficiency over 26%," Nature Energy, Nature, vol. 2(5), pages 1-8, May.
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