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Biomass Polygeneration System for the Thermal Conversion of Softwood Waste into Hydrogen and Drop-In Biofuels

Author

Listed:
  • Lorenzo Bartolucci

    (Department of Industrial Engineering, University of Rome “Tor Vergata”, Via del Politecnico 1, 00133 Rome, Italy)

  • Enrico Bocci

    (Department of Nuclear, Subnuclear and Radiation Physics, Marconi University, 00193 Rome, Italy)

  • Stefano Cordiner

    (Department of Industrial Engineering, University of Rome “Tor Vergata”, Via del Politecnico 1, 00133 Rome, Italy)

  • Emanuele De Maina

    (Department of Industrial Engineering, University of Rome “Tor Vergata”, Via del Politecnico 1, 00133 Rome, Italy)

  • Francesco Lombardi

    (Department of Civil Engineering and Computer Science Engineering, University of Rome “Tor Vergata”, Via del Politecnico 1, 00133 Rome, Italy)

  • Vera Marcantonio

    (Unit of Process Engineering, Department of Engineering, University “Campus Bio-Medico” di Roma, Via Álvaro Del Portillo 21, 00128 Rome, Italy)

  • Pietro Mele

    (Department of Industrial Engineering, University of Rome “Tor Vergata”, Via del Politecnico 1, 00133 Rome, Italy)

  • Vincenzo Mulone

    (Department of Industrial Engineering, University of Rome “Tor Vergata”, Via del Politecnico 1, 00133 Rome, Italy)

  • Davide Sorino

    (Department of Civil Engineering and Computer Science Engineering, University of Rome “Tor Vergata”, Via del Politecnico 1, 00133 Rome, Italy)

Abstract

In order to keep the +1.5 °C over-temperature, previously predicted with high confidence by IPPC Sixth Assessment, as minimal as feasible, it is more than vital to achieve a low-emission energy system. Polygeneration systems based on thermochemical processes involve biomass conversion in multi-output of bioenergy carriers and chemicals. Due to reduced energy input and input/output diversification, polygeneration energy systems are considered interesting pathways that can increase competitiveness of biomass-derived products. The proposed route of fast pyrolysis, sorption-enhanced biochar gasification and crude bio-oil hydrodeoxygenation to produce drop-in biofuel and hydrogen is examined. Both kinetic and equilibrium approaches were implemented in Aspen Plus to take into account the effect of the major operating parameters on the process performance and then validated against the literature data. Results show how the process integration leads to improved mass conversion yield and increases overall energy efficiency up to 10%-points, reaching the maximum value of 75%. Among the various parameters investigated, pyrolysis temperature influences mainly the products distribution while Steam/Biochar and Sorbent/Biochar affect the energy conversion efficiency.

Suggested Citation

  • Lorenzo Bartolucci & Enrico Bocci & Stefano Cordiner & Emanuele De Maina & Francesco Lombardi & Vera Marcantonio & Pietro Mele & Vincenzo Mulone & Davide Sorino, 2023. "Biomass Polygeneration System for the Thermal Conversion of Softwood Waste into Hydrogen and Drop-In Biofuels," Energies, MDPI, vol. 16(3), pages 1-15, January.
    • Handle: RePEc:gam:jeners:v:16:y:2023:i:3:p:1286-:d:1046518
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    References listed on IDEAS

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    1. Vera Marcantonio & Michael Müller & Enrico Bocci, 2021. "A Review of Hot Gas Cleaning Techniques for Hydrogen Chloride Removal from Biomass-Derived Syngas," Energies, MDPI, vol. 14(20), pages 1-15, October.
    2. Chen, Yu-Kai & Lin, Cheng-Han & Wang, Wei-Cheng, 2020. "The conversion of biomass into renewable jet fuel," Energy, Elsevier, vol. 201(C).
    3. Zahra Echresh Zadeh & Ali Abdulkhani & Basudeb Saha, 2020. "Characterization of Fast Pyrolysis Bio-Oil from Hardwood and Softwood Lignin," Energies, MDPI, vol. 13(4), pages 1-14, February.
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    5. Vera Marcantonio & Enrico Bocci & Danilo Monarca, 2019. "Development of a Chemical Quasi-Equilibrium Model of Biomass Waste Gasification in a Fluidized-Bed Reactor by Using Aspen Plus," Energies, MDPI, vol. 13(1), pages 1-15, December.
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    Cited by:

    1. Matteo Baldelli & Lorenzo Bartolucci & Stefano Cordiner & Giorgio D’Andrea & Emanuele De Maina & Vincenzo Mulone, 2023. "Biomass to H2: Evaluation of the Impact of PV and TES Power Supply on the Performance of an Integrated Bio-Thermo-Chemical Upgrading Process for Wet Residual Biomass," Energies, MDPI, vol. 16(7), pages 1-17, March.

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