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Design of a 1 MW th Pilot Plant for Chemical Looping Gasification of Biogenic Residues

Author

Listed:
  • Falko Marx

    (Institute for Energy Systems & Technology, Technische Universität Darmstadt, Otto-Berndt-Str. 2, 64287 Darmstadt, Germany)

  • Paul Dieringer

    (Institute for Energy Systems & Technology, Technische Universität Darmstadt, Otto-Berndt-Str. 2, 64287 Darmstadt, Germany)

  • Jochen Ströhle

    (Institute for Energy Systems & Technology, Technische Universität Darmstadt, Otto-Berndt-Str. 2, 64287 Darmstadt, Germany)

  • Bernd Epple

    (Institute for Energy Systems & Technology, Technische Universität Darmstadt, Otto-Berndt-Str. 2, 64287 Darmstadt, Germany)

Abstract

Chemical looping gasification (CLG) is a promising process for the thermochemical solid to liquid conversion route using lattice oxygen, provided by a solid oxygen carrier material, to produce a nitrogen free synthesis gas. Recent advances in lab-scale experiments show that CLG with biomass has the possibility to produce a carbon neutral synthesis gas. However, all experiments have been conducted in externally heated units, not enabling autothermal operation. In this study, the modification of an existing pilot plant for demonstrating autothermal operation of CLG is described. Energy and mass balances are calculated using a validated chemical looping combustion process model extended for biomass gasification. Based on six operational cases, adaptations of the pilot plant are designed and changes discussed. A reactor configuration using two circulating fluidized bed reactors with internal solid circulation in the air reactor is proposed and a suitable operating strategy devised. The resulting experimental unit enables a reasonable range of operational parameters within restrictions imposed from autothermal operation.

Suggested Citation

  • Falko Marx & Paul Dieringer & Jochen Ströhle & Bernd Epple, 2021. "Design of a 1 MW th Pilot Plant for Chemical Looping Gasification of Biogenic Residues," Energies, MDPI, vol. 14(9), pages 1-25, April.
    • Handle: RePEc:gam:jeners:v:14:y:2021:i:9:p:2581-:d:547299
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    References listed on IDEAS

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    1. Chen, Liangyong & Bao, Jinhua & Kong, Liang & Combs, Megan & Nikolic, Heather S. & Fan, Zhen & Liu, Kunlei, 2016. "The direct solid-solid reaction between coal char and iron-based oxygen carrier and its contribution to solid-fueled chemical looping combustion," Applied Energy, Elsevier, vol. 184(C), pages 9-18.
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    7. Ohlemüller, Peter & Alobaid, Falah & Gunnarsson, Adrian & Ströhle, Jochen & Epple, Bernd, 2015. "Development of a process model for coal chemical looping combustion and validation against 100kWth tests," Applied Energy, Elsevier, vol. 157(C), pages 433-448.
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    1. Paul Dieringer & Falko Marx & Jochen Ströhle & Bernd Epple, 2023. "System Hydrodynamics of a 1 MW th Dual Circulating Fluidized Bed Chemical Looping Gasifier," Energies, MDPI, vol. 16(15), pages 1-46, July.

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