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Hollow Cd0.9In0.1Se/Cu2MoS4 nanocube S-scheme heterojunction towards high photocatalytic hydrogen production

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  • Peng, Jiaru
  • Han, Yue
  • Ma, Dingxuan
  • Zhao, Ruiyang
  • Han, Jishu
  • Wang, Lei

Abstract

The solar-driven hydrogen production from water splitting using the composite photocatalyst is a potentially efficient strategy to achieve a stable supply of renewable hydrogen energy. Herein, hollow Cd0.9In0.1Se/Cu2MoS4 nanocubes were prepared through hydrothermal and thermal deposition methods. And the optimized Cd0.9In0.1Se/Cu2MoS4 photocatalyst displayed a high hydrogen production rate of 6358.42 μmol g−1 h−1 and great long-term recyclability. The hollow structure of Cu2MoS4 efficiently improved the utilization ratio of visible light. When Cd0.9In0.1Se nanoparticles was modified on the surface of hollow Cu2MoS4 nanocubes, the S-scheme heterojunction was formed and the built-in electric field at the interface was produced. It effectively facilitated the charge separation and transfer and reduced the recombination of photo-generated electrons and holes, thus enhancing the photocatalytic hydrogen production activity. This work provides a new insight for improving photocatalytic hydrogen production performance from the point of view of the hollow structure composite photocatalyst.

Suggested Citation

  • Peng, Jiaru & Han, Yue & Ma, Dingxuan & Zhao, Ruiyang & Han, Jishu & Wang, Lei, 2023. "Hollow Cd0.9In0.1Se/Cu2MoS4 nanocube S-scheme heterojunction towards high photocatalytic hydrogen production," Renewable Energy, Elsevier, vol. 212(C), pages 984-993.
    • Handle: RePEc:eee:renene:v:212:y:2023:i:c:p:984-993
    DOI: 10.1016/j.renene.2023.05.124
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    References listed on IDEAS

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    1. Yimeng Li & Li Yang & Huijie He & Lei Sun & Honglei Wang & Xu Fang & Yanliang Zhao & Daoyuan Zheng & Yu Qi & Zhen Li & Weiqiao Deng, 2022. "In situ photodeposition of platinum clusters on a covalent organic framework for photocatalytic hydrogen production," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    2. Xuehua Wang & Xianghu Wang & Jianfeng Huang & Shaoxiang Li & Alan Meng & Zhenjiang Li, 2021. "Interfacial chemical bond and internal electric field modulated Z-scheme Sv-ZnIn2S4/MoSe2 photocatalyst for efficient hydrogen evolution," Nature Communications, Nature, vol. 12(1), pages 1-11, December.
    3. Xiaowei Shi & Chao Dai & Xin Wang & Jiayue Hu & Junying Zhang & Lingxia Zheng & Liang Mao & Huajun Zheng & Mingshan Zhu, 2022. "Protruding Pt single-sites on hexagonal ZnIn2S4 to accelerate photocatalytic hydrogen evolution," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
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